Air pollution levels in the United States have decreased dramatically over the past decades, yet national racial-ethnic exposure disparities persist. For ambient fine particulate matter ( PM 2.5 ), we investigate three emission-reduction approaches and compare their optimal ability to address two goals: 1) reduce the overall population average exposure (“overall average”) and 2) reduce the difference in the average exposure for the most exposed racial-ethnic group versus for the overall population (“national inequalities”). We show that national inequalities in exposure can be eliminated with minor emission reductions (optimal: ~1% of total emissions) if they target specific locations. In contrast, achieving that outcome using existing regulatory strategies would require eliminating essentially all emissions (if targeting specific economic sectors) or is not possible (if requiring urban regions to meet concentration standards). Lastly, we do not find a trade-off between the two goals (i.e., reducing overall average and reducing national inequalities); rather, the approach that does the best for reducing national inequalities (i.e., location-specific strategies) also does as well as or better than the other two approaches (i.e., sector-specific and meeting concentration standards) for reducing overall averages. Overall, our findings suggest that incorporating location-specific emissions reductions into the US air quality regulatory framework 1) is crucial for eliminating long-standing national average exposure disparities by race-ethnicity and 2) can benefit overall average exposures as much as or more than the sector-specific and concentration-standards approaches.

The partitioning of available energy into surface sensible and latent heat fluxes impacts the accuracy of simulated near surface temperature and humidity in numerical weather prediction models. This case study evaluates the performance of the Weather Research and Forecasting (WRF) model on the simulation of surface heat fluxes using field observations collected from a surface flux tower in Oregon, USA. Further, WRF-modeled heat flux sensitivities to North American Mesoscale (NAM) and North American Regional Reanalysis (NARR) large-scale input forcing datasets; U.S. Geological Survey (USGS) and the Moderate Resolution Imaging Spectroradiometer (MODIS) land use datasets; Pleim-Xiu (PX) and Noah land surface models (LSM); Yonsei University (YSU) and Mellor-Yamada-Janjic (MYJ) planetary boundary layer (PBL) schemes using the Noah LSM; and Asymmetric Convective Model version 2 (ACM2) PBL scheme using PX LSM are investigated. The errors for simulating 2-m temperature, 2-m humidity, and 10-m wind speed were reduced on average when using NAM compared with NARR. Simulated friction velocity had a positive bias on average, with the YSU PBL scheme producing the largest overestimation in the innermost domain (0.5 km horizontal grid resolution). The simulated surface sensible heat flux had a similar temporal behavior as the observations but with a larger magnitude. The PX LSM produced lower and more reliable sensible heat fluxes compared with the Noah LSM. However, Noah latent heat fluxes were improved with a lower RMSE compared to PX, when NARR forcing data was used. Overall, these results suggest that there is not one WRF configuration that performs best for all the simulated variables (surface heat fluxes and meteorological variables) and situations (day and night).

We developed a hybrid chemical transport model and receptor model (CTM-RM) to conduct source apportionment of both primary and secondary PM2.5 (particulate matter ≤2.5 μm in diameter) at 36 km resolution throughout the U.S. State of Georgia for the years 2005 and 2007. This novel source apportionment model enabled us to estimate and compare associations of short-term changes in 12 PM2.5 source concentrations (agriculture, biogenic, coal, dust, fuel oil, metals, natural gas, non-road mobile diesel, non-road mobile gasoline, on-road mobile diesel, on-road mobile gasoline, and all other sources) with emergency department (ED) visits for pediatric respiratory diseases. ED visits for asthma (N = 49,651), pneumonia (N = 25,558), and acute upper respiratory infections (acute URI, N = 235,343) among patients aged ≤18 years were obtained from patient claims records. Using a case-crossover study, we estimated odds ratios per interquartile range (IQR) increase for 3-day moving average PM2.5 source concentrations using conditional logistic regression, matching on day-of-week, month, and year, and adjusting for average temperature, humidity, and holidays. We fit both single-source and multi-source models. We observed positive associations between several PM2.5 sources and ED visits for asthma, pneumonia, and acute URI. For example, for asthma, per IQR increase in the source contribution in the single-source model, odds ratios were 1.022 (95% CI: 1.013, 1.031) for dust; 1.050 (95% CI: 1.036, 1.063) for metals, and 1.091 (95% CI: 1.064, 1.119) for natural gas. These sources comprised 5.7%, 2.2%, and 6.3% of total PM2.5 mass, respectively. PM2.5 from metals and natural gas were positively associated with all three respiratory outcomes. In addition, non-road mobile diesel was positively associated with pneumonia and acute URI.