This study attempts to quantify the radiative impact over Réunion Island (21° S, 55° E) in the southern tropical Indian Ocean of the aerosols and water vapor (WV) injected into the stratosphere by the eruption of the Hunga underwater volcano in the South Pacific on 15 January 2022 . Ground-based lidar and satellite passive instruments are used to parameterize a state-of-the-art radiative transfer (RT) model for the first 13 months after the volcano eruption. The descending rate of the aerosol volcanic plume is −8 m d⁻¹. At this rate, aerosols are expected to be present in the stratosphere until the first half of 2025. The overall aerosol and water vapor impact on the Earth's radiation budget for the whole period is negative (cooling, −0.82 ± 0.35 W m⁻²) and dominated by the aerosol impact (∼ 95 %; the remaining ∼ 5 % is due to the water vapor). At the Earth's surface, aerosols are the main drivers and produce a negative (cooling, −1.04 ± 0.36 W m⁻²) radiative impact. Water vapor has hardly any radiative effect at the surface. Between the short-term (months 2 to 4 after the eruption, February–April 2022) and mid-term (months 5 to 14 after the eruption, May 2022–February 2023) periods, the aerosol and water vapor radiative effect at the surface and top of atmosphere (TOA) reduces by 22 % and 25 %, respectively. During the mid-term period, heating $/$ cooling (H / C) rate profiles show a clear vertical difference locally in the stratosphere between the aerosol warming impact (18 to 26 km) and the water vapor cooling (22 to 30 km). The resulting aerosol and water vapor heating $/$ cooling rate profile follows an S-shaped curve with peaks slightly larger for the moist layer (−0.09 K d⁻¹) than for the sulfate layer (+0.06 K d⁻¹).

Fires occur seasonally in Southern Africa, from June to November, increasing tropospheric aerosol loading and triggering harmful consequences for the environment and human health. This study aims to examine 13 years of aerosol optical characteristics and types over Southern Africa and Reunion Island. Using AERONET sun photometers and MODIS observations, we found that a high aerosol optical depth and Angström exponent are associated with two predominant types of aerosols (biomass burning/urban industrial and mixed type) throughout the spring season. According to CALIOP observations, the major aerosol types with occurrence frequencies above 10% are polluted continental/smoke, polluted dust, and elevated smoke, whereas dust, clean continental, and dusty marine have occurrence frequencies below 1%. In comparison to other seasons, the vertical profiles of elevated smoke have different shapes in spring, with a seasonal shift in the peak altitude (from 3–4 km), when fire activity is at its maximum. At these altitudes, the northern regions presented occurrence frequencies of 32% on average, while lower values were found for the southern or farthest regions (<10–20% on average). The Lagrangian HYSPLIT model back-trajectories demonstrated eastward transport, with air masses from South America and the Atlantic Ocean that recirculate around the study sites. The aerosols are mainly derived from active biomass burning areas near the study sites and, to a lesser extent, from remote sources such as South America.

This study investigates the influence of the 2015 Calbuco eruption (41.2^∘ S, 72.4^∘ W; Chile) on the total columnar aerosol optical properties over the Southern Hemisphere. The well-known technic of sun photometry was applied for the investigation of the transport and spatio-temporal evolution of the optical properties of the volcanic plume. The CIMEL sun photometer measurements performed at six South American and three African sites were statistically analysed. This study involves the use of the satellite observations and a back-trajectory model. The passage of the Calbuco plume is statistically detectable in the aerosol optical depth (AOD) observations obtained from sun photometer and MODIS observations. This statistical detection confirms that the majority of the plume was transported over the northeastern parts of South America and reached the South African region 1 week after the eruption. The plume impacted the southern parts of South America to a lesser extent. The highest AOD anomalies were observed over the northeastern parts of South America. Over the South African sites, the AOD anomalies induced by the spread of the plume were quite homogeneously distributed between the east and west coasts. The optical characteristics of the plume near the source region were consistent with an ash-bearing plume. Conversely, sites further from the Calbuco volcano were influenced by ash-free plume. The optical properties discussed in this paper will be used as inputs for numerical models for further investigation of the ageing of the Calbuco plume in a forthcoming study.

The present study investigates the optical properties of aerosols on daily and seasonal scales with the use of the aerosol optical depth (AOD) and Angström exponent (AE) data retrieved from AErosol RObotic NETwork (AERONET) and collected at four stations in Southern Morocco—Saada (31.63° N; 8.16° W), Ouarzazate (30.93° N; 6.91° W), Oukaïmeden (31.21° N; 7.86° W) and Ras-El-Aïn (31.67° N; 7.60° W). An evaluation of the aerosol volumetric size distribution (AVSD) is also obtained for Saada and Ouarzazate. An AOD inter-comparison is performed between AERONET data and satellite sensors (MODerate resolution Imaging Spectroradiometer—MODIS), as well as assimilation products (Modern-Era Retrospective analysis for Research and Applications, version 2 (MERRA-2) and Copernicus Atmosphere Monitoring Service (CAMS)), by the means of a linear regression. Regardless of site location and elevation, the results show the prevalence of the annual cycle of AOD, with a maximum in summer and a minimum in winter. In association with this seasonal variation, the variations in AE and AVSD showed an increase in coarse mode over Ouarzazate and Saada during summer (July to August), underlining that Southern Morocco is prone to the regular transport of desert dust on a seasonal basis. The inter-comparison reveals that the MERRA-2 dataset is slightly more appropriate for the study region, since it shows correlation coefficients (r) ranging from 0.758 to 0.844 and intercepts ranging from 0.021 to 0.070, depending on the study site. The statistical analysis of the back-trajectories simulated by the HYbrid Single Particle Lagrangian Integrated Trajectory (HYSPLIT) model were consistent with the observations and confirmed the dominance of desert dust aerosols during the summer over the study region. On the other hand, the winter season reveals a predominance of anthropogenic and oceanic aerosols originating from the north and the west of the study site.

During the 2020 austral summer, the pristine atmosphere of the southwest Indian Ocean (SWIO) basin experienced significant perturbations. This study examines the variability of aerosols and carbon monoxide (CO) over this remote oceanic region and investigates the underlying processes in the upper troposphere–lower stratosphere (UT-LS). Aerosol profiles in January and February 2020 revealed a multi-layer structure in the tropical UT-LS. Numerical models – the FLEXible PARTicle dispersion model (FLEXPART) and the Modèle Isentropique de transport Mésoéchelle de l'Ozone Stratosphérique par Advection (MIMOSA) – indicated that the lower-stratospheric aerosol content was influenced by the intense and persistent stratospheric aerosol layer generated during the 2019–2020 extreme Australian bushfire events. A portion of this layer was transported eastward by prevailing easterly winds, leading to increased aerosol extinction profiles over Réunion on 27 and 28 January. Analysis of advected potential vorticity revealed isentropic transport of air masses containing Australian biomass burning aerosols from extratropical latitudes to Réunion at the 400 K isentropic level on 28 January. Interestingly, we found that biomass burning (BB) activity in eastern Africa, though weak during this season, significantly influenced (contributed up to 90 % of) the vertical distribution of CO and aerosols in the upper troposphere over the SWIO basin. Ground-based observations at Réunion confirmed the simultaneous presence of African and Australian aerosol layers. This study provides the first evidence of African BB emissions impacting the CO and aerosol distribution in the upper troposphere over the SWIO basin during the convective season.