We report the giant enhanced optical harmonic generation in all-dielectric silicon nitride (SiN) based resonant waveguide gratings (RWGs) of quasi-bound states in the continuum (BICs) of ultra-high Q factor and localized field. The BICs are realized by tuning the excitation of the guided modes modulated by geometry parameters of four-part grating layer. At a feasible structure of quasi-BIC for nanofabrication, the SHG and THG are enhanced by 103 and 106, compared with those from the RWGs of traditional two-part grating layer, respectively, and even up to 108 and 1010 compared with those from the planar SiN film, respectively. The resonance wavelength of quasi-BICs can be effectively tuned by the angle of incidence, while almost not affect the enhancement of SHG and THG response. Our results show that the efficiency harmonic generation from all-nonlinear-dielectric RWGs of quasi-BICs has potential applications for the integrated nonlinear photonic devices.
Linear and nonlinear optical properties of periodic triangular Au nanoparticle arrays were investigated. We compared the optical nonlinearity of periodic Au nanoparticle arrays with that of the ultra-thin gold film consisting of randomly distributed spheroidal clusters. A pronounced enhancement of the third-order nonlinear optical susceptibility χ((3)) in Au arrays was observed, and the figure of merit, χ((3))/α, of the periodic nanoparticle arrays is one order of magnitude larger than that of the ultra-thin film. Such an enhancement of the optical nonlinearity could be due to the strong local field near the triangular nanoparticles.
We investigate second harmonic generation (SHG) in all-dielectric resonance nanostructures of high-Q factors assisted by quasi-bound states in the continuum (quasi-BICs). The typical resonators, e.g., guided-mode resonance gratings and asymmetric metasurfaces, fabricated by AlGaAs were numerically studied with the consideration of nonlinear refraction of AlGaAs. The resonance peak and line-shape of linear transmission and SHG spectra in the resonators can be dramatically changed under intense pump intensities. The SHG conversion efficiency in the nanostructures working at quasi-BICs is much lower than the traditionally expected values without considering the nonlinear refraction of dielectrics. The ultimate SHG conversion efficiency is finally obtained. The investigation has the significance for the design and understanding of efficient nonlinear metasurfaces of high-Q factors.
The electromagnetic fields distributed on the surface region of the nanostructure is very important to improve the performance of the sensor. Here, we proposed a highly sensitive sensor based on toroidal dipole (TD) governed by bound state in the continuum (BIC) in all-dielectric metasurface consisting of single non-coaxial core-shell cylinder nanostructure array. The excitation of TD resonance in a single nanostructure is still challenging. The designed nanostructure not only supports TD resonance in a single nanostructure but also has very high Q-factor. More importantly, its electric field distributes at the surface of outer cylinder-shell, which is very suitable for biosensing. To evaluate the sensing performance of our proposed structure, we investigated the sensitivity and the figure of merit (FOM) of nanostructure with different structural parameters. Maximum sensitivity and FOM can reach up to 342 nm/RIU and 1295 when the asymmetric parameter d =10 nm. These results are of great significance to the research of TD resonance and the development of ultrasensitive sensor.
Localized surface plasmon resonance (LSPR) optical fiber biosensing is an advanced and powerful label-free technique which gets great attention for its high sensitivity to refractive index change in surroundings. However, the pursuit of a higher sensitivity is still challenging and should be further investigated. In this paper, based on a monolayer graphene/gold nanoparticles (Grm/Au NPs) three-dimensional (3D) hybrid structure, we fabricated a D-shaped plastic optical fiber (D-POF) LSPR sensor using a facile two-step method. The coupling enhancement of the resonance of this multilayer structure was extremely excited by the surface plasmon property of the stacked Au NPs/Grm layer. We found that the number of plasmonic structure layers was of high importance to the performance of the sensor. Moreover, the optimal electromagnetic field enhancement effect was found in three-layer plasmonic structure. Besides, the n*(Grm/Au NPs)/D-POF sensor exhibited outstanding performance in sensitivity (2160 nm/RIU), linearity (linear fitting coefficient R2 = 0.996) and reproducibility. Moreover, the sensor successfully detected the concentration of glucose, achieving a sensitivity of 1317.61 nm/RIU, which suggested a promising prospect for the application in medicine and biotechnology.
High-Q factor can enhance the interaction between light and matter, which is an important parameter to decrease the threshold of nanolasers. Here, we theoretically propose an eccentric nanoring structure with a high and controllable Q factor to realize a low-threshold and controllable nanolaser by amplifying the quasi-bound states in the continuum (quasi-BIC). The designed nanostructure supports a quasi-BIC because of the symmetry protection-breaking of the nanostructure. The quasi-BIC has a very high Q factor of about 9.6×104 and can also be adjusted by changing structural parameters. We use the energy level diagram of the four-level two-electron system to study the lasing action of the eccentric nanoring structure. The results show that the nanolaser has a relatively low threshold of about 6.46 μJ/cm2. Furthermore, the lasing behavior can be tuned by controlling the structural parameters of the eccentric circular ring structure.