Metalens are planar lenses composed of the subwavelength arrays, which have unconventional and versatile functionalities to manipulate the light fields compared with the traditional lens. It is noted that the most metalens are designed in a monochromatic mode in the visible or mid-infrared range (mid-IR), however, the broadband range is needed in many practical applications, such as spectroscopy, sensing, and imaging. Here, we design and demonstrate a broadband achromatic dielectric metalens in the mid-IR range of 4 µm–5 µm for near diffraction-limited (1.0 λ ) focusing. The broadband achromatic propagation and focusing of the metalens are designed and simulated by constructing and optimizing the phase profile. The Pancharatnam-Berry (P-B) phases of all the elements contribute to the main phase increment of the whole phase profile of the metalens. The additional phase is constructed and optimized by using the random search algorithm to obtain the optimized size of all the elements. The focusing efficiency of the achromatic metalens is also optimized and averaged as the result of phase optimization within a wide band for the building elements, while it is lowered comparing with the regular metalens without broadband achromatic designing. Using this combined designing approach, various flat achromatic devices with the broadband metalens can find a new way for full-color detection and imaging.
22 January 2019 in The Journal of Physical Chemistry Letters
Optical trapping and manipulation of nanoparticles (NPs) have been widely used in nanotechnology and biology. Here, we demonstrate an optically directed assembly (ODA) route for bottom-up fabrication of stable nanostructured grating patterns in solution using laser standing evanescent wave (LSEW) fields. The control mechanism is the intriguing cooperative action of the periodically line-centered attractive optical gradient force and the near field dipolar coupling force induced by LSEW, which leads to assembly of the colloidal silver NPs into robust grating patterns within minutes. The anisotropic polarization nature of the grating patterns was studied further by examining the morphology correlation of the surface-enhanced Raman scattering (SERS)-based signal amplification. We show the LSEW ODA method can optimize and stabilize the strongest dipolar coupling style among the NPs during pattern assembly. These results advance the further understanding of ODA of colloid NPs and might have many potential applications in SERS, catalysis, nanophotonics and nano-fabrication.
Nano‐patterned colloidal plasmonic metasurfaces are capable of manipulation of light at the subwavelength scale. However, achieving controllable lithography‐free nano‐patterning for colloidal metasurfaces still remains a major challenge, limiting their full potential in building advanced plasmonic devices. Here, we demonstrate plasmonic field guided patterning (PFGP) of ordered colloidal metallic nano‐patterns using orthogonal laser standing evanescent wave (LSEW) fields. We achieved colloidal silver nano‐patterns with a large area of 30 mm 2 in <10 min by using orthogonal LSEW fields with a non‐focused ultralow fluence irradiation of 0.25 W cm −2 . The underlying mechanism of the formation of the nano‐patterns is the light‐induced polarization of the nanoparticles (NPs), which leads to a dipole‐dipole interaction for stabilizing the nano‐pattern formation, as confirmed by polarization‐dependent surface‐enhanced Raman spectroscopy. This optical field‐directed self‐assembly of NPs opens an avenue for designing and fabricating reconfigurable colloidal nano‐patterned metasurfaces in large areas.