The poor radiative efficiency in quantum-box luminescence is tentatively explained as an intrinsic effect rather than the usually invoked effect of etch damages. From the recently calculated decreased relaxation rate in zero-dimensional (0D) systems under 100–200-nm lateral quantization, we propose that electrons captured from the barriers in the upper levels of quantum boxes are retained in their cascade to the fundamental states for more than nanoseconds. Due to the mutual orthogonality of quantum states in a box, no luminescence, or much less than in 2D or 3D, can be obtained from these stored electrons with reasonable assumptions for the hole population. Magnetic-confinement experiments in quantum-well lasers support our conclusion. A realistic model at low temperature describes more quantitatively the observed strong decay of the radiative efficiency in quantum boxes and pseudowires with decreased lateral dimensions.
The “textbook” phonon mean free path of heat carrying phonons in silicon at room temperature is . However, a large contribution to the thermal conductivity comes from low-frequency phonons with much longer mean free paths. We present a simple experiment demonstrating that room-temperature thermal transport in Si significantly deviates from the diffusion model already at micron distances. Absorption of crossed laser pulses in a freestanding silicon membrane sets up a sinusoidal temperature profile that is monitored via diffraction of a probe laser beam. By changing the period of the thermal grating we vary the heat transport distance within the range . At small distances, we observe a reduction in the effective thermal conductivity indicating a transition from the diffusive to the ballistic transport regime for the low-frequency part of the phonon spectrum.
11 August 2008 in Angewandte Chemie International Edition
Passive radiative cooling (RC) enables the cooling of objects below ambient temperature during daytime without consuming energy, promising to be a game changer in terms of energy savings and CO2 reduction. However, so far most RC surfaces are obtained by energy‐intensive nanofabrication processes or make use of unsustainable materials. These limitations are overcome by developing cellulose films with unprecedentedly low absorption of solar irradiance and strong mid‐infrared (mid‐IR) emittance. In particular, a cellulose‐derivative (cellulose acetate) is exploited to produce porous scattering films of two different thicknesses, L ≈ 30 µm (thin) and L ≈ 300 µm (thick), making them adaptable to above and below‐ambient cooling applications. The thin and thick films absorb only of the solar irradiance, which represents a net cooling power gain of at least 17 W m−2, compared to state‐of‐the‐art cellulose‐based radiative‐cooling materials. Field tests show that the films can reach up to ≈5 °C below ambient temperature, when solar absorption and conductive/convective losses are minimized. Under dryer conditions (water column = 1 mm), it is estimated that the films can reach average minimum temperatures of ≈7–8 °C below the ambient. The work presents an alternative cellulose‐based material for efficient radiative cooling that is simple to fabricate, cost‐efficient and avoids the use of polluting materials.
Recent years have witnessed the boom of cavity optomechanics, which exploits the confinement and coupling of optical and mechanical waves at the nanoscale. Among their physical implementations, optomechanical (OM) crystals built on semiconductor slabs enable the integration and manipulation of multiple OM elements in a single chip and provide gigahertz phonons suitable for coherent phonon manipulation. Different demonstrations of coupling of infrared photons and gigahertz phonons in cavities created by inserting defects on OM crystals have been performed. However, the considered structures do not show a complete phononic bandgap, which should enable longer lifetimes, as acoustic leakage is minimized. Here we demonstrate the excitation of acoustic modes in a one-dimensional OM crystal properly designed to display a full phononic bandgap for acoustic modes at 4 GHz. The modes inside the complete bandgap are designed to have high-mechanical Q-factors, limit clamping losses and be invariant to fabrication imperfections.
20 January 2016 in The European Physical Journal B