Self-assembled architectures of soft matter have fascinated scientists for centuries due to their unique physical properties originated from controllable orientational and/or positional orders, and diverse optic and photonic applications. If one could know how to design, fabricate, and manipulate these optical microstructures in soft matter systems, such as liquid crystals (LCs), that would open new opportunities in both scientific research and practical applications, such as the interaction between light and soft matter, the intrinsic assembly of the topological patterns, and the multidimensional control of the light (polarization, phase, spatial distribution, propagation direction). Here, we summarize recent progresses in self-assembled optical architectures in typical thermotropic LCs and bio-based lyotropic LCs. After briefly introducing the basic definitions and properties of the materials, we present the manipulation schemes of various LC microstructures, especially the topological and topographic configurations. This work further illustrates external-stimuli-enabled dynamic controllability of self-assembled optical structures of these soft materials, and demonstrates several emerging applications. Lastly, we discuss the challenges and opportunities of these materials towards soft matter photonics, and envision future perspectives in this field.

Circularly polarized luminescent (CPL) materials have received significant attention in the field of fundamental science recently. These materials offer substantial advancement of technological applications, such as optical data storage, displays, and quantum communication. Various strategies have been proposed in self‐assembled materials consisting of inorganic, organic, and hybrid systems, particularly in the chiral orientationally ordered soft matter systems (e.g., chiral liquid crystals (LCs) and LC polymers). However, developing scientific approaches to achieve the pronounced and steerable circularly polarized light emission remains challenging. Herein, we present a comprehensive review on the recent development of CPL materials based on chiral LCs, including thermotropic LCs (cholesteric LCs and bent‐core LCs), lyotropic LCs (nanocellulose LCs and polyacetylene‐based LCs), and LC polymers (cholesteric LC‐based polymers, helical nanofibers, and helical network). In addition, the fundamental mechanisms, design principles, and potential applications based on these chiral LCs and LC polymers in soft matter systems are systematically reviewed. This review summarizes with a prospect on the latent challenges, which can strengthen our understanding of the basic principles of CPL in chiral orientationally ordered soft matter systems and provide a new insight into the progress in several fields, such as chemistry, materials science, optics, electronics, and biology.

A non-reciprocity sensor based on a layered structure with multitasking is proposed, which realizes biological detection and angle sensing. Through an asymmetrical arrangement of different dielectrics, the sensor obtains non-reciprocity on the forward and backward scales, thus achieving multi-scale sensing in different measurement ranges. The structure sets the analysis layer. Injecting the analyte into the analysis layers by locating the peak value of the photonic spin Hall effect (PSHE) displacement, cancer cells can accurately be distinguished from normal cells via refractive index (RI) detection on the forward scale. The measurement range is 1.569∼1.662, and the sensitivity (S) is 2.97 × 10⁻² m/RIU. On the backward scale, the sensor is able to detect glucose solution with 0∼400 g/L concentrations (RI = 1.3323∼1.38), with S = 1.16 × 10⁻³ m/RIU. When the analysis layers are filled with air, high-precision angle sensing can be achieved in the terahertz range by locating the incident angle of the PSHE displacement peak; 30°∼45°, and 50°∼65° are the detection ranges, and the highest S can reach 0.032 THz/°. This sensor contributes to detecting cancer cells and biomedical blood glucose and offers a new way to the angle sensing.