The mining and processing of naturally occurring radioactive materials (NORMs) could result in elevated levels of natural radionuclides in the environment. The gold mining in the goldfields of the Witwatersrand Basin of South Africa has resulted in numerous tailing dams that have high concentrations of NORM bearing residue. The aim of this study was to evaluate the radioactivity levels in tailing dams, soils and rocks, and the consequential radiological exposure to the public in the gold mining areas of Gauteng Province, South Africa. The activity concentrations of ²³⁸U, ²³²Th, and ⁴⁰K were assessed using a gamma ray spectrometer (RS-230), and the activity concentrations ranges in the mine tailings were 209.95–2578.68 Bq/kg, 19.49–108.00 Bq/kg, and 31.30–626.00 Bq/kg, respectively. The radionuclides show significant spatial variability in soils, with high activities recorded in soils located in close proximity to tailings although regionally, the soil radioactivity levels mainly depend on the chemistry of the underlying rocks. The estimated annual effective doses were higher than the recommended regulatory limit of 0.25 mSv/y in particular tailing dams and soil impacted by tailings. Therefore, to ensure the protection of people and the environment, further monitoring and regulatory control measures targeting these areas are required.

The history of gold mining in the Witwatersrand Basin has led to exponential growth in the economy, residential development, and the abundance of radionuclides in the environment, including the water system. This study aimed to evaluate the radionuclide levels in drinking water (municipal water and groundwater) and the health risks associated with the ingestion of the water in the communities of the West Rand region of Gauteng Province. The activity concentrations of uranium, radium, and thorium radioisotopes were established through alpha spectrometry and the activities were subsequently used to assess the health impacts. The results indicated that the groundwaters contain elevated activities of most radionuclides owing to prolonged periods of water–rock interactions. Similarly, the highest annual effective doses were recorded in groundwaters with a range of 0.0237–0.3106 mSv/yr, with most samples exceeding the WHO- and EU-prescribed limits of 0.1 mSv/yr. Cancer morbidity and mortality risks were higher in females than in males due to the higher life expectancy of females. Nonetheless, all morbidity and mortality risks were well below the USEPA radiological risk limit of 0.001. Based on the findings of this study, continuous monitoring is paramount to ensure that the activities remain below recommended regulatory limits.

This paper presents a comprehensive hydrogeological investigation that involves field work, aquifer test, hydrogeochemical analysis, environmental isotope analysis, and interpretations around a proposed nuclear power facility in South Africa. The study was undertaken to test the complementarity of the various methods in the coastal aquifer and to verify the hydrogeological conditions within and around the site. The study revealed the presence of two types of aquifers: an upper primary aquifer made up of the Cenozoic deposits of the Algoa Group, and a deeper fractured aquifer made of the Palaezoic Table Mountain Group (TMG) metasedimentary rocks. Owing to ductile deformation in the form of folding, the fractured quartzite and shale aquifers resulted in an artesian condition, often characterized by slightly acidic (pH ≤ 6) and iron-rich groundwater. The most important hydrogeochemical processes responsible for the observed changes in the hydrochemical composition and facies are mineral dissolution, ion exchange and mixing. The environmental isotope results suggest that all groundwater samples are characterized by a depleted δ¹⁸O and δ²H signal, indicating high latitude moisture source (southern polar region) and recharge from rainfall, with no or minimal evaporation before and during infiltration. Similarities in the stable isotope signatures between the deeper and shallow aquifer confirm the presence of a strong hydraulic link. The residence time of groundwater in the aquifers underlying the proposed nuclear power plant is estimated using tritium (³H) and ¹⁴C, and the results indicate that in the shallow aquifer it ranges from recent recharge to 50 years, and in the deeper aquifer, it ranges from 430 ± 5 years to 1000 ± 10 years, which exists in a quasi-pristine condition.

Coal mining and combustion have the potential to increase exposure to radon, a form of radioactive gas recognized as one of the major contributors to lung cancer incidents. In South Africa, coal is used as the primary energy source for producing electricity and for heating, predominantly in informal settlements and township communities. Most of the existing coal-fired power plants are found in the Mpumalanga province. This paper presents long-term radon (²²²Rn) measurements in dwellings surrounding coal mining centres in the Mpumalanga province and evaluates their contributions to indoor radon exposures. The indoor radon measurements were conducted using solid-state nuclear track detectors and were performed during warm and cold seasons. It was found that the overall indoor radon activity concentrations ranged between 21 Bq/m³ and 145 Bq/m³, with a mean value of 40 Bq/m³. In all the measured dwellings, the levels were below the WHO reference level of 100 Bq/m³ and 300 Bq/m³ reference level recommended by the IAEA and ICRP, with the exception of one dwelling that was poorly ventilated. The results reveal that individuals residing in the surveyed homes are not exposed to radon levels higher than the WHO, ICRP, and IAEA reference levels. The main source influencing indoor radon activity concentrations was found to be primarily the concentration of uranium found in the geological formations in the area, with ventilation being an additional contributing factor of radon levels in dwellings. To maintain good air quality in homes, it is recommended that household occupants should keep their dwellings well ventilated to keep indoor radon levels as low as possible.

Mine tailing dumps are one of the prevalent environmental legacies of gold mining in the Witwatersrand Basin, which are typically enriched in Naturally Occurring Radioactive Materials (NORMs). This study aimed to evaluate radionuclide levels and the associated exposure risks from external gamma radiation in mine tailing dumps and soils near residential areas in historical mining towns of the upper West Rand region in Gauteng Province, South Africa. The activity concentrations of various radioisotopes were measured using Gamma spectrometry. The activity concentrations of ²³⁸U (87.2–449 Bq/kg), ²³⁵U (4.19–21.6 Bq/kg), ²³⁴U (88.9–458 Bq/kg), ²³²Th (12.3–78.1 Bq/kg), ²²⁸Th (12.5–81 Bq/kg), ²²⁸Ra (12.3–78.1 Bq/kg), ²²⁶Ra (14.5–2650 Bq/kg) and ⁴⁰ K (1.89–125 Bq/kg) were highly variable in all samples. All but ²²⁶Ra activity concentrations fell below the prescribed limits of 500 Bq/kg and 50 000 Bq/kg (⁴⁰ K). The presence of tailings material in some of the sampled soils signifies the extensive environmental impacts of tailings on the surrounding areas and the potential radiological risks to public health. Annual effective dose estimates ranged between 0.062 and 0.282 mSv/y, and fall far below the IAEA and NCRP’s 1 mSv/y regulatory limit, albeit most samples’ estimates exceeding UNSCEAR’s 0.08 mSv/y global average value. It is recommended that continuous monitoring of different geological materials near residential areas be established to ensure compliance with regulatory standards and the public’s protection from radiological damage. Moreover, mine tailings dumps rehabilitation is crucial to prevent further environmental contamination and lower radiological risks to public health.