We report on chemically prepared silver nanowires (diameters around 100 nm) sustaining surface plasmon modes with wavelengths shortened to about half the value of the exciting light. As we find by scattered light spectroscopy and near-field optical microscopy, the nonradiating character of these modes together with minimized damping due to the well developed wire crystal structure gives rise to large values of surface plasmon propagation length and nanowire end face reflectivity of about 10 microm and 25%, respectively. We demonstrate that these properties allow us to apply the nanowires as efficient surface plasmon Fabry-Perot resonators.
We propose the idea of a subwavelength-sized light guide represented by a linear chain of spherical metal nanoparticles in which light is transmitted by electrodynamic interparticle coupling. The light-transport properties of this system are investigated by use of model calculations based on generalized Mie theory. Considering Ag particles of 50-nm diameter, we find optimum guiding conditions for an interparticle spacing of 25 nm, and a corresponding signal-damping length of 900 nm is evaluated. The proposed principle of optical energy transport may be useful for subwavelength transmission lines within integrated optics circuits and for near-field optical microscopy.
We report on the experimental observation of near-field optical effects close to Au nanoparticles using a photon scanning tunneling microscope (PSTM). Constant height operation of the PSTM allowed an unprecedented direct comparison with theoretical computations of the distribution of the optical near-field intensity. An unexpected squeezing of the optical near field due to plasmon coupling was observed above a chain of Au nanoparticles.
We probe the influence of grating effects on plasmon excitations in gold nanoparticles arranged in regular two-dimensional patterns. Samples produced by electron-beam lithography are investigated by femtosecond time-resolved and spectroscopic methods. We find a strong dependence of the plasmon lifetime and resonance wavelength on the grating constant.
We report the experimental realization of highly efficient optical elements built up from metal nanostructures to manipulate surface plasmon polaritons propagating along a silver/polymer interface. Mirrors, beamsplitters, and interferometers produced by electron-beam lithography are investigated. The plasmon fields are imaged by detecting the fluorescence of molecules dispersed in the polymer.