Quantum de Haas-van Alphen oscillations and semiclassical angular magnetoresistance oscillations are observed in the quasi-two-dimensional organic metal κ-(BETS)₂GaCl₄. The behavior of these oscillations attests to the existence of two cylindrical Fermi surface sheets with axes perpendicular to the conducting plane. The cross-sectional areas of these cylinders in the conducting plane are equal to about 20 and 100% of the corresponding cross section of the Brillouin zone. It is shown that the many-particle interaction can be suppressed significantly in this compound.

The interlayer and intralayer resistances and Shubnikov-de Haas oscillations in a new dual-layered quasi-two-dimensional organic metal (BETS)₄CoBr₄(C₆H₄Cl₂) with a periodically varying structure of cation layers have been studied. It has been shown that the interlayer resistivity corresponds to an incoherent or weakly incoherent transport regime. The oscillations of the magnetoresistance have been described by a model of a chain of coherent magnetic breakdown orbits taking into account the quantum interference effect. The behavior of the interlayer transport, as well as quantum oscillations, is in good agreement with the theoretical calculations of the band structure.