We have experimentally achieved spin polarization by a lateral current in a single nonmagnetic semiconductor heterojunction. The effect does not require an applied magnetic field. The current-induced spin orientation can be seen as the inverse of the circular photogalvanic effect (also often referred to as spin photocurrents): the nonequilibrium spin changes its sign as the current reverses.
The excellent optoelectronic performance of lead halide perovskites has generated great interest in their fundamental properties. The polar nature of the perovskite lattice means that electron-lattice coupling is governed by the Fröhlich interaction. Still, considerable ambiguity exists regarding the phonon modes that participate in this crucial mechanism. Here, we use multiphonon Raman scattering and THz time-domain spectroscopy to investigate Fröhlich coupling in CsPbBr3. We identify a longitudinal optical phonon mode that dominates the interaction, and surmise that this mode effectively defines exciton-phonon scattering in CsPbBr3, and possibly similar materials. It is additionally revealed that the observed strength of the Fröhlich interaction is significantly higher than the expected intrinsic value for CsPbBr3, and is likely enhanced by carrier localization in the colloidal perovskite nanocrystals. Our experiments also unearthed a dipole-related dielectric relaxation mechanism which may impact transport properties.
The electron g factor in an ensemble of InAs/InP quantum dots with emission wavelengths around 1.4 μm is measured using time-resolved pump-probe Faraday rotation spectroscopy in different magnetic field orientations. Thereby, we can extend recent single dot photoluminescence measurements significantly towards lower optical transition energies through 0.86 eV. This allows us to obtain detailed insight into the dispersion of the recently discovered g factor anisotropy in these infrared emitting quantum dots. We find with decreasing transition energy over a range of 50 meV a strong enhancement of the g factor difference between magnetic field normal and along the dot growth axis, namely, from 1 to 1.7. We argue that the g factor cannot be solely determined by the confinement energy, but the dot asymmetry underlying this anisotropy therefore has to increase with increasing dot size.
Due to their small sizes and low threshold, nanolasers play a pivotal role in the field of low-energy scalable photonic technologies. High-speed modulation of nanolasers is needed for their application in data communication, but its implementation has been hampered by the small scales involved, leading to large electrical parasitics. Here we experimentally demonstrate the proof-of-principle of a novel modulation technique, namely, mode-field switching, which unlocks the control of the laser operation via the modulation of the electromagnetic field. In particular, we show that stimulated emission can be inhibited by switching the lasing mode from bright to dark in a three-coupled cavity system. The experimental results are in good agreement with a model that combines coupled-mode theory and rate equations. Using this model, we show that time-dependent detuning schemes enable storage and release of energy under the form of short pulses, placing mode-field switching among the techniques for laser modulation and pulse generation. This scheme is general and can be implemented in every platform displaying coupled and tuneable resonances.
The paper reports optical orientation experiments performed in the narrow GaAs/AlGaAs quantum wells doped with Mn. We experimentally demonstrate a control over the spin polarization by means of the optical orientation via the impurity-to-band excitation and observe a sign inversion of the luminescence polarization depending on the pump power. The factor of a hole localized on the Mn acceptor in the quantum well was also found to be considerably modified from its bulk value due to the quantum confinement effect. This finding shows the importance of the local environment on magnetic properties of the dopants in semiconductor nanostructures.