In the past three decades, China has built more than 87 000 dams with a storage capacity of ≈6560 km3 and the total surface area of inland water has increased by 6672 km2. Leaching of N from fertilized soils to rivers is the main source of N pollution in China, but the exposure of a growing inland water area to direct atmospheric N deposition and N leaching caused by N deposition on the terrestrial ecosystem, together with increased N deposition and decreased N flow, also tends to raise N concentrations in most inland waters. The contribution of this previously ignored source of N deposition to freshwaters is estimated in this study, as well as mitigation strategies. The results show that the annual amounts of N depositions ranged from 4.9 to 16.6 kg · ha−1 · yr−1 in the 1990s to exceeding 20 kg · ha−1 · yr−1 in the 2010s over most of regions in China, so the total mass of ΔN (the net contribution of N deposition to the increase in N concentration) for lakes, rivers and reservoirs change from 122.26 Gg N · yr−1 in the 1990s to 237.75 Gg N · yr−1 in the 2010s. It is suggested that reducing the N deposition from various sources, shortening the water-retention time in dams and decreasing the degree of regulation for rivers are three main measures for preventing a continuous increase in the N-deposition pollution to inland water in China.
1 September 2010 in Journal of Hazardous Materials
Protecting groundwater from nitrogen contamination is an important public-health concern and a major national environmental issue in China. In this study, we monitored water quality in 29 wells from 2009 to 2010 in a village in Shanghai city, whick belong to typical rural-urban continuum in China. The total N and NO3-N exhibited seasonal changes, and there were large fluctuations in NH4-N in residential areas, but without significant seasonal patterns. NO2-N in the water was not stable, but was present at high levels. Total N and NO3-N were significantly lower in residential areas than in agricultural areas. The groundwater quality in most wells belonged to Class III and IV in the Chinese water standard, which defines water that is unsuitable for human consumption. Our health risk assessments showed that NO3-N posed the greatest carcinogenic risk, with risk values ranging from 19×10−6 to 80×10−6, which accounted for more than 90% of the total risk in the study area.
Karst topography covers more than 1/3 of the People's Republic of China in area. The porous, fissured, and soluble nature of the underlying karst bedrock (primarily dolomite and limestone) leads to the formation of underground drainage systems. Karst conduit networks dominate this system, and rainfall takes a crucial role on water cycle at China karst area. Nitrogen loss from the karst system is of particular concern, with regard to nutrient use efficiency as well as water quality, as much of the karst system, including steeply sloping terrain, is used for intensive agriculture. We use simulated rainfall experiments to determine the relationship between rainfall and nitrogen loss at typical karst slope land and then estimate nitrogen loss from the karst soil. The results show that both surface runoff and subsurface runoff have a significant linear correlation with rainfall at all studied sites. Subsurface runoff is larger than surface runoff at two karst sites, while the opposite is true at the non‐karst site. Exponential function satisfactorily described the correlation between rainfall and nitrogen concentrations in runoff. Nitrates accounted for 60%–95% of the dissolved nitrogen loss (DN, an index of N‐loss in this research). The estimated annual N‐loss load varies between 1.05 and 1.67 Tg N/year in the whole karst regions of China from 1961 to 2014. Approximately, 90% of the N‐loss load occurred during the wet season, and 90% of that passed through the subsurface. Understanding the processes and estimating N‐loss is highly valuable in determining long‐term soil security and sustainability in karst regions.