With the establishment of ceilometer networks by national weather services, a discussion commenced to which extent these simple backscatter lidars can be used for aerosol research. Though primarily designed for the detection of clouds it was shown that at least observations of the vertical structure of the boundary layer might be possible. However, an assessment of the potential of ceilometers for the quantitative retrieval of aerosol properties is still missing. In this paper we discuss different retrieval methods to derive the aerosol backscatter coefficient βp, with special focus on the calibration of the ceilometers. Different options based on forward and backward integration methods are compared with respect to their accuracy and applicability. It is shown that advanced lidar systems such as those being operated in the framework of the European Aerosol Research Lidar Network (EARLINET) are excellent tools for the calibration, and thus βp retrievals based on forward integration can readily be implemented and used for real-time applications. Furthermore, we discuss uncertainties introduced by incomplete overlap, the unknown lidar ratio, and water vapor absorption. The latter is relevant for the very large number of ceilometers operating in the spectral range around λ = 905–910 nm. The accuracy of the retrieved βp mainly depends on the accuracy of the calibration and the long-term stability of the ceilometer. Under favorable conditions, a relative error of βp on the order of 10% seems feasible. In the case of water vapor absorption, corrections assuming a realistic water vapor distribution and laser spectrum are indispensable; otherwise errors on the order of 20% could occur. From case studies it is shown that ceilometers can be used for the reliable detection of elevated aerosol layers below 5 km, and can contribute to the validation of chemistry transport models, e.g., the height of the boundary layer. However, the exploitation of ceilometer measurements is still in its infancy, so more studies are urgently needed to consolidate the present state of knowledge, which is based on a limited number of case studies.
The three main objectives of the Global Climate Observing System (GCOS) Reference Upper-Air Network (GRUAN) are to provide long-term high-quality climate records of vertical profiles of selected essential climate variables (ECVs), to constrain and calibrate data from more spatially comprehensive global networks, and to provide measurements for process studies that permit an in-depth understanding of the properties of the atmospheric column. In the five years since the first GRUAN implementation and coordination meeting and the printing of an article (Seidel et al.) in this publication, GRUAN has matured to become a functioning network that provides reference-quality observations to a community of users. This article describes the achievements within GRUAN over the past five years toward making reference-quality observations of upper-air ECVs. Milestones in the evolution of GRUAN are emphasized, including development of rigorous criteria for site certification and assessment, the formal certification of the first GRUAN sites, salient aspects of the GRUAN manual and guide to operations, public availability of GRUAN’s first data product, outcomes of a network expansion workshop, and key results of scientific studies designed to provide a sound scientific foundation for GRUAN operations. Two defining attributes of GRUAN are 1) that every measurement is accompanied by a traceable estimate of the measurement uncertainty and 2) that data quality and continuity are maximized because network changes are minimized and managed. This article summarizes how these imperatives are being achieved for existing and planned data products and provides an outlook for the future, including expected new data streams, network expansion, and critical needs for the ongoing success of GRUAN.
29 April 2013 in Atmospheric Chemistry and Physics
The eruption of the Icelandic volcano Eyjafjallajökull in April–May 2010 represents a "natural experiment" to study the impact of volcanic emissions on a continental scale. For the first time, quantitative data about the presence, altitude, and layering of the volcanic cloud, in conjunction with optical information, are available for most parts of Europe derived from the observations by the European Aerosol Research Lidar NETwork (EARLINET). Based on multi-wavelength Raman lidar systems, EARLINET is the only instrument worldwide that is able to provide dense time series of high-quality optical data to be used for aerosol typing and for the retrieval of particle microphysical properties as a function of altitude. In this work we show the four-dimensional (4-D) distribution of the Eyjafjallajökull volcanic cloud in the troposphere over Europe as observed by EARLINET during the entire volcanic event (15 April–26 May 2010). All optical properties directly measured (backscatter, extinction, and particle linear depolarization ratio) are stored in the EARLINET database available at http://www.earlinet.org. A specific relational database providing the volcanic mask over Europe, realized ad hoc for this specific event, has been developed and is available on request at http://www.earlinet.org. During the first days after the eruption, volcanic particles were detected over Central Europe within a wide range of altitudes, from the upper troposphere down to the local planetary boundary layer (PBL). After 19 April 2010, volcanic particles were detected over southern and south-eastern Europe. During the first half of May (5–15 May), material emitted by the Eyjafjallajökull volcano was detected over Spain and Portugal and then over the Mediterranean and the Balkans. The last observations of the event were recorded until 25 May in Central Europe and in the Eastern Mediterranean area. The 4-D distribution of volcanic aerosol layering and optical properties on European scale reported here provides an unprecedented data set for evaluating satellite data and aerosol dispersion models for this kind of volcanic events.