The magnetochiral effect (MCE) of phonons, a nonreciprocal acoustic propagation arising due to symmetry principles, is demonstrated in the chiral-lattice ferrimagnet . Our high-resolution ultrasound experiments reveal that the sound velocity differs for parallel and antiparallel propagation with respect to the external magnetic field. The sign of the nonreciprocity depends on the chirality of the crystal in accordance with the selection rule of the MCE. The nonreciprocity is enhanced below the magnetic ordering temperature and at higher ultrasound frequencies, which is quantitatively explained by a proposed magnon-phonon hybridization mechanism.
We experimentally demonstrate one-way transparency of light in multiferroic . The material is rendered transparent for light propagating in one direction, while opaque for light propagating in the opposite direction. The novel transparency results from a destructive interference of the electric dipole and magnetic dipole transitions. The realization of the effect has been accomplished by the application of a high magnetic field and the proper selection of the propagation direction of light in agreement with our quantum mechanical formulation of nonreciprocal directional dichroism.
Magnetization measurements of have been carried out up to 133 T, generated with a destructive pulse magnet at a wide temperature range from 2 to 120 K. A novel magnetic transition was found at T and K, which is characterized by its transition field increasing with increasing temperature. At , the previously reported transition at T was observed. Based on the obtained phase diagram and the Clausius-Clapeyron relation, the entropy of the high-field phase at 80 K is found to be smaller for about J than that of the low-field phase. We suggest that the observed two high-field phases may originate in different spatial orders of the spin states and possibly other degrees of freedom such as orbitals. An inherent strong correlation of spin states among cobalt sites should have triggered the emergence of the ordered phases in at high magnetic fields.
Under magnetic fields, quantum magnets often undergo exotic phase transitions with various kinds of order. The discovery of a sequence of fractional magnetization plateaus in the Shastry-Sutherland compound SrCu2(BO3)2 has played a central role in the high-field research on quantum materials, but so far this system could only be probed up to half the saturation value of the magnetization. Here, we report the first experimental and theoretical investigation of this compound up to the saturation magnetic field of 140 T and beyond. Using ultrasound and magnetostriction techniques combined with extensive tensor-network calculations (iPEPS), several spin-supersolid phases are revealed between the 1/2 plateau and saturation (1/1 plateau). Quite remarkably, the sound velocity of the 1/2 plateau exhibits a drastic decrease of -50%, related to the tetragonal-to-orthorhombic instability of the checkerboard-type magnon crystal. The unveiled nature of this paradigmatic quantum system is a new milestone for exploring exotic quantum states of matter emerging in extreme conditions.
A high-speed 100 MHz strain monitor using a fiber Bragg grating, an optical filter, and a mode-locked optical fiber laser has been devised, whose resolution is . The strain monitor is sufficiently fast and robust for the magnetostriction measurements of materials under ultrahigh magnetic fields generated with destructive pulse magnets, where the sweep rate of the magnetic field is in the range of 10–100 T/ s. As a working example, the magnetostriction of LaCoO3 was measured at room temperature, 115 K, and 7 4.2 K up to a maximum magnetic field of 150 T. The smooth dependence on the squared magnetic field and the first-order transition were observed at 115 K and 7 4.2 K, respectively, reflecting the field-induced spin state evolution.
Magnetization measurements and magnetotransmission spectroscopy of the solid oxygen phase were performed in ultrahigh magnetic fields of up to 193 T. An abrupt increase in magnetization with large hysteresis was observed when pulsed magnetic fields greater than 120 T were applied. Moreover, the transmission of light significantly increased in the visible range. These experimental findings indicate that a first-order phase transition occurs in solid oxygen in ultrahigh magnetic fields, and that it is not just a magnetic transition. Considering the molecular rearrangement mechanism found in the dimer system, we conclude that the observed field-induced transition is caused by the antiferromagnetic phase collapsing and a change in the crystal structure.