At stations on the Natsui River and the Same River in Fukushima Prefecture, Japan, effects of a heavy rain event on radiocesium export were studied after Typhoon Roke during 21–22 September 2011, six months after the Fukushima Dai-ichi Nuclear Power Plant accident. Radioactivity of 134Cs and 137Cs in river waters was 0.009–0.098 Bq L−1 in normal flow conditions during July–September 2011, but it increased to 0.85 Bq L−1 in high flow conditions because of heavy rains occurring with the typhoon. The particulate fractions of 134Cs and 137Cs were 21–56% of total radiocesium in the normal flow condition, but were close to 100% after the typhoon. These results indicate that the pulse input of radiocesium associated with suspended particles from land to coastal ocean occurred because of the heavy rain event. Export flux of 134Cs and 137Cs attributable to the heavy rain accounts for 30–50% of the annual radiocesium flux from inland to coastal ocean region in 2011. Results show that rain events are one factor contributing to the transport and dispersion of radiocesium in river watersheds and coastal marine environments.
10 October 2014 in Journal of Radioanalytical and Nuclear Chemistry
At stations on the Natsui River and the Same River in Fukushima Prefecture, Japan, effects of a heavy rain event on radiocesium export were studied after Typhoon Roke during 21–22 September 2011, six months after the Fukushima Dai-ichi Nuclear Power Plant accident. Radioactivity of 134Cs and 137Cs in river waters was 0.009–0.098 Bq L−1 in normal flow conditions during July–September 2011, but it increased to 0.85 Bq L−1 in high flow conditions because of heavy rains occurring with the typhoon. The particulate fractions of 134Cs and 137Cs were 21–56% of total radiocesium in the normal flow condition, but were close to 100% after the typhoon. These results indicate that the pulse input of radiocesium associated with suspended particles from land to coastal ocean occurred because of the heavy rain event. Export flux of 134Cs and 137Cs attributable to the heavy rain accounts for 30–50% of the annual radiocesium flux from inland to coastal ocean region in 2011. Results show that rain events are one factor contributing to the transport and dispersion of radiocesium in river watersheds and coastal marine environments.
Total suspended particles (TSP) were collected in Vladivostok, Russia, which is a typical port city. This study investigated the concentration, potential sources, and long-term variation in particle PAHs and NPAHs in the atmosphere of Vladivostok. The PAH and NPAH concentrations were higher in winter than in summer (PAHs: winter: 18.6 ± 9.80 ng/m3 summer: 0.54 ± 0.21 ng/m3; NPAHs: winter: 143 ± 81.5 pg/m3 summer: 143 ± 81.5 pg/m3). The diagnostic ratios showed that PAHs and NPAHs mainly came from vehicle emissions in both seasons, while heating systems were the main source of air pollution in winter. The TEQ assessment values were 2.90 ng/m3 and 0.06 ng/m3 in winter and summer, respectively, suggesting a significant excess cancer risk in the general population in winter. The ILCR values conveyed a potential carcinogenic risk because the value was between 1 × 10−5 and 1 × 10−7 and ingestion was a main contributor in Vladivostok. However, it is worth noting that the concentrations of PAHs and NPAHs showed an overall downward trend from 1999 to 2020. An important reason for this is the cogenerations project implemented by the Far Eastern Center for Strategic Research on Fuel and Energy Complex Development in 2010. This research clarified the latest variations in PAHs and NPAHs to provide continuous observation data for future chemical reaction or model prediction research.