Carbonaceous aerosol, one of the major components of atmospheric aerosols, significantly affects haze episodes, climate change, and human health. Northeastern China suffers severe air pollution, especially in some periods (e.g., the Spring Festival). However, studies on carbonaceous aerosols in typical northeast industrial cities (i.e., Changchun) are rare, limiting further comprehension of the atmospheric haze formation. In this study, we monitored the concentrations of carbonaceous aerosols (i.e., OC and EC) in Changchun during the Lunar New Year of 2018 (i.e., from Lunar 20 December to Lunar 20 January), and analyzed the temporal variation and source contributions via the HYbrid-Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model with the potential source contribution factor weights (PSCF) method. The daily concentrations of OC and EC were 9.00 ± 2.81 and 1.57 ± 0.46 µg m⁻³, respectively, and were significantly lower at nighttime than at the day during the Spring Festival. The concentrations during the major period (i.e., OC: 8.13 ± 2.93 µg m⁻³; EC: 1.47 ± 0.47 µg m⁻³ in festival days), including the Lunar Little New Year; the Lunar New Year’s Eve; New Year’s Day; Lunar 5 January, and the Spring Lantern Festival, were mainly from the northwestward with the wind speed of 4–6 m/s being lower than that of normal period (OC: 9.87 ± 2.46 µg m⁻³; EC: 1.67 ± 0.44 µg m⁻³) from the southeastward with a wind speed of 6–7 m/s. The direction of the airflow trajectory was mainly in local, northwestward, and northward, carrying particulate matter and gaseous pollutants. In major period, the daily concentration of atmospheric pollutants presented a bimodal trend, with peaks appearing regularly from 11:00 a.m. to 12:00 p.m. and 5:00 p.m. 10:00 p.m., which might be related to traffic, cooking, and firecrackers. The OC/EC was greater than 2 during the whole period, indicating the generation of secondary organic aerosols (i.e., SOC). This study was essential to understand the formation mechanisms of severe pollution episodes and develop control measures for the industrial cities of Northeast China during the Spring Festival.

Harbin is a northmost megacity in the cold regions of China and experiences severe PM_2.5 pollution. However, comprehensive investigations for severe haze formation are few. In this study, we simultaneously measured aerosol composition in real time to assess the sources apportionment, regional transport and its interaction with meteorology from 1 October 2018 to 1 May 2019 by using the single particle aerosol mass spectrometer (SPAMS). The daily average PM_2.5 concentration was 51.21 µg/m³ with the hourly maximum of 900.45 µg/m³. Winter coal combustion was the largest source of PM_2.5 aerosols during this period. Open straw burning from surrounding and adjacent areas by short-distance transport could aggravate air quality deterioration in Harbin. Three extreme haze events (i.e., Ep1, Ep2 and Ep3) were observed in this study, showing the typical characteristics of local winter pollution. The pollutants of PM_2.5 and SO₂ emitted from coal combustion played an important role in haze episode during Ep1, whereas Ep2 was caused by the joint effect of coal combustion and straw burning. Ep3 was characterized by long-distance transport of windblown dust from southeast Inner Mongolia and northwest Harbin. Real-time source apportionment of fine particulate matter highlights the importance of joint control of coal and straw burning from the surrounding cities of Harbin.

Open-field crop residue burning (OCRB) is a widespread agricultural practice with significant impacts on regional environments and public health. The effective management of OCRB remains a challenging task that requires timely access to various forms of monitored and forecasted information. Addressing this worldwide need, an open-source platform named AgriFireInfo v1.0, which is specifically tailored to monitoring and regulating regional OCRB activities, was developed. This technical note thoroughly illustrates the platform’s architecture, major modules, and visualization processes. Through AgriFireInfo v1.0, government agencies can access timely information about the spatial distribution of fire spots and emissions as well as meteorological conditions and air quality status. AgriFireInfo v1.0 also introduces an innovative Prevention Alarming Index, designed to identify regions prone to OCRB and promote comprehensive crop residue utilization. Furthermore, it offers the burning window and crop residue yields for controlled OCRB activities and can be used to analyze shifts in farmers’ burning behaviors and intensities. Future enhancements will focus on supplying holistic information on the burning windows and burning amounts of crop residues to further facilitate refined controlled burning activities and optimize decision-making processes. The flexibility and scalability of this platform can potentially allow users to easily customize and apply it to other regions or countries.

The emissions of reactive nitrogen (Nr) from cropland links the pedosphere and atmosphere, playing a crucial role in the Earth’s nitrogen cycle while significantly impacting regional climate change, air quality, and human health. Among various Nr species, nitrogen oxide (NO) and nitrous acid (HONO) have garnered increasing attention as critical precursors to surface ozone (O₃) formation due to their participation in photochemical reactions. While most studies focus on Nr emissions from soils, the specific contributions of cropland Nr emissions considering planting activities to regional O₃ pollution remain insufficiently investigated. This study applied the enhanced process-based agroecological model (FEST-C*) coupled with the air quality (CMAQ) model to quantify cropland Nr emissions and assess their contributions to regional O₃ formation across China in June 2020. The simulated results indicated that the fertilizer-induced total Nr emission was estimated at 1.26 Tg in China, with NO emissions accounting for 0.66 Tg and HONO emissions for 0.60 Tg. North China was identified as a hotspot for cropland Nr emissions, contributing 43% of the national total. The peak emissions of cropland NO and HONO occurred in June, with emissions of 169 and 192 Gg, respectively. Cropland Nr emissions contributed approximately 8% to the national monthly mean MDA8 O₃ concentration, with localized enhancements exceeding 9% in agricultural hotspots in summer. North China experienced the largest MDA8 O₃ increase, reaching 11.71 μg m⁻³, primarily due to intensive fertilizer application and favorable climatic conditions. Conversely, reductions in nighttime hourly O₃ concentrations were observed in southern North China and northern Southeast China due to the rapid titration of O₃ via NO. In this study, the contributions of cropland Nr emissions to MDA8 O₃ concentrations across different regions of China have been further constrained. Incorporating cropland Nr emissions into the CMAQ model improved simulation accuracy and reduced mean biases in MDA8 O₃ predictions. This study offers a detailed quantification of the contribution of cropland Nr emissions in regional ozone formation across China and highlights the critical need to address cropland NO and HONO emissions in air quality management strategies.