Significance: Exceedingly high levels of fine particulate matter (PM) occur frequently in China, but the mechanism of severe haze formation remains unclear. From atmospheric measurements in two Chinese megacities and laboratory experiments, we show that the oxidation of SO 2 by NO 2 occurs efficiently in aqueous media under two polluted conditions: first, during the formation of the 1952 London Fog via in-cloud oxidation; and second, on fine PM with NH 3 neutralization during severe haze in China. We suggest that effective haze mitigation is achievable by intervening in the sulfate formation process with NH 3 and NO 2 emission control measures. Hence, our results explain the outstanding sulfur problem during the historic London Fog formation and elucidate the chemical mechanism of severe haze in China.
11 June 2020 in Proceedings of the National Academy of Sciences
Various mitigation measures have been implemented to fight the coronavirus disease 2019 (COVID-19) pandemic, including widely adopted social distancing and mandated face covering. However, assessing the effectiveness of those intervention practices hinges on the understanding of virus transmission, which remains uncertain. Here we show that airborne transmission is highly virulent and represents the dominant route to spread the disease. By analyzing the trend and mitigation measures in Wuhan, China, Italy, and New York City, from January 23 to May 9, 2020, we illustrate that the impacts of mitigation measures are discernable from the trends of the pandemic. Our analysis reveals that the difference with and without mandated face covering represents the determinant in shaping the pandemic trends in the three epicenters. This protective measure alone significantly reduced the number of infections, that is, by over 78,000 in Italy from April 6 to May 9 and over 66,000 in New York City from April 17 to May 9. Other mitigation measures, such as social distancing implemented in the United States, are insufficient by themselves in protecting the public. We conclude that wearing of face masks in public corresponds to the most effective means to prevent interhuman transmission, and this inexpensive practice, in conjunction with simultaneous social distancing, quarantine, and contact tracing, represents the most likely fighting opportunity to stop the COVID-19 pandemic. Our work also highlights the fact that sound science is essential in decision-making for the current and future public health pandemics.
Air pollution epidemic: The lockdown enforced in most cities in China in response to the outbreak of severe acute respiratory syndrome coronavirus 2 (SARS-CoV-2) resulted in the virtual absence of motor vehicle traffic and sharply reduced manufacturing activity for several weeks. Le et al. report some of the anticipated and unanticipated effects that this had on air pollution there, including unexpectedly high levels of particulate matter abundances and severe haze formation in some areas. This natural experiment will help in the assessment of air pollution mitigation strategies. Science , this issue p. 702
1 November 2016 in Journal of the Atmospheric Sciences
Over the past decade, the number of studies that investigate aerosol–cloud interactions has increased considerably. Although tremendous progress has been made to improve the understanding of basic physical mechanisms of aerosol–cloud interactions and reduce their uncertainties in climate forcing, there is still poor understanding of 1) some of the mechanisms that interact with each other over multiple spatial and temporal scales, 2) the feedbacks between microphysical and dynamical processes and between local-scale processes and large-scale circulations, and 3) the significance of cloud–aerosol interactions on weather systems as well as regional and global climate. This review focuses on recent theoretical studies and important mechanisms on aerosol–cloud interactions and discusses the significances of aerosol impacts on radiative forcing and precipitation extremes associated with different cloud systems. The authors summarize the main obstacles preventing the science from making a leap—for example, the lack of concurrent profile measurements of cloud dynamics, microphysics, and aerosols over a wide region on the observation side and the large variability of cloud microphysics parameterizations resulting in a large spread of modeling results on the modeling side. Therefore, large efforts are needed to escalate understanding. Future directions should focus on obtaining concurrent measurements of aerosol properties and cloud microphysical and dynamic properties over a range of temporal and spatial scales collected over typical climate regimes and closure studies, as well as improving understanding and parameterizations of cloud microphysics such as ice nucleation, mixed-phase properties, and hydrometeor size and fall speed.
28 March 2016 in Proceedings of the National Academy of Sciences
Significance: Although black carbon (BC) represents a key short-lived climate forcer, its direct radiative forcing remains highly uncertain. The available results from available studies of absorption enhancement of BC particles during atmospheric aging are conflicting. Using a novel environmental chamber method, we have, for the first time to our knowledge, quantified the aging and variation in the optical properties of BC particles under ambient urban conditions representative of developed and developing countries. Our results indicate that BC under polluted urban environments could contribute significantly to both pollution development and large positive radiative forcing, implying that reduction of BC emissions under polluted environments achieves a cobenefit in simultaneously controlling air pollution and protecting climate, especially for developing countries.