We control the electronic structure of the silicon-vacancy (SiV) color-center in diamond by changing its static strain environment with a nano-electro-mechanical system. This allows deterministic and local tuning of SiV optical and spin transition frequencies over a wide range, an essential step towards multiqubit networks. In the process, we infer the strain Hamiltonian of the SiV revealing large strain susceptibilities of order 1 PHz/strain for the electronic orbital states. We identify regimes where the spin-orbit interaction results in a large strain susceptibility of order 100 THz/strain for spin transitions, and propose an experiment where the SiV spin is strongly coupled to a nanomechanical resonator.

Concerted efforts are underway to establish an infrastructure for a global quantum Internet to realise a spectrum of quantum technologies. This will enable more precise sensors, secure communications, and faster data processing. Quantum communications are a front‐runner with quantum networks already implemented in several metropolitan areas. A number of recent proposals have modelled the use of space segments to overcome range limitations of purely terrestrial networks. Rapid progress in the design of quantum devices have enabled their deployment in space for in‐orbit demonstrations. We review developments in this emerging area of space‐based quantum technologies and provide a roadmap of key milestones towards a complete, global quantum networked landscape. Small satellites hold increasing promise to provide a cost effective coverage required to realise the quantum Internet. The state of art in small satellite missions is reviewed and the most current in‐field demonstrations of quantum cryptography are collated. The important challenges in space quantum technologies that must be overcome and recent efforts to mitigate their effects are summarised. A perspective on future developments that would improve the performance of space quantum communications is included. The authors conclude with a discussion on fundamental physics experiments that could take advantage of a global, space‐based quantum network.

We demonstrate the first solid-state spin-wave optical quantum memory with on-demand read-out. Using the full atomic frequency comb scheme in a ${\mathrm{Pr}}^{3+}:{\mathrm{Y}}_2{\mathrm{SiO}}_5$ crystal, we store weak coherent pulses at the single-photon level with a signal-to-noise ratio $>10$. Narrow-band spectral filtering based on spectral hole burning in a second ${\mathrm{Pr}}^{3+}:{\mathrm{Y}}_2{\mathrm{SiO}}_5$ crystal is used to filter out the excess noise created by control pulses to reach an unconditional noise level of $(2.0\pm 0.3)\times {10}^{-3}$ photons per pulse. We also report spin-wave storage of photonic time-bin qubits with conditional fidelities higher than achievable by a measure and prepare strategy, demonstrating that the spin-wave memory operates in the quantum regime. This makes our device the first demonstration of a quantum memory for time-bin qubits, with on-demand read-out of the stored quantum information. These results represent an important step for the use of solid-state quantum memories in scalable quantum networks.

We report on the quantum storage and retrieval of photonic polarization quantum bits onto and out of a solid state storage device. The qubits are implemented with weak coherent states at the single photon level, and are stored for a predetermined time of 500~ns in a praseodymium doped crystal with a storage and retrieval efficiency of 10%, using the atomic frequency comb scheme. We characterize the storage by using quantum state tomography, and find that the average conditional fidelity of the retrieved qubits exceeds 95% for a mean photon number $\mu${}=0.4. This is significantly higher than a classical benchmark, taking into account the Poissonian statistics and finite memory efficiency, which proves that our crystal functions as a quantum storage device for polarization qubits. These results extend the storage capabilities of solid state quantum light matter interfaces to polarization encoding, which is widely used in quantum information science.

The silicon-vacancy center in diamond offers attractive opportunities in quantum photonics due to its favorable optical properties and optically addressable electronic spin. Here, we combine both to achieve all-optical coherent control of its spin states. We utilize this method to explore spin dephasing effects in an impurity-rich sample beyond the limit of phonon-induced decoherence: Employing Ramsey and Hahn-echo techniques at temperatures down to 40 mK we identify resonant coupling to a substitutional nitrogen spin bath as limiting decoherence source for the electron spin.

Global-scale quantum communication links will form the backbone of the quantum internet. However, exponential loss in optical fibres precludes any realistic application beyond few hundred kilometres. Quantum repeaters and space-based systems offer solutions to overcome this limitation. Here, we analyse the use of quantum memory (QM)-equipped satellites for quantum communication focussing on global range repeaters and memory-assisted (MA-) QKD, where QMs help increase the key rate by synchronising otherwise probabilistic detection events. We demonstrate that satellites equipped with QMs provide three orders of magnitude faster entanglement distribution rates than existing protocols based on fibre-based repeaters or space systems without QMs. We analyse how entanglement distribution performance depends on memory characteristics, determine benchmarks to assess the performance of different tasks and propose various architectures for light-matter interfaces. Our work provides a roadmap to realise unconditionally secure quantum communications over global distances with near-term technologies.