To effectively optimize the mechanical behavior of a traditional anti-slide pile and reduce environmental destruction, a new method for slope reinforcement by a spatial arc crown beam composite supporting structure was proposed. First, a numerical model was validated through lab-scale model test data obtained herein, and then a full-scale numerical model was created for an in-depth understanding of the distribution regularity of displacement along the pile, the soil pressure, the crown beam stiffness, and so on. The results demonstrated that: (1) The spatial arc crown beam is simplified to a two-hinged arch, and the maximum value of the bending moment in the arc crown beam is about one-third of the straight crown beam through theoretical calculation. (2) The spatial arc crown beam redistributes the load sharing among different piles, and the extreme bending moment of other piles varies within 10% along the downhill direction except for the piles at the slope foot. (3) Bending moments are close to zero at the pile end, and the anti-slide pile can be simplified as a vertical beam with one end fixed and the other end hinged. (4) The axial force in the spatial arc crown beam is always presented as pressure, so the crown beam can make full utilization of the compression resistance of concrete. (5) The distribution characteristic of soil pressure in front of the pile at the arch foot is different from that in other positions, and the stable soil at the slope foot provides greater soil resistance for anti-piles. (6) As the crown beam stiffness is above five times the reference value, the axial force of the crown beam tends to be stable, and as the crown beam stiffness increases continually, the maximum value of M_y is −1013.13 kN·m, and the constraining effect of the crown beam is gradually weakened.