Tunable attosecond pulses are necessary for various attosecond resolved spectroscopic applications, which can potentially be obtained through the tuning of high harmonic generation. Here we show theoretically, using the time-dependent Schrödinger equation and strong field approximation, a continuously tunable spectral shift of high-order harmonics by exploiting the interaction of two delayed identical infrared (IR) pulses within the single-atom response. The tuning spans more than twice the driving frequency (∼2ω) range, for several near-cutoff harmonics, with respect to only one control parameter: the change in delay between the two IR pulses. We show that two distinct mechanisms contribute to the spectral shift of the harmonic spectra. The dominant part of the spectral shift of the harmonics is due to the modulation of the central frequency of the composite IR-IR pulse with respect to delay. The second contribution comes from the non-adiabatic phase-shift of the recolliding electron wavepacket due to the change in amplitude of the subcycle electric field within the double pulse envelope. For optical few-cycle pulses this scheme can produce tunable attosecond pulse trains (APT), and in the single-cycle regime the same can be used for tuning isolated attosecond pulses (IAP). We quantify the dependence of tuning range and tuning rate on the laser pulse duration. We envision that the proposed scheme can be easily implemented with compact in-line setups for generating frequency tunable APT/IAP.

We introduce an ultra-thin attosecond optical delay line based on controlled wavefront division of a femtosecond infrared pulse after transmission through a pair of micrometer-thin glass plates with negligible dispersion effects. The time delay between the two pulses is controlled by rotating one of the glass plates from absolute zero to several optical cycles, with 2.5 as to tens of attosecond resolution with 2 as stability, as determined by interferometric self-calibration. The performance of the delay line is validated by observing attosecond-resolved oscillations in the yield of high harmonics induced by time delayed infrared pulses, in agreement with a numerical simulation for a simple model atom. This approach can be extended in the future for performing XUV-IR attosecond pump–probe experiments.

High harmonic generation (HHG) from atoms near a plasmonic nanostructure interacting with a relatively low intensity driving laser field is a promising candidate for table top attosecond pulse source. The effect of carrier envelope phase (CEP) of the few cycle driving pulse on inhomogeneous high harmonics generation is well studied in literature, for example, the harmonic cut-off can be efficiently controlled by tuning the CEP. Here, we show selective enhancements of harmonic spectra due to half-cycle cutoff (HCO) which is highly sensitive to the CEP, in both spatially homogeneous and inhomogeneous driving laser fields. Essentially the selective enhancement of spectral structures results from contributions of both short and long trajectories in certain HCO regions. Compared to the homogeneous HHG in the presence of inhomogeneity, these enhanced groups eventually merge to the background with the increase of the strength of inhomogeneity. This limits the maximum possible tunability of selective enhancement. Further, near cut-off harmonics can be a good candidate to produce isolated attosecond pulses, with substantial control via CEP of the driving laser pulse along with the strength of inhomogeneity.