The electron paramagnetic resonance (EPR) signal in the mixed valence perovskite was investigated in the paramagnetic regime for O and O isotope substituted compounds. The characteristic differences observed in EPR intensity and linewidth for the two isotope samples can be explained by a model in which a bottlenecked spin relaxation takes place from the exchange-coupled constituent ions via the Jahn-Teller ions to the lattice. For the ferromagnetic exchange energy exhibits a oxygen isotope effect of . The observed isotope effects suggest the presence of Jahn-Teller polarons in these materials.
In its orthorhombic Td polymorph, MoTe2 is a type-II Weyl semimetal, where the Weyl fermions emerge at the boundary between electron and hole pockets. Non-saturating magnetoresistance and superconductivity were also observed in Td-MoTe2. Understanding the superconductivity in Td-MoTe2, which was proposed to be topologically non-trivial, is of eminent interest. Here, we report high-pressure muon-spin rotation experiments probing the temperature-dependent magnetic penetration depth in Td-MoTe2. A substantial increase of the superfluid density and a linear scaling with the superconducting critical temperature Tc is observed under pressure. Moreover, the superconducting order parameter in Td-MoTe2 is determined to have 2-gap s-wave symmetry. We also exclude time-reversal symmetry breaking in the superconducting state with zero-field μSR experiments. Considering the strong suppression of Tc in MoTe2 by disorder, we suggest that topologically non-trivial s+− state is more likely to be realized in MoTe2 than the topologically trivial s++ state.
The in-plane magnetic field penetration depth () in single-crystal was investigated by muon-spin rotation (). The temperature dependence of has an inflection point around 10–15 K, suggesting the presence of two superconducting gaps: a large gap () with -wave and a small gap () with -wave symmetry. The zero-temperature values of the gaps at were found to be and .
Recent EPR and susceptibility measurements in support the existence of a bottleneck EPR regime up to 1000 K quantitatively. The EPR linewidth and electrical conductivity follow the same temperature dependence in the range of 250 to 650 K predicted by the small polaron hopping model. This indicates that spin-lattice relaxation in manganates is due to the relaxation of spins of Jahn-Teller polarons to the lattice.
The in-plane magnetic penetration depth of the iron selenide superconductor with the nominal composition was studied by means of muon-spin rotation. The measurements of are inconsistent with a simple isotropic -wave type of the order parameter but are rather in favor of two-gap and anisotropic -wave order parameter symmetries, thus implying that the superconducting energy gap in contains no nodes.