Dissecting Cooper Pairs: Angle-resolved photoemission spectroscopy (ARPES) is used in the study of the electronic structure of complex materials. Recently, time-resolved ARPES has become possible, where the state of the system is excited by a short “pump” pulse, and ARPES is performed using a second “probe” pulse applied after varying times.Smallwoodet al.(p.1137) used this technique to study the recombination of Cooper pairs—the fundamental charge carriers in superconductors—in a cuprate high-temperature superconductor.
27 June 2011 in Proceedings of the National Academy of Sciences
The Landau–Fermi liquid picture for quasiparticles assumes that charge carriers are dressed by many-body interactions, forming one of the fundamental theories of solids. Whether this picture still holds for a semimetal such as graphene at the neutrality point, i.e., when the chemical potential coincides with the Dirac point energy, is one of the long-standing puzzles in this field. Here we present such a study in quasi-freestanding graphene by using high-resolution angle-resolved photoemission spectroscopy. We see the electron–electron and electron–phonon interactions go through substantial changes when the semimetallic regime is approached, including renormalizations due to strong electron–electron interactions with similarities to marginal Fermi liquid behavior. These findings set a new benchmark in our understanding of many-body physics in graphene and a variety of novel materials with Dirac fermions.
A universal high energy anomaly in the single particle spectral function is reported in three different families of high temperature superconductors by using angle-resolved photoemission spectroscopy. As we follow the dispersing peak of the spectral function from the Fermi energy to the valence band complex, we find dispersion anomalies marked by two distinctive high energy scales, and . marks the energy above which the dispersion splits into two branches. One is a continuation of the near parabolic dispersion, albeit with reduced spectral weight, and reaches the bottom of the band at the point at . The other is given by a peak in the momentum space, nearly independent of energy between and . Above , a bandlike dispersion reemerges. We conjecture that these two energies mark the disintegration of the low-energy quasiparticles into a spinon and holon branch in the high cuprates.
We present in-depth measurements of the electronic band structure of the transition-metal dichalcogenides (TMDs) and using angle-resolved photoemission spectroscopy, with focus on the energy splittings in their valence bands at the point of the Brillouin zone. Experimental results are interpreted in terms of our parallel first-principles computations. We find that interlayer interaction only weakly contributes to the splitting in bulk , resolving previous debates on its relative strength. We additionally find that across a range of TMDs, the band gap generally decreases with increasing magnitude of the valence-band splitting, molecular mass, or ratio of the out-of-plane to in-plane lattice constant. Our results provide an important reference for future studies of electronic properties of and and their applications in spintronics and valleytronics devices.
Revealing spin-orbit coupling in a cuprate: Strong coupling between the spin and orbital degrees of freedom is crucial in generating the exotic band structure of topological insulators. The combination of spin-orbit coupling with electronic correlations could lead to exotic effects; however, these two types of interactions are rarely found to be strong in the same material. Gotlieb et al. used spin- and angle-resolved photoemission spectroscopy to map out the spin texture in the cuprate Bi2212. Surprisingly, they found signatures of spin-momentum locking, not unlike that seen in topological insulators. Thus, in addition to strong electronic correlations, this cuprate also has considerable spin-orbit coupling. Science , this issue p. 1271