CoFe(2)O(4) nanoparticles were fabricated by a sol-gel method and then were coated with Co(3)Fe(7)-Co by means of a simple reduction process at different temperatures under 2% H(2) with the protection of argon to generate the dielectric-core/metallic-shell structure. The optimum reflection loss (RL) calculated from permittivity and permeability of the 80 wt% CoFe(2)O(4)/Co(3)Fe(7)-Co and 20 wt% epoxy resin composites reached - 34.4 dB, which was much lower than that of unreduced CoFe(2)O(4) and epoxy resin composites, at 2.4 GHz with a matching thickness of 4.0 mm. Moreover the RL exceeding - 10 dB in the maximum frequency range of 2.2-16 GHz was achieved for a thickness of composites of 1.0-4.5 mm with 600 °C thermal reduction process. The improved microwave absorption properties are a consequence of a proper electromagnetic match and the enhanced magnetic loss besides its dielectric loss due to the existence of the core/shell structure in CoFe(2)O(4) composites. Thus, the reductive CoFe(2)O(4) nanoparticles have great potential for being a highly efficient microwave absorber.
Current-induced magnetization reversal via spin-orbit torques (SOTs) has been intensively studied in heavy-metal/ferromagnetic-metal/oxide heterostructures due to its promising application in low-energy consumption logic and memory devices. Here, we systematically study the function of Joule heating and SOTs in the current-induced magnetization reversal using Pt/Co/SmOx and Pt/Co/AlOx structures with different perpendicular magnetic anisotropies (PMAs). The SOT-induced effective fields, anisotropy field, switching field and switching current density (Jc) are characterized using electric transport measurements based on the anomalous Hall effect and polar magneto-optical Kerr effect (MOKE). The results show that the current-generated Joule heating plays an assisted role in the reversal process by reducing switching field and enhancing SOT efficiency. The out-of-plane component of the damping-like-SOT effective field is responsible for the magnetization reversal. The obtained Jc for Pt/Co/SmOx and Pt/Co/AlOx structures with similar spin Hall angles and different PMAs remains roughly constant, revealing that the coherent switching model cannot fully explain the current-induced magnetization reversal. In contrast, by observing the domain wall nucleation and expansion using MOKE and comparing the damping-like-SOT effective field and switching field, we conclude that the current-induced magnetization reversal is dominated by the depinning model and Jc also immensely relies on the depinning field.