We report on the first experimental observation, to the best of our knowledge, of soliton molecules in a spatiotemporal mode-locked multimode fiber (MMF) laser. By adjusting the waveplates inside the cavity, not only the spatiotemporal mode-locking state with a stable single pulse but also soliton molecules are observed. Various soliton molecules, including soliton pairs, soliton triplets, and soliton quartets with different pulse separations, are achieved. Transition of different operation states with pump power is given. The results would be beneficial for further understanding of the nonlinear dynamics in spatiotemporal mode-locked MMF lasers.

Dissipative nonlinear wave dynamics have been investigated extensively in mode-locked lasers with single transverse mode, whereas there are few studies related to three-dimensional nonlinear dynamics within lasers. Recently, spatiotemporal mode locking (STML) was proposed in lasers with small modal (i.e., transverse-mode) dispersion, which has been considered to be critical for achieving STML in those cavities because the small dispersion can be easily balanced. Here, we demonstrate that STML can also be achieved in multimode lasers with much larger modal dispersion, where we find that the intracavity saturable absorber plays an important role for counteracting the large modal dispersion. Furthermore, we observe a new STML phenomenon of passive nonlinear autoselection of single-mode mode locking, resulting from the interaction between spatiotemporal saturable absorption and spatial gain competition. Our work significantly broadens the design possibilities for useful STML lasers thus making them much more accessible for applications, and extends the explorable parameter space of the novel dissipative spatiotemporal nonlinear dynamics that can be achieved in these lasers.

Bound solitons with various phase differences and pulse separations were observed in a net-anomalous-dispersion erbium fiber laser mode-locked by carbon nanotubes, including two-soliton bound states with phase differences close to $\pi$ (out of phase), 0 (in phase), and $\pm \pi /2$, as well as triple-soliton bound states. To our knowledge, this is the first time that in-phase two-soliton bound states have been obtained experimentally in fiber lasers. Evolution of bound states with change of pump power was investigated, and stability of different bound states was compared. Mechanisms why and how various bound states appeared in the same fiber laser are discussed and analyzed.

Experimental observations of spatiotemporal mode-locked multiple-soliton, including harmonic mode locking and multiple pulses, in multimode fiber (MMF) lasers are reported. Numerical simulations are conducted to investigate the nonlinear dynamics of multi-pulsing. The influences of cavity parameters on the spatiotemporal outputs are analyzed by simulations, which agree with the experimental observations qualitatively. This work would contribute to understanding the complex spatiotemporal nonlinear dynamics in MMF lasers.

Benefiting from ultrafast temporal resolution, broadband spectral bandwidth, as well as high peak power, passively mode-locked fibre lasers have attracted growing interest and exhibited great potential from fundamental sciences to industrial and military applications. As a nonlinear system containing complex interactions from gain, loss, nonlinearity, dispersion, etc., ultrafast fibre lasers deliver not only conventional single soliton but also soliton bunching with different types. In analogy to molecules consisting of several atoms in chemistry, soliton molecules (in other words, bound solitons) in fibre lasers are of vital importance for in-depth understanding of the nonlinear interaction mechanism and further exploration for high-capacity fibre-optic communications. In this Review, we summarize the state-of-the-art advances on soliton molecules in ultrafast fibre lasers. A variety of soliton molecules with different numbers of soliton, phase-differences and pulse separations were experimentally observed owing to the flexibility of parameters such as mode-locking techniques and dispersion control. Numerical simulations clearly unravel how different nonlinear interactions contribute to formation of soliton molecules. Analysis of the stability and the underlying physical mechanisms of bound solitons bring important insights to this field. For a complete view of nonlinear optical phenomena in fibre lasers, other dissipative states such as vibrating soliton pairs, soliton rains, rogue waves and coexisting dissipative solitons are also discussed. With development of advanced real-time detection techniques, the internal motion of different pulsing states is anticipated to be characterized, rendering fibre lasers a versatile platform for nonlinear complex dynamics and various practical applications.

Multimode fiber (MMF) lasers are emerging as a remarkable testbed to study nonlinear spatiotemporal physics with potential applications spanning from high energy pulse generation, precision measurement to nonlinear microscopy. The underlying mechanism for the generation of ultrashort pulses, which can be understood as a spatiotempoal dissipative soliton (STDS), in the nonlinear multimode resonators is the spatiotemporal mode-locking (STML) with simultaneous synchronization of temporal and spatial modes. In this review, we first introduce the general principles of STML, with an emphasize on the STML dynamics with large intermode dispersion. Then, we present the recent progress of STML, including measurement techniques for STML, exotic nonlinear dynamics of STDS, and mode field engineering in MMF lasers. We conclude by outlining some perspectives that may advance STML in the near future.