Noncollinear antiferromagnets with a (, ) hexagonal structure have garnered much attention for their potential applications in topological spintronics. Here, we report the deposition of continuous epitaxial thin films of such a material, , and characterize their crystal structure using a combination of x-ray diffraction and transmission electron microscopy. Growth of films with both (0001) -axis orientation and () texture is achieved. In the latter case, the thin films exhibit a small uncompensated Mn moment in the basal plane, quantified via magnetometry and x-ray magnetic circular dichroism experiments. This cannot account for the large anomalous Hall effect simultaneously observed in these films, even at room temperature, with magnitude and coercive field . We attribute the origin of this anomalous Hall effect to momentum-space Berry curvature arising from the symmetry-breaking inverse triangular spin structure of . Upon cooling through the transition to a glassy ferromagnetic state at around 50 K, a peak in the Hall resistivity close to the coercive field emerges. This indicates the onset of a topological Hall effect contribution, arising from a nonzero scalar spin chirality that generates a real-space Berry phase. We demonstrate that the polarity of this topological Hall effect, and hence the chiral nature of the noncoplanar magnetic structure driving it, can be controlled using different field-cooling conditions.
Cooperative effects determine the spin-state bistability of spin-crossover molecules (SCMs). Herein, the ultimate scale limit at which cooperative spin switching becomes effective is investigated in a complex [Fe(H2B(pz)2)2(bipy)] deposited on a highly oriented pyrolytic graphite surface, using x-ray absorption spectroscopy. This system exhibits a complete thermal- and light-induced spin transition at thicknesses ranging from submonolayers to multilayers. On increasing the coverage from 0.35(4) to 10(1) monolayers, the width of the temperature-induced spin transition curve narrows significantly, evidencing the buildup of cooperative effects. While the molecules at the submonolayers exhibit an apparent anticooperative behavior, the multilayers starting from a double-layer exhibit a distinctly cooperative spin switching, with a free-molecule-like behavior indicated at around a monolayer. These observations will serve as useful guidelines in designing SCM-based devices.
For spintronics application, which requires fast field switching, it is important to have a kind of soft magnetic material with large damping coefficient. Here, we present the studies of the Nd dopant-level-dependent damping coefficient of Nd-Py thin films (30 nm) in a dilute region utilizing ferromagnetic resonance (FMR). With the Nd content increasing, the film structure was found to be changing from polycrystalline to amorphous when the Nd content is around 3.4%. Meanwhile, the magnetization decreases linearly. Interestingly, we find that along the easy axis, both low coercivity and high hysteresis squareness are simultaneously maintained in the system; i.e., the magnetic softness has been well kept. By theoretical fitting of the angular dependence of the FMR field, the first- and second-order magnetic anisotropy constants, and , and the Lande factor are obtained and discussed quantitatively. The measurements of angular and frequency dependence of the ferromagnetic resonance linewidth, as well as the theoretical fitting by considering the contributions of Gilbert damping, two-magnon scattering, and inhomogeneous broadening, show that the damping coefficient increases rapidly (about 25-fold) as the Nd content increases to 11.6%, which is mainly due to the enhanced spin-orbit coupling by the Nd additives, supported by x-ray magnetic circular dichroism measurements.
Odorant binding proteins (OBPs) and chemosensory proteins (CSPs) of arthropods are thought to be involved in chemical recognition which regulates pivotal behaviors including host choice, copulation and reproduction. In insects, OBPs and CSPs located mainly in the antenna but they have not been systematically characterized yet in Bemisia tabaci which is a cryptic species complex and could damage more than 600 plant species. In this study, among the 106,893 transcripts in the head assembly, 8 OBPs and 13 CSPs were identified in B. tabaci MED based on head transcriptomes of adults. Phylogenetic analyses were conducted to investigate the relationships of B. tabaci OBPs and CSPs with those from several other important Hemipteran species, and the motif-patterns between Hemiptera OBPs and CSPs were also compared by MEME. The expression profiles of the OBP and CSP genes in different tissues of B. tabaci MED adults were analyzed by real-time qPCR. Seven out of the 8 OBPs found in B. tabaci MED were highly expressed in the head. Conversely, only 4 CSPs were enriched in the head, while the other nine CSPs were specifically expressed in other tissues. Our findings pave the way for future research on chemical recognition of B. tabaci at the molecular level.
The electronic reconstruction occurring at oxide interfaces may be the source of interesting device concepts for future oxide electronics. Among oxide devices, multiferroic tunnel junctions are being actively investigated as they offer the possibility to modulate the junction current by independently controlling the switching of the magnetization of the electrodes and of the ferroelectric polarization of the barrier. In this Letter, we show that the spin reconstruction at the interfaces of a multiferroic tunnel junction is the origin of a spin filtering functionality that can be turned on and off by reversing the ferroelectric polarization. The ferroelectrically controlled interface spin filter enables a giant electrical modulation of the tunneling magnetoresistance between values of 10% and 1000%, which could inspire device concepts in oxides-based low dissipation spintronics.
The sweet potato whitefly Bemisia tabaci is a major agricultural pest with a wide host range throughout the world. The species designation for B. tabaci includes numerous distinct cryptic species or biotypes. Two invasive B. tabaci biotypes, MEAM1 (B) and MED (Q), were found in China at the end of the 20th century and at the beginning of the 21st century. MEAM1 (B) and MED (Q) show higher pesticide resistance levels than native strains, and the levels of resistance vary with changes in insecticide selection pressure. Recent studies have revealed metabolic resistance mechanisms and target site mutations in invasive B. tabaci strains that render them resistant to a range of insecticides and have uncovered the frequency of these resistance-related mutations in B. tabaci populations in China. Novel pest control agents, such as RNA-based pesticides and nano-pesticides, have achieved effective control effects in the laboratory and are expected to be applied for field control of B. tabaci in the future. In this review, we discuss the mechanisms of resistance developed by these invasive B. tabaci populations since their invasion into China. We also provide suggestions for ecologically sound and efficient B. tabaci control.
About Me
Prof. Dr. Luo works on insecticide resistance and pest management.
Prof. Dr. Luo works on insecticide resistance and pest management.