Cuprous oxide ( $$\hbox {Cu}{}_2\hbox {O}$$ ) has recently emerged as a promising material in solid-state quantum technology, specifically for its excitonic Rydberg states characterized by large principal quantum numbers (n). The significant wavefunction size of these highly-excited states (proportional to $$n^2$$ ) enables strong long-range dipole-dipole (proportional to $$n^4$$ ) and van der Waals interactions (proportional to $$n^{11}$$ ). Currently, the highest-lying Rydberg states are found in naturally occurring $$\hbox {Cu}_2\hbox {O}$$ . However, for technological applications, the ability to grow high-quality synthetic samples is essential. The fabrication of thin-film $$\hbox {Cu}{}_2\hbox {O}$$ samples is of particular interest as they hold potential for observing extreme single-photon nonlinearities through the Rydberg blockade. Nevertheless, due to the susceptibility of high-lying states to charged impurities, growing synthetic samples of sufficient quality poses a substantial challenge. This study successfully demonstrates the CMOS-compatible synthesis of a $$\hbox {Cu}{}_2\hbox {O}$$ thin film on a transparent substrate that showcases Rydberg excitons up to $$n = 8$$ which is readily suitable for photonic device fabrications. These findings mark a significant advancement towards the realization of scalable and on-chip integrable Rydberg quantum technologies.
14 December 2022 in The Journal of Chemical Physics
In this work, we study the magnetic phases of a spatially modulated chain of spin-1 Rydberg excitons. Using the Density Matrix Renormalization Group (DMRG) technique, we study various magnetic and topologically nontrivial phases using both single-particle properties, such as local magnetization and quantum entropy, and many-body ones, such as pair-wise Néel and long-range string correlations. In particular, we investigate the emergence and robustness of the Haldane phase, a topological phase of anti-ferromagnetic spin-1 chains. Furthermore, we devise a hybrid quantum algorithm employing restricted Boltzmann machine to simulate the ground state of such a system that shows very good agreement with the results of exact diagonalization and DMRG.
We explore the dissipative phase transition of the two-photon Dicke model, a topic that has garnered significant attention recently. Our analysis reveals that while single-photon loss does not stabilize the intrinsic instability in the model, the inclusion of two-photon loss restores stability, leading to the emergence of superradiant states, which coexist with the normal vacuum states. Using a second-order cumulant expansion for the photons, we derive an analytical description of the system in the thermodynamic limit, which agrees well with the exact calculation results. Additionally, we present the Wigner function for the system, shedding light on the breaking of the Z_{4} symmetry inherent in the model. These findings offer valuable insights into stabilization mechanisms in open quantum systems and pave the way for exploring complex nonlinear dynamics in two-photon Dicke models.
All-optical neural networks (AONNs) promise transformative gains in speed and energy efficiency for artificial intelligence (AI) by leveraging light's intrinsic parallelism and wave nature. However, their scalability has been fundamentally limited by the high power requirements of conventional nonlinear optical elements. Here, we present a low-power nonlinear activation scheme based on a three-level quantum system driven by dual laser fields. This platform introduces a two-channel nonlinear activation matrix with self- and cross-nonlinearities, enabling true multi-input, multi-output optical processing. The system supports tunable activation behaviors, including sigmoid and ReLU functions, at ultralow power levels (17 μ W per neuron). We validate our approach through theoretical modeling and experimental demonstration in rubidium vapor cells, showing the feasibility of scaling to deep AONNs with millions of neurons operating under 20 W of total optical power. Crucially, we demonstrate the all-optical generation of gradient-like signals with backpropagation, paving the way for all-optical training. These results mark a significant advance toward scalable, high-speed, and energy-efficient optical AI hardware.
Solid-state platforms provide exceptional opportunities for advancing on-chip quantum technologies by enhancing interaction strengths through coupling, scalability, and robustness. Cuprous oxide (Cu2O) has recently emerged as a promising medium for scalable quantum technology due to its high-lying Rydberg excitonic states, akin to those in hydrogen atoms. To harness these nonlinearities for quantum applications, the confinement dimensions must match the Rydberg blockade size, which can reach several microns in Cu2O. Using a CMOS-compatible growth technique, this study demonstrates the bottom-up fabrication of site-selective arrays of Cu2O microparticles. We observed Rydberg excitons up to the principal quantum number n = 5 within these Cu2O arrays on a quartz substrate and analyzed the spatial variation of their spectrum across the array, showing robustness and reproducibility on a large chip. These results lay the groundwork for the deterministic growth of Cu2O around photonic structures, enabling substantial light-matter interaction on integrated photonic platforms and paving the way for scalable, on-chip quantum devices.
Due to their quantum nature, single-photon emitters (SPE) generate individual photons in bursts or streams. They are paramount in emerging quantum technologies such as quantum key distribution, quantum repeaters, and measurement-based quantum computing. Many such systems have been reported in the last three decades, from rubidium atoms coupled to cavities to semiconductor quantum dots and color centers implanted in waveguides. This review article highlights different solid-state and atomic systems with on-demand and controlled single-photon generation. We discuss and compare the performance metrics, such as purity and indistinguishability, for these sources and evaluate their potential for different applications. Finally, a new potential single-photon source, based on the Rydberg exciton in solid-state metal oxide thin films, is introduced, where we discuss its promising features and unique advantages in fabricating quantum chips for quantum photonic applications.