Powering aircraft by sustainable aviation fuels (SAFs) is a pathway to reduce the climate impact of aviation by lowering aviation lifecycle CO₂ emissions and by reducing ice crystal numbers and radiative forcing from contrails. While the effect of SAF blends on contrails has been measured previously, here we present novel measurements on particle emission and contrails from 100 % SAF combustion. During the ECLIF3 (Emission and CLimate Impact of alternative Fuels) campaign, a collaboration between the Deutsches Zentrum für Luft- und Raumfahrt (DLR), Airbus, Rolls-Royce, and Neste, the DLR Falcon 20 research aircraft performed in situ measurements following an Airbus A350-941 source aircraft powered by Rolls-Royce Trent XWB-84 engines in 1 to 2 min old contrails at cruise altitudes. Apparent ice emission indices of 100 % HEFA-SPK (hydro-processed esters and fatty acids–synthetic paraffinic kerosene) were measured and compared to Jet A-1 fuel contrails at similar engine and ambient ice-supersaturated conditions within a single flight. A 56 % reduction in ice particle numbers per mass of burned fuel was measured for 100 % HEFA-SPK compared to Jet A-1 under engine cruise conditions. The measured 35 % reduction in soot particle numbers suggests reduced ice activation by the low-sulfur HEFA fuel. Contrail properties are consistently modeled with a contrail plume model. Global climate model simulations for the 2018 fleet conservatively estimate a 26 % decrease in contrail radiative forcing and stronger decreases for larger particle reductions. Our results indicate that higher hydrogen content fuels as well as clean engines with low particle emissions may lead to reduced climate forcing from contrails.

In order to reduce aviation's CO₂ emissions and comply with current climate targets, the European Union plans a mandatory quota of 2 % sustainable aviation fuel (SAF) by 2025, rising up to ≥70 % SAF by 2050. In addition to a reduction of life cycle CO₂ emissions, the use of SAF can also have a positive impact on particle emissions and contrail properties. In this study we present observations from the ECLIF3 (Emission and CLimate Impact of alternative Fuels) aircraft campaign, which investigated exhaust and contrail characteristics of an Airbus A350-941 equipped with Rolls-Royce Trent XWB-84 engines. For the first time, non-volatile and total particle emissions of 100 % HEFA-SPK (hydroprocessed esters and fatty acids–synthetic paraffinic kerosene) SAF, a blended fuel and a reference Jet A-1 fuel were measured in flight. A maximum reduction in non-volatile particle number emissions of ∼41 % compared to the reference Jet A-1 fuel was measured at low cruise engine power settings when using 100 % HEFA-SPK. The reduction decreases to ∼29 % for typical cruise engine settings and to ∼22 % at high cruise engine power settings. The size of non-volatile particles was slightly smaller for HEFA-SPK compared to Jet A-1. We show a comprehensive analysis of the hydrogen content of globally available fuels. Our results demonstrate the impact of the fuel composition in terms of its aromatic, hydrogen, and sulfur content as well as of the effect of engine power settings on particle emissions. We demonstrate that the use of HEFA-SPK can significantly reduce particle emissions and thus contrail ice particles and therefore can provide an aviation climate benefit.

Nitrogen oxides, emitted from air traffic, are of concern due to their impact on climate by changing atmospheric ozone and methane levels. Using the DLR research aircraft Falcon, total reactive nitrogen (NO_y) in-flight measurements were carried out at high altitudes to characterize emissions in the fresh aircraft exhaust from the latest-generation Rolls-Royce Trent XWB-84 engine aboard the long-range Airbus A350-941 aircraft during the ECLIF3 (Emission and CLimate Impact of alternative Fuels 3) experiment. The impact of different engine thrust settings, monitored in terms of combustor inlet temperature, pressure and engine fuel flow, was tested for two different fuel types: Jet A-1 and, for the first time, a 100 % sustainable aviation fuel (SAF) under similar atmospheric conditions. In addition, a range of combustor temperatures and an additional blended SAF were tested during ground-based emission measurements. For the data measured during ECLIF3, we confirm that the NO_x emission index increases with increasing combustion temperature, pressure and fuel flow. We find that as expected, the fuel type has no measurable effect on the NO_x emission index. These measurements are used to compare to cruise NO_x emission index estimates from three engine emission prediction methods. Our measurements thus help to understand the ground to cruise correlation of current engine emission prediction methods while serving as input for climate modelling and extending the extremely sparse data set on in-flight aircraft nitrogen oxide emissions to newer engine generations.

Ambient weather conditions strongly impact contrail formation and persistence. The implementation of contrail avoidance and mitigation strategies, therefore, requires regional and altitude-dependent information on the frequency of contrail occurrence. To this end, we have developed a method to quantify the potential contrail cover based on 10 years of high-resolution reanalysis of climatology and weather data from the European Center for Medium-Range Weather Forecast (ECMWF). We use the Schmidt–Appleman threshold temperature for contrail formation and additionally select thresholds for the relative humidity to evaluate the occurrence of persistent contrails and assess their regional and seasonal variation. We find a potential contrail cirrus cover of 10% to 20% above Europe at higher altitudes of 200 and 250 hPa in the 10-year climatology and a weak seasonal variation. At lower altitudes, near 300 hPa, a steep onset and a high potential contrail cirrus cover of 20% is found in late fall and in winter, decreasing to 2% potential contrail cirrus cover in summer. In comparison to ECMWF data, evaluations using data from the National Centers for Environmental Prediction (NCEP) show a significantly lower potential contrail cirrus cover. Our results help to investigate the seasonal and altitude dependence of contrail mitigation strategies, in particular for warming nighttime contrails that contribute strongly to the total climate impact from aviation.

Contrail cirrus clouds are a main contributor to the climate forcing from aviation ¹ . Yet, the number of contrail ice crystals forming behind aircraft with modern lean-burn engines is unknown. Theory spans a four orders of magnitude range in ice crystal numbers ^2,3 —rendering related climate effects unpredictable. Here we show that lean-burn combustion reduces soot particle number emissions by three orders of magnitude compared with conventional rich–quench–lean engines ^4,5 —but does not significantly decrease volatile particles or contrail ice crystal numbers—both can exceed 10 ¹⁵ particles per kg of burned fuel. Our findings arise from in-flight observations behind an A321neo aircraft with lean-burn engines, thus providing real-world confirmation of some laboratory work ⁶ and narrowing the range of theoretical expectations. Our results indicate that the tested lean-burn engine configurations alone are unlikely to reduce the warming effect of contrails, suggesting that modifications of fuel composition and lubrication oil venting architecture may be required. We show that contrail ice particle numbers in the low-soot regime can be reduced by using low-sulfur fuels and that organic fuel constituents and lubrication oil vapours can increase contrail ice particle numbers. Future research should explore how reductions in volatile particles, apart from soot, affect contrail ice formation.

Nitrogen oxides, emitted from air traffic, are of concern due to their impact on climate by changing atmospheric ozone and methane levels. Using the DLR research aircraft Falcon, total reactive nitrogen (NOy) measurements were carried out at high altitudes to characterize emissions in the fresh aircraft exhaust from the latest generation Rolls-Royce Trent XWB-84 engine aboard the long-range Airbus A350-941 aircraft. The impact of different engine thrust settings, monitored in terms of combustor inlet temperature, pressure, and engine fuel flow, was tested for three different fuel types under similar atmospheric conditions: Jet A-1, for the first time a 100% sustainable aviation fuel (SAF), and a blend of both fuels. In addition, a range of combustor temperatures were tested during ground emission measurements. We confirm that the NOx emission index increases with increasing combustion temperature, pressure and fuel flow. We find that as expected, the fuel type has no measurable effect on the NOx emission index. These measurements are used to evaluate cruise NOx emission index estimates from three engine emission models. Our measurements thus help to evaluate the ground to cruise correlation of current engine models, serve as input for climate modelling, and extend the extremely sparse data set on in-flight aircraft NOx emissions to newer engine generations.