A Tm,Ho:CALGO laser passively mode-locked by a GaSb-based SESAM generated pulses as short as 52 fs at a central wavelength of 2015 nm with a broad spectral bandwidth of 82 nm (full width at half maximum) owing to the combined gain profiles of both dopants for σ-polarized light. The average output power reached 376 mW at a repetition rate of 85.65 MHz. In the continuous-wave regime, the laser was power scaled up to 1.01 W at 2080.6 nm with a slope efficiency of 32.0%, a laser threshold of 155 mW and π-polarized emission. Polarized spectroscopic properties of Ho³⁺ ions in singly doped and codoped CALGO crystals were revisited to explain the observed laser performance.

Mode-locked laser operation near 2.05 µm based on a mixed sesquioxide T m : L u Y O 3 ceramic is demonstrated. Continuous-wave and wavelength-tunable operation is also investigated. Employing a GaSb-based semiconductor saturable absorber mirror as a saturable absorber, a maximum average output power of 133 mW is obtained for a pulse duration of 59 fs. Pulses as short as 54 fs, i.e., eight optical cycles are generated at a repetition rate of ∼ 78 M H z with an average output power of 51 mW. To the best of our knowledge, this result represents the shortest pulse duration ever achieved from Tm-based solid-state mode-locked lasers.

Structured ultrashort-pulse laser beams, and in particular eigenmodes of the paraxial Helmholtz equation, are currently extensively studied for novel potential applications in various fields, e.g., laser plasma acceleration, attosecond science, and fine micromachining. To extend these prospects further, in the present work we push forward the advancement of such femtosecond structured laser sources into the 2-μm spectral region. Ultrashort-pulse Hermite– and Laguerre–Gaussian laser modes both with a pulse duration around 100 fs are successfully produced from a compact solid-state laser in combination with a simple single-cylindrical-lens converter. The negligible beam astigmatism, the broad optical spectra, and the almost chirp-free pulses emphasize the high reliability of this laser source. This work, as a proof of principle study, paves the way toward few-cycle pulse generation of optical vortices at 2 μm. The presented light source can enable new research in the fields of interaction with organic materials, next generation optical detection, and optical vortex infrared supercontinuum.

We report on sub-50 fs pulse generation from a passively mode-locked (ML) Tm,Ho-codoped crystalline laser operating in a 2 µm spectral region. A T m , H o : C a ( G d , L u ) A l O 4 laser delivers pulses as short as 46 fs at 2033 nm with an average power of 121 mW at a pulse repetition rate of ∼ 78 M H z employing a semiconductor saturable absorber mirror as a saturable absorber. To the best of our knowledge, this result represents the shortest pulses ever generated from a Tm- and/or Ho-based solid-state laser. Polarization switching in the anisotropic gain material is observed in the ML regime without any polarization selection elements which is essential for the shortest pulses.

We report on the crystal growth, spectroscopic investigation and laser performance of Tm³⁺-doped monoclinic magnesium tungstate (Tm:MgWO₄), for the first time, to the best of our knowledge. A high-quality crystal has been grown by the top seeded solution growth method. The relevant spectroscopic properties are characterized in terms of absorption, luminescence and Raman spectroscopy. Judd-Ofelt (J-O) analysis is performed to evaluate the spontaneous emission probabilities and the radiative lifetimes. The absorption, stimulated-emission and gain cross-section spectra are determined for the principal light polarizations. The first laser action in the 2 μm spectral range is demonstrated in the regime of continuous-wave operation with a maximum output power of 775 mW and a slope efficiency of 39%.

Pulses as short as 44 fs (6 optical cycles) with a spectral width of 120 nm are generated from a mode-locked solid-state laser near 2 µm employing an orthorhombic Tm:GdScO₃ perovskite crystal. The average power amounts to 188 mW at a repetition rate of ∼77.6 MHz. The strong inhomogeneous line broadening in GdScO₃ suggests optimum conditions for few-optical-cycle pulse generation of rare-earth ion doped GdScO₃ bulk lasers.