We present a fixed-lag ensemble Kalman smoother for estimating emissions for a global aerosol transport model from remote sensing observations. We assimilate AERONET AOT and AE as well as MODIS Terra AOT over ocean to estimate the emissions for dust, sea salt and carbon aerosol and the precursor gas SO2. For January 2009, globally dust emission decreases by 26% (to 3,244 Tg/yr), sea salt emission increases by 190% (to 9073 Tg/yr), while carbon emission increases by 45% (to 136 Tg/yr), compared with the standard emissions. Remaining errors in global emissions are estimated at 62% (dust), 18% (sea salt) and 78% (carbons), with the large errors over land mostly due to the sparseness of AERONET observations. The new emissions are verified by comparing a forecast run against independent MODIS Aqua AOT, which shows significant improvement over both ocean and land. This paper confirms the usefulness of remote sensing observations for improving global aerosol modelling.

This study proposed an aerosol characterization process using satellites for severe biomass burning events. In general, these severely hazy cases are labeled as “undecided” or “hazy.” Because atmospheric aerosols are significantly affected by factors such as air quality, global climate change, local environmental risk, and human and biological health, efficient and accurate algorithms for aerosol retrieval are required for global satellite data processing. Our previous classification of aerosol types was based primarily on near-ultraviolet (UV) data, which facilitated subsequent aerosol retrieval. In this study, algorithms for aerosol classification were expanded to events with serious biomass burning aerosols (SBBAs). Once a biomass burning event is identified, the appropriate radiation simulation method can be applied to characterize the SBBAs. The second-generation global imager (SGLI) on board the Japanese mission JAXA/Global Change Observation Mission-Climate contains 19 channels, including red (674 nm) and near-infrared (869 nm) polarization channels with a high resolution of 1 km. Using the large-scale wildfires in Kalimantan, Indonesia in 2019 as an example, the complementarity between the polarization information and the nonpolarized radiance measurements from the SGLI was demonstrated to be effective in radiation simulations for biomass burning aerosol retrieval. The retrieved results were verified using NASA/AERONET ground-based measurements, and then compared against JAXA/SGLI/L2-version-1 products, and JMA/Himawari-8/AHI observations.

The severity of wildfires is increasing globally. In this study, we used data from the Global Change Observation Mission-Climate/Second-generation Global Imager (GCOM-C/SGLI) to characterize the biomass burning aerosols that are generated by large-scale wildfires. We used data from the September 2020 wildfires in western North America. The target area had a complex topography, comprising a basin among high mountains along a coastal region. The SGLI was essential for dealing with the complex topographical changes in terrain that we encountered, as it contains 19 polarization channels ranging from near ultraviolet (380 nm and 412 nm) to thermal infrared (red at 674 nm and near-infrared at 869 nm) and has a fine spatial resolution (1 km). The SGLI also proved to be efficient in the radiative transfer simulations of severe wildfires through the mutual use of polarization and radiance. We used a regional numerical model SCALE (Scalable Computing for Advanced Library and Environment) to account for variations in meteorological conditions and/or topography. Ground-based aerosol measurements in the target area were sourced from the National Aeronautics and Space Administration-Aerosol Robotic Network; currently, official satellite products typically do not provide the aerosol properties for very optically thick cases of wildfires. This paper used satellite observations, ground-based observations, and a meteorological model to define an algorithm for retrieving the aerosol properties caused by severe wildfire events.

The NASA/AErosol RObotic NETwork field campaign Distributed Regional Aerosol Gridded Observation Networks/Joint work to the AerosoL Properties and Process Simulations was conducted from March 2020 to May 2021 in Nagano, Japan. Twelve sun photometers were installed around Nagano prefecture. The effects of topography on aerosols were studied using observations and simulations. In this study, a regional chemical transport model (SCALE‐Chem) was employed. Three numerical experiments were conducted: E1 (control experiment), E2 (E1 without topography), and E3 (E1 with removal of all anthropogenic emissions over Nagano prefecture). In E2, the terrain effect was not considered; the difference between E1 and E2 indicated the influence of mountains. The differences between E1 and E3 evaluate the local emission effect. In some cases, the mountainous terrain seemed to have suppressed aerosol inflow (i.e., reduced aerosol concentration), while in other cases, the mountains contributed to aerosol retention on days when aerosols tended to accumulate in mountain basins due to local emissions. Thus, while mountains prevent the inflow of aerosols from outside, they also contribute to increased aerosol concentration in the basin. Naturally, more significant effects are produced by meteorological conditions and the presence or absence of transboundary pollution from the outside. From observations and model simulations, we found that the aerosol concentration was not high around the J‐ALPS site because of the mountain effect that prevents advection from the outside, even when transboundary pollution was observed in Japan in March 2020.

It is well known that the aerosol distribution in Asia is complex due to both the increasing emissions of the anthropogenic aerosols associated with economic growth and the behavior of natural dusts. Therefore, detailed observations of atmospheric particles in Asian urban cities are important. In this work, we focus on the spatial and temporal variations of atmospheric particles around Higashi-Osaka in Japan. Higashi-Osaka is located in the eastern part of Osaka, the second-largest city in Japan, and is famous for small- and medium-sized manufacturing enterprises. For this study, we placed various ground measurement devices around the Higashi-Osaka campus of Kinki University including a Cimel sunphotometer supported by NASA/AERONET (Aerosol robotics network), suspended particulate matter (SPM) sampler and LIDAR (light detection and ranging). Individual particle analyses with a SEM (scanning electron microscope)/EDX (energy-dispersive X-ray analyzer) show the temporal variations of particle properties, such as size, shape and components, during a dust event on 21 March 2010. The simultaneous measurement using a portable sun photometer with AERONET was conducted from April to November 2011. A comparison of the data at each site and the combination of the observed LIDAR data and model simulations indicate the difference in the transportation processes between dust and anthropogenic particles. We suppose this difference is attributed to the differences in the vertical aerosol profiles, where one aerosol is transported over Mount Ikoma and the other is blocked by it.

Increasing emission of anthropogenic particles is causing heavy air pollution. This work intends to analyze the air pollution in greater metropolitan area of Asia and its influence on the environment. We focus on Osaka in Japan because our group has been monitoring suspended particulate matter (PM) at Osaka/AERONET since 2004. PM is usually used as an indicator of air quality, because high PM concentrations can degrade air quality. Osaka is the second largest metropolitan region of Japan and its air is significantly polluted by anthropogenic particles emitted from vehicles and industry. In this study, seasonal variation of air pollutants in Osaka is investigated using ground observations such as PM sampling, AERONET photometry, and numerical model simulation. Results indicate that PM concentrations are high during spring and summer because of yellow dust events and photochemical reactions, respectively. In addition, the impact of anthropogenic PM around Osaka is significant in summer.