Zhonghao Liu

Dr. Zhonghao Liu

Shanghai Institute of Microsystem and Information Technology Chinese Academy of Sciences, Shanghai, China

Research Focus & Metrics

Academic Career Length

8Years (2019-Present)

(Calculated once Scilit publication data is synced: current year − year of first publication + 1)

Representative Publications

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25 May 2021 in Nature Communications
Verified
Journal Article
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MLMan Li
Man Li
QWQi Wang
Qi Wang
GWGuangwei Wang
Guangwei Wang
ZYZhihong Yuan
Zhihong Yuan
WSWenhua Song
Wenhua Song
SWShancai Wang
Shancai Wang
Kagome-lattices of 3d-transition metals hosting Weyl/Dirac fermions and topological flat bands exhibit non-trivial topological characters and novel quantum phases, such as the anomalous Hall effect and fractional quantum Hall effect. With consideration of spin–orbit coupling and electron correlation, several instabilities could be induced. The typical characters of the electronic structure of a kagome lattice, i.e., the saddle point, Dirac-cone, and flat band, around the Fermi energy (EF) remain elusive in magnetic kagome materials. We present the experimental observation of the complete features in ferromagnetic kagome layers of YMn6Sn6 helically coupled along the c-axis, by using angle-resolved photoemission spectroscopy and band structure calculations. We demonstrate a Dirac dispersion near EF, which is predicted by spin-polarized theoretical calculations, carries an intrinsic Berry curvature and contributes to the anomalous Hall effect in transport measurements. In addition, a flat band and a saddle point with a high density of states near EF are observed. These multi-sets of kagome features are of orbital-selective origin and could cause multi-orbital magnetism. The Dirac fermion, flat band and saddle point in the vicinity of EF open an opportunity in manipulating the topological properties in magnetic materials.

10 August 2020 in Nature Communications
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ZLZhonghao Liu
Zhonghao Liu
MLMan Li
Man Li
QWQi Wang
Qi Wang
GWGuangwei Wang
Guangwei Wang
CWChenhaoping Wen
Chenhaoping Wen
SWShancai Wang
Shancai Wang
Layered kagome-lattice 3d transition metals are emerging as an exciting platform to explore the frustrated lattice geometry and quantum topology. However, the typical kagome electronic bands, characterized by sets of the Dirac-like band capped by a phase-destructive flat band, have not been clearly observed, and their orbital physics are even less well investigated. Here, we present close-to-textbook kagome bands with orbital differentiation physics in CoSn, which can be well described by a minimal tight-binding model with single-orbital hopping in Co kagome lattice. The capping flat bands with bandwidth less than 0.2 eV run through the whole Brillouin zone, especially the bandwidth of the flat band of out-of-plane orbitals is less than 0.02 eV along Γ−M. The energy gap induced by spin-orbit interaction at the Dirac cone of out-of-plane orbitals is much smaller than that of in-plane orbitals, suggesting orbital-selective character of the Dirac fermions.

14 October 2021 in Physical Review X
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ZLZhonghao Liu
Zhonghao Liu
NZNingning Zhao
Ningning Zhao
QYQiangwei Yin
Qiangwei Yin
CGChunsheng Gong
Chunsheng Gong
ZTZhijun Tu
Zhijun Tu
SWShancai Wang
Shancai Wang
Recently discovered Z2 topological kagome metals AV3Sb5 (A=K, Rb, and Cs) exhibit charge-density-wave (CDW) phases and novel superconducting paring states providing a versatile platform for studying the interplay between electron correlation and quantum orders. Here we directly visualize CDW-induced bands renormalization and energy gaps in RbV3Sb5 using angle-resolved photoemission spectroscopy pointing to the key role of tuning van Hove singularities to the Fermi energy in mechanisms of ordering phases. Near the CDW transition temperature, the bands around the Brillouin zone (BZ) boundary are shifted to high-binding energy, forming an M-shaped band with singularities near the Fermi energy. The Fermi surfaces are partially gapped, and the electronic states on the residual ones should be possibly dedicated to the superconductivity. Our findings are significant in understanding CDW formation and its associated superconductivity.

10 August 2020 in Nature Communications
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Jia-Xin YinJia-Xin Yin
Jia-Xin Yin
NSNana Shumiya
Nana Shumiya
MMMardanya Mardanya
Mardanya Mardanya
QWQi Wang
Qi Wang
SZSongtian S. Zhang
Songtian S. Zhang
MHM. Zahid Hasan
M. Zahid Hasan
Kagome-nets, appearing in electronic, photonic and cold-atom systems, host frustrated fermionic and bosonic excitations. However, it is rare to find a system to study their fermion–boson many-body interplay. Here we use state-of-the-art scanning tunneling microscopy/spectroscopy to discover unusual electronic coupling to flat-band phonons in a layered kagome paramagnet, CoSn. We image the kagome structure with unprecedented atomic resolution and observe the striking bosonic mode interacting with dispersive kagome electrons near the Fermi surface. At this mode energy, the fermionic quasi-particle dispersion exhibits a pronounced renormalization, signaling a giant coupling to bosons. Through the self-energy analysis, first-principles calculation, and a lattice vibration model, we present evidence that this mode arises from the geometrically frustrated phonon flat-band, which is the lattice bosonic analog of the kagome electron flat-band. Our findings provide the first example of kagome bosonic mode (flat-band phonon) in electronic excitations and its strong interaction with fermionic degrees of freedom in kagome-net materials.

14 August 2023 in Nature Communications
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ZJZhicheng Jiang
Zhicheng Jiang
ZLZhengtai Liu
Zhengtai Liu
HMHaiyang Ma
Haiyang Ma
WXWei Xia
Wei Xia
ZLZhonghao Liu
Zhonghao Liu
DSDawei Shen
Dawei Shen
A representative class of kagome materials, AV3Sb5 (A = K, Rb, Cs), hosts several unconventional phases such as superconductivity, $${{\mathbb{Z}}}_{2}$$ Z 2 non-trivial topological states, and electronic nematic states. These can often coexist with intertwined charge-density wave states. Recently, the discovery of the isostructural titanium-based single-crystals, ATi3Bi5 (A = K, Rb, Cs), which exhibit similar multiple exotic states but without the concomitant charge-density wave, has opened an opportunity to disentangle these complex states in kagome lattices. Here, we combine high-resolution angle-resolved photoemission spectroscopy and first-principles calculations to investigate the low-lying electronic structure of RbTi3Bi5. We demonstrate the coexistence of flat bands and several non-trivial states, including type-II Dirac nodal lines and $${{\mathbb{Z}}}_{2}$$ Z 2 non-trivial topological surface states. Our findings also provide evidence for rotational symmetry breaking in RbTi3Bi5, suggesting a directionality to the electronic structure and the possible emergence of pure electronic nematicity in this family of kagome compounds.

7 February 2020 in Physical Review Letters
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YSY. K. Song
Y. K. Song
GWG. W. Wang
G. W. Wang
SLS. C. Li
S. C. Li
WLW. L. Liu
W. L. Liu
XLX. L. Lu
X. L. Lu
DSD. W. Shen
D. W. Shen
Topological nodal-line semimetals with exotic quantum properties are characterized by symmetry-protected line-contact bulk band crossings in the momentum space. However, in most of identified topological nodal-line compounds, these topological nontrivial nodal lines are enclosed by complicated topological trivial states at the Fermi energy (EF), which would perplex their identification and hinder further applications. Utilizing angle-resolved photoemission spectroscopy and first-principles calculations, we provide compelling evidence for the existence of Dirac nodal-line fermions in the monoclinic semimetal SrAs3, which possesses a simple nodal loop in the vicinity of EF without the distraction from complicated trivial Fermi surfaces. Our calculations revealed that two bands with opposite parities were inverted around Y near EF, resulting in the single nodal loop at the Γ−Y−S plane with a negligible spin-orbit coupling effect. The band crossings were tracked experimentally and the complete nodal loop was identified quantitatively, which provide a critical experimental support for the existence of nodal-line fermions in the CaP3 family of materials. Hosting simple topological nontrivial bulk electronic states around EF and without complication from the trivial states, SrAs3 is expected to be a potential platform for topological quantum state investigation and applications.