Identifying dust aerosols from passive satellite images is of great interest for many applications. In this study, we developed five different machine-learning (ML) based algorithms, including Logistic Regression, K Nearest Neighbor, Random Forest (RF), Feed Forward Neural Network (FFNN), and Convolutional Neural Network (CNN), to identify dust aerosols in the daytime satellite images from the Visible Infrared Imaging Radiometer Suite (VIIRS) under cloud-free conditions on a global scale. In order to train the ML algorithms, we collocated the state-of-the-art dust detection product from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) with the VIIRS observations along the CALIOP track. The 16 VIIRS M-band observations with the center wavelength ranging from deep blue to thermal infrared, together with solar-viewing geometries and pixel time and locations, are used as the predictor variables. Four different sets of training input data are constructed based on different combinations of VIIRS pixel and predictor variables. The validation and comparison results based on the collocated CALIOP data indicate that the FFNN method based on all available predictor variables is the best performing one among all methods. It has an averaged dust detection accuracy of about 81%, 89%, and 85% over land, ocean and whole globe, respectively, compared with collocated CALIOP. When applied to off-track VIIRS pixels, the FFNN method retrieves geographical distributions of dust that are in good agreement with on-track results as well as CALIOP statistics. For further evaluation, we compared our results based on the ML algorithms to NOAA’s Aerosol Detection Product (ADP), which is a product that classifies dust, smoke, and ash using physical-based methods. The comparison reveals both similarity and differences. Overall, this study demonstrates the great potential of ML methods for dust detection and proves that these methods can be trained on the CALIOP track and then applied to the whole granule of VIIRS granule.

Smoke from fires significantly influences climate, weather, and human health. Fire smoke is traditionally detected using an aerosol index calculated from spectral contrast changes. However, such methods usually miss thin smoke plumes. It also remains challenging to accurately separate smoke plumes from dust, clouds, and bright surfaces. To improve smoke plume detections, this paper presents a new scattering-based smoke detection algorithm (SSDA) depending mainly on visible and infrared imaging radiometer suite (VIIRS) blue and green bands. The SSDA is established based on the theory of Mie scattering that occurs when the diameter of an atmospheric particulate is similar to the wavelength of the scattered light. Thus, smoke commonly causes Mie scattering in VIIRS blue and green bands because of the close correspondence between smoke particulate diameters and the blue/green band wavelengths. For developing the SSDA, training samples were selected from global fire-prone regions in North America, South America, Africa, Indonesia, Siberia, and Australia. The SSDA performance was evaluated against the VIIRS aerosol detection product and smoke detections from the ultraviolet aerosol index using manually labeled fire smoke plumes as a benchmark. Results show that the SSDA smoke detections are superior to existing products due chiefly to the improved ability of the algorithm to detect thin smoke and separate fire smoke from other surface types. Moreover, the SSDA smoke distribution pattern exhibits a high spatial correlation with the global fire density map, suggesting that SSDA is capable of detecting smoke plumes of fires in near real-time across the globe.

Formaldehyde (HCHO) is one of the most important carcinogenic air contaminants in outdoor air. However, the lack of monitoring of the global surface concentration of HCHO is currently hindering research on outdoor HCHO pollution. Traditional methods are either restricted to small areas or, for research on a global scale, too data-demanding. To alleviate this issue, we adopted neural networks to estimate the 2019 global surface HCHO concentration with confidence intervals, utilizing HCHO vertical column density data from TROPOMI, and in-situ data from HAPs (harmful air pollutants) monitoring networks and the ATom mission. Our results show that the global surface HCHO average concentration is 2.30 μg/m³. Furthermore, in terms of regions, the concentrations in the Amazon Basin, Northern China, South-east Asia, the Bay of Bengal, and Central and Western Africa are among the highest. The results from our study provide the first dataset on global surface HCHO concentration. In addition, the derived confidence intervals of surface HCHO concentration add an extra layer of confidence to our results. As a pioneering work in adopting confidence interval estimation to AI-driven atmospheric pollutant research and the first global HCHO surface distribution dataset, our paper paves the way for rigorous study of global ambient HCHO health risk and economic loss, thus providing a basis for pollution control policies worldwide.

In the near future, there will be several new instruments measuring atmospheric composition from geostationary orbit over North America, East Asia, and Europe. This constellation of satellites will provide high resolution, time resolved measurements of trace gases and aerosols for monitoring air quality and tracking pollution sources. This paper describes a detailed, fast, and accurate (less than 1.0% uncertainty) method for calculating synthetic top of the atmosphere (TOA) radiances from a global simulation with a mesoscale free running model, the GEOS-5 Nature Run, for remote sensing instruments in geostationary orbit that measure in the ultraviolet-visible spectral range (UV-Vis). Generating these synthetic observations is the first step of an Observing System Simulation Experiment (OSSE), a framework for evaluating the impact of a new observation or algorithm. This paper provides details of the model sampling, aerosol and cloud optical properties, surface reflectance modeling, Rayleigh scattering calculations, and a discussion of the uncertainties of the simulated TOA radiance. An application for the simulated TOA radiance observations is demonstrated in the manuscript. Simulated TEMPO (Tropospheric Emissions: Monitoring of Pollution) and GOES-R (Geostationary Operational Environmental Satellites) observations were used to show how observations from the two instruments could be combined to facilitate aerosol type discrimination. The results demonstrate the viability of a detailed instrument simulator for radiance measurements in the UV-Vis that is capable of accurately simulating high resolution, time-resolved measurements with reasonable computational efficiency.

Increasing emissions of ambient pollutants have caused considerable air pollution and negative health impact for human in various regions of China over the past decade. The resulting premature mortality and excessive morbidity caused huge human economic losses to the entire society. To identify the differences of health economic losses in various regions of China and help decision-making on targeting pollutants control, spatial assessment of health economic losses due to ambient pollutants in China is indispensable. In this study, to better represent the spatial variability, the satellite-based retrievals of the concentrations of various pollutants (PM₁₀, PM_2.5, O₃, NO₂, SO₂ and CO) for the time period from 2007 to 2017 in China are used instead of using in-situ data. Population raster data were applied together with exposure-response function to calculate the spatial distribution of health impact and then the health impact is further quantified by using amended human capital (AHC) approach. The results which presented in a spatial resolution of 0.25° × 0.25°, show the signification contribution from the spatial assessment to revealing the spatial distribution and variance of health economic losses in various regions of China. Spatial assessment of overall health economic losses is different from conventional result due to more detail spatial information. This spatial assessment approach also provides an alternative method for losses measurement in other fields.