The molecular high-order-harmonic generation (molecular HHG) of HeH is investigated by numerical integration of the non-Born-Oppenheimer time-dependent Schrödinger equation. The results show that multichannel interference plays a very important role in the process of asymmetric molecular high-order-harmonic generation. By means of the classical returning kinetic energy map and the time-frequency distribution, the mechanism of molecular HHG for HeH is discussed in detail. Further studies show that asymmetric molecular harmonic emission is very sensitive to the nuclear signatures, i.e., the initial vibrational state and the isotopic effect. Besides, the electron-nuclear probability density distributions are calculated to better understand the process of the asymmetric molecular HHG, from which the electron-nuclear dynamics can be revealed.
The multichannel recombination in high-order-harmonic generation (HHG) from the asymmetric molecular ion HeH has been investigated by numerically solving the time-dependent Schrödinger equation based on the non-Born-Oppenheimer approximation. In this paper, not only has the physical image in harmonic emission from the asymmetric molecular ion been established, but also the distinguishing of recombination channels has been achieved. Moreover, our quantitative calculations show that the recombination channels from different electronic states make different contributions to HHG. Furthermore, by means of the time-frequency maps, electron-nuclear probability density distributions, and the laser dressed state picture, the physical mechanism of the multichannel recombination has been revealed.
Quantum key distribution (QKD) can provide information-theoretically secure keys for two parties of legitimate communication, and information reconciliation, as an indispensable component of QKD systems, can correct errors present in raw keys based on error-correcting codes. In this paper, we first describe the basic knowledge of information reconciliation and its impact on continuous variable QKD. Then we introduce the information schemes and the corresponding error correction codes employed. Next, we introduce the rate-compatible codes, the hardware acceleration of the reconciliation algorithm, the research progress of information reconciliation, and its application in continuous variable QKD. Finally, we discuss the future challenges and conclude.
27 June 2024 in Journal of Colloid and Interface Science
The molecular multiple rescattering processes have been theoretically investigated via solving the time-dependent Schrödinger equation. Not only has the physical model been established, but also the related rescatterings originating from recombination with parent nucleus and with neighboring nucleus have been distinguished. Moreover, it has shown that the rescatterings originating from recombination with parent nucleus are similar with those atomic rescatterings, while those rescatterings from recombination with neighboring nucleus both before and after reversing the direction of the laser field are more sensitive to the internuclear distance. With time-frequency distribution and classical electron dynamics, the underlying mechanisms are revealed.
The Co3S4@NiCo-LDH/NF nanocomposite exhibits outstanding electrocatalytic performances toward both the HER and OER at high current densities, along with a remarkable durability.