We report efficient amplification of chirped supercontinuum pulses in a two-stage stimulated Raman amplifier based on double tungstate [ K G d ( W O 4 ) 2 ] crystals, pumped with 1.2 ps transform-limited pulses at a 1030 nm wavelength. The second stage demonstrates a conversion efficiency of 55% with an output pulse energy of 0.6 mJ at a 1135 nm wavelength. The amplified Stokes bandwidth is 10 times the pump bandwidth, providing 145 fs pulses after compression.

We present a compact and cost-effective mJ-level femtosecond laser system operating at a center wavelength of approximately 2.15 μm. An affordable two-stage ytterbium-doped yttrium aluminum garnet (Yb:YAG) chirped pulse amplifier provides more than 10 mJ, approximately 1.2 ps pulses at 1030 nm to pump a three-stage optical parametric chirped pulse amplifier (OPCPA) based on bismuth borate crystals and to drive the supercontinuum seed in the YAG crystal. The energy of the amplified pulses in the wavelength range of 1.95–2.4 μm reached 2.25 mJ with a pump-to-signal conversion efficiency of approximately 25% in the last OPCPA stage. These pulses were compressed to 38 fs in a pair of Suprasil 300 glass prisms.

Three different stimulated Brillouin scattering (SBS) configurations in perfluorooctane were experimentally compared to achieve the ultimate compression of ~1.1 ns pulses from a commercially available Nd:YAG mini-laser. These schemes contained either a focusing lens and a plane feedback mirror, a spherical mirror, or variable pulse splitting to provide self-seeding of the SBS. In the optimal configuration with a focusing lens and return mirror, 93 ps pulses with an energy of 9.5 mJ were achieved at the output of the double-pass phase-conjugated Nd:YAG amplifier. The resulting diffraction-free, high-quality beams with M²~1.2 and excellent pointing stability are of practical interest for scientific, medical, and industrial applications.

The synthesis of adjacent overlapped Stokes spectra in two stages of a transient stimulated Raman chirped-pulse amplifier, tuned respectively to the vibrational modes at 901 and 767 cm⁻¹ of a potassium gadolinium tungstate [KGd(WO₄)₂] crystal, is demonstrated. The contribution of the spatio-temporal overlap of seed and pump pulses, as well as the self-phase modulation, was investigated. The noncollinear configuration allows the composite bandwidth at the central wavelength of 1120 nm to be increased by a factor of 23 compared to the pump pulse bandwidth of 1.6 nm. After reaching a conversion efficiency of 35% in the second stage, the compressibility of a chirped Stokes pulse with a tailored spectrum was also investigated.

Multiple higher-order Stokes of rotational stimulated Raman scattering (SRS) in compressed hydrogen covered the wavelength range from ~1.1 µm to ~1.4 µm using ~1.2 ps pump pulses from a Yb:YAG laser. In this study, the influence of polarization, energy, and the focusing conditions of the pump pulse, as well as gas pressure, on the conversion efficiency and modification of the spectral envelope of rotational and vibrational SRS was investigated. The use of a supercontinuum seed, as well as circular polarization of pump pulses at high hydrogen pressure, made it possible to significantly reduce the threshold for rotational SRS and suppress vibrational Stokes modes. The cascade excitation of rotational SRS, corresponding to a shift of 587 cm⁻¹, ensured a spectrum spanning four Stokes orders withs a conversion efficiency of 52% and an output energy exceeding 3 mJ. The synthesized spectrum corresponded to ~14 fs transform-limited pulses.

The combination of optical parametric and transient stimulated Raman amplification of chirped pulses demonstrates a new approach for idler energy buildup in the short-wave (SW)IR range. Optical parametric chirped-pulse amplification (OPCPA) output pulses in the wavelength range from ∼1800 nm to ∼2000 nm for the signal and from ∼2100 nm to ∼2400 nm for the idler were used as pump and Stokes seed, respectively, in a stimulated Raman amplifier based on a KGd(WO₄)₂ crystal. Both OPCPA and its supercontinuum seed were pumped with ∼1.2-ps transform-limited pulses from a Yb:YAG chirped-pulse amplifier. The transient stimulated Raman chirped-pulse amplifier provides a 33% increase in idler energy with nearly transform-limited ∼53-fs pulses after compression.