Hyperfine interaction parameters near clean and Ag-covered Fe(110) surfaces could be measured for the first time, for the first and the second monolayer separately, by means of in situ conversion-electron Mössbauer spectroscopy of oligatomic Fe(110) films on W(110) with monolayer probes. Quadrupole splitting deviates strongly from zero in the topmost monolayer only, indicating the reduced symmetry; it can be used to measure first- to second-layer self-diffusion. Magnetic hyperfine fields provide information on magnetic order near the surface with monolayer resolution.
We studied the effect of densification on the vibrational dynamics of a glass. The density of vibrational states (DOS) has been measured using nuclear inelastic scattering. The corresponding changes in the microscopic, intermediate-range, and macroscopic properties have also been investigated. The results reveal that, in the absence of local structure transformations, the Debye level and the glass-specific excess of vibrational states above it have the same dependence on density, and the evolution of the DOS is fully described by the transformation of the elastic medium.
1 April 2021 in Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
High-quality and impurity-free magnetite surfaces with reconstruction have been obtained for the epitaxial films deposited on . Based on atomically resolved scanning tunneling microscopy images for both negative and positive sample polarity and density-functional-theory calculations, a model of the magnetite (001) surface terminated with Fe ions forming dimers on the reconstructed octahedral iron layer is proposed.