Nanoscale thin films are widely implemented across a plethora of technological and scientific areas, and form the basis for many advancements that have driven human progress, owing to the high degree of functional tunability based on the chemical composition. Pulsed laser deposition is one of the multiple physical vapour deposition routes to fabricate thin films, employing laser energy to eject material from a target in the form of a plasma. A substrate, commonly a single-crystal oxide, is placed in the path of the plume and acts as a template for the arriving species from the target to coalesce and self-assemble into a thin film. This technique is tremendously useful to produce crystalline films, due to the wide range of atmospheric conditions and the extent of possible chemical complexity of the target. However, this flexibility results in a high degree of complexity, oftentimes requiring rigorous optimisation of the growth parameters to achieve high quality crystalline films with desired composition. In this tutorial review, we aim to reduce the complexity and the barrier to entry for the controlled growth of complex oxides by pulsed laser deposition. We present an overview of the fundamental and practical aspects of pulsed laser deposition, discuss the consequences of tailoring the growth parameters on the thin film properties, and describe in situ monitoring techniques that are useful in gaining a deeper understanding of the properties of the resultant films. Particular emphasis is placed on the general relationships between the growth parameters and the consequent structural, chemical and functional properties of the thin films. In the final section, we discuss the open questions within the field and possible directions to further expand the utility of pulsed laser deposition.

Many in-memory computing frameworks demand electronic devices with specific switching characteristics to achieve the desired level of computational complexity. Existing memristive devices cannot be reconfigured to meet the diverse volatile and non-volatile switching requirements, and hence rely on tailored material designs specific to the targeted application, limiting their universality. “Reconfigurable memristors” that combine both ionic diffusive and drift mechanisms could address these limitations, but they remain elusive. Here we present a reconfigurable halide perovskite nanocrystal memristor that achieves on-demand switching between diffusive/volatile and drift/non-volatile modes by controllable electrochemical reactions. Judicious selection of the perovskite nanocrystals and organic capping ligands enable state-of-the-art endurance performances in both modes – volatile (2 × 10⁶ cycles) and non-volatile (5.6 × 10³ cycles). We demonstrate the relevance of such proof-of-concept perovskite devices on a benchmark reservoir network with volatile recurrent and non-volatile readout layers based on 19,900 measurements across 25 dynamically-configured devices.

LASER ablation propulsion (LAP) is a major new electric propulsion concept with a 35-year history. In LAP, an intense\ud laser beam [pulsed or continuous wave (CW)] strikes a condensedmatter surface (solid or liquid) and produces a jet of vapor or plasma.\ud Just as in a chemical rocket, thrust is produced by the resulting reaction force on the surface. Spacecraft and other objects can be propelled in this way. In some circumstances, there are advantages for this technique compared with other chemical and electric propulsion schemes. It is difficult to make a performance metric for LAP, because only a few of its applications are beyond the research phase and because it can be applied in widely different circumstances that would require entirely different metrics. These applications range from milliwatt-average-power satellite attitude-correction\ud thrusters through kilowatt-average-power systems for reentering near-Earth space debris and megawatt-to-gigawatt systems for direct launch to lowEarth orbit (LEO). \ud We assume an electric laser rather than a gas-dynamic or\ud chemical laser driving the ablation, to emphasize the performance as an electric thruster. How is it possible for moderate laser electrical efficiency to givevery high electrical efficiency? Because laser energy can be used to drive an exothermic reaction in the target material controlled by the laser input, and electrical efficiency only measures the ratio of exhaust power to electrical power. This distinction may\ud seem artificial, but electrical efficiency is a key parameter for space applications, in which electrical power is at a premium.\ud The laser system involved in LAP may be remote from the\ud propelled object (on another spacecraft or planet-based), for\ud example, in laser-induced space-debris reentry or payload launch to low planetary orbit. In other applications (e.g., the laser–plasma microthruster that we will describe), a lightweight laser is part of the propulsion engine onboard the spacecraft

Photoelectrochemical (PEC) water splitting is recognized as a sustainable strategy for hydrogen generation due to its abundant hydrogen source, utilization of inexhaustible solar energy, high‐purity product, and environment‐friendly process. To actualize a practical PEC water splitting, it is paramount to develop efficient, stable, safe, and low‐cost photoelectrode materials. Recently, graphitic carbon nitride (g‐C₃N₄) has aroused a great interest in the new generation photoelectrode materials because of its unique features, such as suitable band structure for water splitting, a certain range of visible light absorption, nontoxicity, and good stability. Some inherent defects of g‐C₃N₄, however, seriously impair further improvement on PEC performance, including low electronic conductivity, high recombination rate of photogenerated charges, and limited visible light absorption at long wavelength range. Construction of g‐C₃N₄‐based nanosized heteroarrays as photoelectrodes has been regarded as a promising strategy to circumvent these inherent limitations and achieve the high‐performance PEC water splitting due to the accelerated exciton separation and the reduced combination of photogenerated electrons/holes. Herein, we summarize in detail the latest progress of g‐C₃N₄‐based nanosized heteroarrays in PEC water‐splitting photoelectrodes. Firstly, the unique advantages of this type of photoelectrodes, including the highly ordered nanoarray architectures and the heterojunctions, are highlighted. Then, different g‐C₃N₄‐based nanosized heteroarrays are comprehensively discussed, in terms of their fabrication methods, PEC capacities, and mechanisms, etc. To conclude, the key challenges and possible solutions for future development on g‐C₃N₄‐based nanosized heteroarray photoelectrodes are discussed.

Fabrication of a polymer light-emitting device was achieved by a laser forward transfer technique using the decomposition of a thin triazene polymer film by a XeCl excimer laser. The dry deposition process allows transfer of a bilayer consisting of the electroluminescent polymer poly[2-methoxy-5-(2-ethylhexyloxy)-1,4-phenylenevinylene] covered with an aluminum electrode onto a receiver substrate. The soft transfer results in laterally well resolved pixels $(\approx 500\mu \mathrm{m})$ , whose fluorescence as well as electroluminescence spectra remain unaltered. The rectifying and smooth current-voltage characteristics add to the merits of this laser-based transfer method that opens up the possibility of direct-writing heat- and UV-sensitive materials.