Light beams with helical phase-fronts are known to carry orbital angular momentum (OAM) and provide an additional degree of freedom to beams of coherent light. While OAM beams can be readily derived from Gaussian laser beams with phase plates or gratings, this is far more challenging in the extreme ultra-violet (XUV), especially for the case of high XUV intensity. Here, we theoretically and numerically demonstrate that intense surface harmonics carrying OAM are naturally produced by the intrinsic dynamics of a relativistically intense circularly-polarized Gaussian beam (i.e. non-vortex) interacting with a target at normal incidence. Relativistic surface oscillations convert the laser pulses to intense XUV harmonic radiation via the well-known relativistic oscillating mirror mechanism. We show that the azimuthal and radial dependence of the harmonic generation process converts the spin angular momentum of the laser beam to orbital angular momentum resulting in an intense attosecond pulse (or pulse train) with OAM.

Effects of nonlinearity in Thomson scattering of a high intensity laser pulse from electrons are analyzed. Analytic expressions for laser pulse shaping in frequency (chirping) are obtained which control spectrum broadening for high laser pulse intensities. These analytic solutions allow prediction of the spectral form and required laser parameters to avoid broadening. Results of analytical and numerical calculations agree well. The control over the scattered radiation bandwidth allows narrow bandwidth sources to be produced using high scattering intensities, which in turn greatly improves scattering yield for future x- and gamma-ray sources.

Scattering of ultraintense short laser pulses off relativistic electrons allows one to generate a large number of X- or gamma-ray photons with the expense of the spectral width—temporal pulsing of the laser inevitable leads to considerable spectral broadening. In this Letter, we describe a simple method to generate optimized laser pulses that compensate the nonlinear spectrum broadening and can be thought of as a superposition of two oppositely linearly chirped pulses delayed with respect to each other. We develop a simple analytical model that allows us to predict the optimal parameters of such a two-pulse—the delay, amount of chirp, and relative phase—for generation of a narrow-band $\gamma$-ray spectrum. Our predictions are confirmed by numerical optimization and simulations including three-dimensional effects.

A description of the spectral and angular distributions of Compton scattered light in collisions of intense laser pulses with high-energy electrons is unwieldy and usually requires numerical simulations. However, due to the large number of parameters affecting the spectra such numerical investigations can become computationally expensive. Using methods of catastrophe theory we predict higher-dimensional caustics in the spectra of the Compton scattered light, which are associated with bright narrow-band spectral lines, and in the simplest case can be controlled by the value of the linear chirp of the pulse. These findings require no full-scale calculations and have direct consequences for the photon yield enhancement of future nonlinear Compton scattering x-ray or gamma-ray sources.

Nonlinear Compton scattering is a promising source of bright gamma rays. Using readily available intense laser pulses to scatter off the energetic electrons, on the one hand, allows us to significantly increase the total photon yield, but on the other hand, leads to a dramatic spectral broadening of the fundamental emission line as well as its harmonics due to the laser pulse shape induced ponderomotive effects. In this Letter we propose to avoid ponderomotive broadening in harmonics by using the polarization gating technique—a well-known method to construct a laser pulse with temporally varying polarization. We show that by restricting harmonic emission only to the region near the peak of the pulse, where the polarization is linear, it is possible to generate a bright narrow bandwidth comb in the gamma region.

The possibility of utilizing plasma undulators and plasma accelerators to produce compact ultraviolet and X-ray sources, has attracted considerable interest for a few decades. This interest has been driven by the great potential to decrease the threshold for accessing such sources, which are mainly provided by a few dedicated large-scale synchrotron or free-electron laser (FEL) facilities. However, the broad radiation bandwidth of such plasma devices limits the source brightness and makes it difficult for the FEL instability to develop. Here, using multi-dimensional particle-in-cell (PIC) simulations, we demonstrate that a plasma undulator generated by the beating of a mixture of high-order laser modes propagating inside a plasma channel, leads to a few percent radiation bandwidth. The strength of the undulator can reach unity, the period can be less than a millimeter, and the number of undulator periods can be significantly increased by a phase locking technique based on the longitudinal tapering. Polarization control of such an undulator can be achieved by appropriately choosing the phase of the modes. According to our results, in the fully beam loaded regime, the electron current in the plasma undulator can reach 0.3 kA level, making such an undulator a potential candidate towards a table-top FEL.