The intelligent electronic devices have urgent demands for electromagnetic interference (EMI) shielding films with excellent heat dissipation capability. However, it is challenging to obtain excellent EMI shielding and thermal conductivity performances simultaneously. Herein, inspired by mille-feuille structure, the multifunctional EMI shielding films developed by a layer-by-layer self-assembly and hot-pressing strategy. The ingenious introduction of silver nanoparticles (AgNPs) with large specific surface area and highly conductive into the network formed by TEMPO-oxidized cellulose nanofibrils (TOCNFs) with large aspect ratio to form the TOCNFs/AgNPs. And the graphene nanoplates (GNPs) with high conductivity loss distributed alternately with TOCNFs/AgNPs to construct mille-feuille structure, which had highly efficient conductive network, complete thermally conduction pathway and rich heterogeneous interfaces. Consequently, the designed films presented high electrical conductivity of 8520 S/cm, superb EMI effectiveness (SE) of 98.05 dB, and excellent thermal conductivity of 18.82 W/(m·K). Furthermore, the films possessed outstanding Joule heating performances with low voltages, including high heating temperature (100 °C), fast response time (< 20 s), and impressive heating stability and reliability. Thus, such high-performance EMI shielding films with fascinating thermal conductivity and Joule heating performances have substantial application in flexible electronics, electromagnetic waves shielding and thermal management.

CQDs are a type of fluorescent nanocarbon material that possess excellent optical properties. They have a wide range of raw material sources, making them a versatile option for various applications. The use of fluorescent materials to enhance the solar energy capture capacity of chloroplasts has the potential to significantly improve natural photosynthesis. CQDs and N-CQDs were prepared from natural Salix wood powder using a simple, green, and environmentally friendly hydrothermal method. These materials can effectively capture ultraviolet (UV) light and were used for photosynthesis to enable chloroplasts to utilize UV light that cannot be absorbed by them. The chlorophyll content of leaves treated with CQDs and N-CQDs increased, with the N-CQDs 25 mg/L treated group showing a 35.6% increase compared to the untreated group. Additionally, the treatment of CQDs and N-CQDs positively affected the transfer of electrons from photosystem II, further enhancing photosynthetic activity. This study presents ideas for expanding the use of solar energy, optimizing the photosynthesis charge transfer pathway, and improving solar energy conversion efficiency.

The lightweight multilayer-structured electromagnetic interference shielding composite coatings with controllable electromagnetic gradient on wood surface were prepared via a simple multiple electroless copper–nickel (Cu–Ni) approach. The surface morphology, conductivity, hydrophobicity property and electromagnetic shielding effectiveness of the composite coatings were investigated. The surface roughness and conductivity of the composite coatings were enhanced with the increase in the number of depositions. The surface morphology demonstrated that the roughness was decreased with the process of multiple electroless. The coatings were compact and homogeneous as the deposition run was three. Here, the Sa (Sa illustrated Surface Roughness) value of coatings was 4.497 μm. The ideal conductivity of composite coatings can be obtained as the number of depositions was four. Electromagnetic shielding effectiveness reached average 90.69 dB in the frequency range from 300 kHz to 2.0 GHz. This study provides a new pathway for fabricating lightweight multilayer-structured electromagnetic interference shielding with controllable electromagnetic gradient and hydrophobic composite coatings-based wood.

With the aggravation of electromagnetic radiation pollution, it is urgent to develop green, lightweight, ultra-thin and high-performance electromagnetic interference shielding materials to eliminate unnecessary electromagnetic interference; however, the construction of wood-based high-performance electromagnetic shielding materials by simple methods remains a challenge. Based on the layer-by-layer assembly strategy, a lightweight Ni/Wood/Ni composite (NWNC) with an interlayer structure was constructed by a simple electroless plating method using natural wood as a substrate for electromagnetic interference shielding. The synthesized NWNC has a smooth surface, and its minimum surface roughness is only 8.34 μm. After 15 min of electroless nickel plating, the contact angle (CA) of NWNC with an ultra-thin nickel layer (65 μm) was 118.3°. When the thickness of the nickel layer is only 0.102 mm, the conductivity can reach 1659.59 S/cm when the three electroless nickel plating time is 15 min. In the L-band, the electromagnetic shielding effectiveness can reach 94.1 dB after three times electroless nickel plating for 20 min. This is due to the conductive loss, magnetic loss and interface polarization loss generated by the electromagnetic network constructed by the nickel layer, which makes the composite material produce an electromagnetic shielding mechanism dominated by absorption. The L-band absorption efficiency can reach 39.01 dB, and due to the porous structure of the original wood, the multiple reflection and absorption inside the wood further lose the electromagnetic wave. This study provides a low-cost and simple method for the design of light, ultra-thin and efficient controllable wood-based electromagnetic shielding materials and has broad application prospects in the fields of construction and aerospace.