This study aimed at understanding the background concentration level of tritium in precipitation in southern Japan, where precipitation samples were collected monthly in 2022 in Okinawa and Kagoshima. Tritium concentration in monthly precipitation collected in Okinawa since 2014 ranged from 0.05 to 0.39 Bq per L with the mean value (2015–2022) of 0.15 ± 0.06 Bq per L. That of Kagoshima since 2022 ranged from < 0.11 to 0.58 Bq per L with the mean value of 0.30 ± 0.13 Bq per L. Our observed values were summarized with reported values, from which a clear latitude effect for tritium concentration was found in precipitation of southern Japan.

Surface collection efficiency (SCE) of a cellulose membrane filter (CMF) and a cellulose-glass fiber filter used in environmental monitoring for alpha-emitting radionuclides from nuclear facilities and natural radioactivity sources was evaluated for particles in the size range of 0.03–0.1 μm at different levels of face velocity. The SCE of the CMF was higher than that of the cellulose-glass fiber filter, and only the membrane filter showed the dependence of SCE on the particle size at higher face velocity. The use of the CMF at higher face velocity in environmental radioactivity monitoring leads to measurements of the background alpha spectrum with more degradation under the changing particle size condition in the atmosphere. Consequently, that fact needs to be taken into account, along with the expected particle size distribution and concentration of the airborne radioactivity being sampled, when selecting a face velocity to achieve the best possible detection limit.

Portable-type electrostatic-collection radon monitors (RAD7) are often used for in-situ measurements of radon in water. In this study, we evaluated the calibration factors and their uncertainties for two RAD7 monitors based on comparative measurements with the liquid scintillation counting method. In the first experiment, we found that both RAD7 monitors had relatively large uncertainties due to leakage of radon gas that bubbled from the gaps between the lids of the desiccant container and the glass vial. Therefore, for the second experiment, these gaps were closed as much as possible using parafilm and clay, respectively. As a result, the relative uncertainties for both RAD7 monitors were significantly decreased. Furthermore, we collected spring water samples to confirm the reliability of radon concentrations. After closing the leakage point, the uncertainty of radon concentrations in spring water we measured using the typical protocol of the RAD7 were significantly lower, which improves the measurement.

The combustion process of the organically bound tritium (OBT) analysis method is difficult and requires sophisticated techniques. For ease, safety, and reproducibility a semi-automatic combustion system was developed. An arbitrary combustion program that prevents sudden ignition was devised and combustion tests were conducted. Analytical test runs were conducted using fish standard samples to confirm the validity of the developed system. The test values were compared with values obtained with another analysis method, and the recovery rate of the combustion water was evaluated. The results confirmed that the analytical values obtained with this combustion system were equivalent to those obtained with another analytical method and were valid for OBT analysis.

This article mainly discusses tritium concentrations in monthly precipitation at Hiroshima City during 2021. The tritium concentrations, which were measured with a low background liquid scintillation counter, fluctuated from 0.16 to 0.78 Bq L−1. Additionally, hydrogen and oxygen stable isotopes and ionic species were measured in order to characterize precipitation, and their trends including tritium concentrations were compared with data collected in other regions of Japan in previous studies. Although the results showed the characteristics of precipitation were similar to those observed in the other regions, the tritium concentrations were found to be contrary to behavior expected from the latitude effect and some of the observed ionic components were suggested to be continental in origin. Since these results are not common at other sites in Japan, the tritium concentration in the westernmost region of Honshu, including Hiroshima City, may be influenced by Asian continental influences.

The concentration of the radioactive cesium (134Cs and 137Cs) in soils and in atmospheric fallouts has been measured at the Koriyama campus, Nihon University, after the Fukushima Dai-ichi Nuclear Power Plant accident for 13 y, from October 2011 till September 2023 and now ongoing. The concentration of them decreased very rapidly due to decontamination activities and weathering effects, with an environmental half-life of 1.21 and 2.82 y in soils, with those of 1.58 and 2.08 y in atmospheric fallouts for 134Cs and 137Cs, respectively. The behavior of the decrease was not simple, due to particles raised from the surface soil in wooded areas that had not been thoroughly decontaminated or that had been accumulated due to the re-release of radioactive cesium by trees after decontaminated activity.