Phytoremediation is an efficient technique for the reclamation of salt-affected soils by growing plants. The present study aims to evaluate the intercropping of halophyte Atriplex nummularia Lindl. with naturally occurring species (Mimosa caesalpiniifolia Benth, Leucaena leucocephala (Lam.) de Wit and Azadirachta indica A. Juss.) adapted to semiarid regions as a management capable of enhancing the phytoremediation capacity of these species. A field experiment was conducted in a randomized block and contained four replicates. Species were cultivated alone and in association with A. nummularia to evaluate their potential uses in the reclamation of soils. Exchangeable Ca²⁺, Mg²⁺, Na^+, and K⁺, as well as salinity and sodicity variables, were evaluated. The evaluations were performed at 9 and 18 months of plant growth. The results indicated that A. nummularia individualized was the treatment most efficient; with reductions of 80%, 63%, and 84% in electrical conductivity, sodium adsorption ratio, and exchangeable sodium percentage values, respectively at 18 months compared to starting of the experiment. However, the use of A. nummularia and species adapted to the semiarid in association, or even alone, promoted beneficial effects on the soil quality after the establishment of the plants.

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