Using natural fibers as reinforcement in polymer matrix composites necessitates evaluating the latter under different modes of solicitation. This allows extracting its material properties for engineering design and research purposes. The main objective of the study is preparing a consistent set of material properties for unidirectional flax fiber-reinforced epoxy composite with defined composition and basic configuration. These data are prerequisites for growing researches on flax fiber-reinforced epoxy composites, especially for numerical analysis purposes using the finite element method. In this work, partially green unidirectional-flax fiber-reinforced epoxy composites are tested for physical and mechanical properties and studied for their failure modes. Tension, compression, flexion, and shear properties, as well as physical properties like density, specific heat capacity and thermal diffusivity, are evaluated according to ASTM standard test methods. Flax fibers, which are composites by themselves, come in bundles in the composites and demonstrate a complex behavior. Therefore, a fractographic analysis has been conducted to understand the macro and microscale failure mechanisms to correlate them with the material properties. The results are in good agreement with those of the literature, when available, but they mainly show the specific behavior of unidirectional-flax composites subject to different solicitation modes, especially compression and direct shear modes evaluated this way for the first time for unidirectional-flax fiber-reinforced epoxy composite. They cover most of the data required for engineering design and numerical analysis by methods like finite element method, particularly for simulating the machining process of flax fiber-reinforced epoxy composite in the ongoing works.

Having environmental and economic advantages, flax fibers have been recognized as a potential replacement for glass fibers as reinforcement in epoxy composites for various applications. Its widening applications require employing failure criteria and analysis methods for engineering design, analysis, and optimization of this material. Among different failure modes, delamination is known as one of the earliest ones in laminated composites and needs to be studied in detail. However, the delamination characteristics of unidirectional (UD) flax/epoxy composites in pure Mode I has rarely been addressed, while Mode II and Mixed-mode I/II have never been addressed before. This work studies and evaluates the interlaminar fracture toughness and delamination behavior of UD flax/epoxy composite under Mode I, Mode II, and Mixed-mode I/II loading. The composites were tested following corresponding ASTM standards and fulfilled all the requirements. The interlaminar fracture toughness of the composite were determined and validated based on the specific characteristics of natural fibers. Considering the variation in the composite structure configuration and its effects, the results of interlaminar fracture toughness fit in the range of those reported for similar composites in the literature and provide a basis for the material properties of this composite.