We have studied the compound nucleus probability, the survival probability, and the evaporation residue cross sections for 6645 projectile-target combinations to synthesize the superheavy nuclei with atomic numbers –126 in the light of the entrance channel effects such as mass asymmetry, charge asymmetry, isospin asymmetry, non-compound nuclear fission probability, and Businaro-Gallone mass asymmetry. The role of quasifission in every reaction has also been considered. Decay chains of various superheavy nuclei produced from the reactions are portrayed as well. The most striking results are that the measured evaporation residue cross sections are of the order of picobarns, whereas the proposed reactions can yield up to microbarn cross sections for the superheavy nuclei with . We suggest future experiments may utilize these hot fusion reactions to synthesize new elements () or to study the properties of the known superheavy nuclei in greater detail. In particular, a proposed reaction containing both projectiles and targets that are naturally abundant, for example, , yields evaporation residue cross sections as high as 31 nb. The presently available experimental setup can test the prediction with ease to make a dream come true by putting a footstep into the eighth row of the periodic table.
We study the quasifission and fusion-fission lifetimes for a number of fusion reactions used to synthesize the superheavy element using a statistical method within the framework of the dinuclear system model. In particular, influence of the target orientation and angular momentum on such lifetimes have been investigated. The quasifission and fusion-fission lifetimes have been compared very well with that of available experiments on successful superheavy element synthesis. We notice further the predicted quasifission and fusion-fission lifetimes of the projectile-target combinations used for the synthesis of the superheavy element also show the similar trend. Furthermore, the fusion-fission lifetime is seen to somewhat decrease with the increase of the angular momentum as well as beam energy. Little effect is seen on fusion barrier of the reaction and fission barrier of superheavy compound nucleus. Variation of quasifission lifetime is also not much with orientation angle, beam energy and fission barrier of the superheavy compound nuclei. Hence, this lifetime study does not provide any good reason why the attempted reactions have failed to synthesize the superheavy nuclei . Furthermore, consideration of the fusion barrier, fissility, mass asymmetry, deformation parameter, fission barrier, etc., leads us to reveal that optimal colliding energy is important to have the largest evaporation residue cross section for any chosen reaction so that it is well within the measurable limit for a specific experimental set up.
1 February 2000 in Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
Synthesizing any elements in the eighth period using either cold or hot fusion reactions remains a big challenge to date. The quasifission mechanism restricts complete fusion to an indeterminably low evaporation residue (ER) cross-section for superheavy nuclei. The entrance channel parameters of the heavy-ion reaction, the fission barrier of the compound nucleus, the deformation parameters of the projectile and target nuclei, and the kinetic energy of the projectile are mainly responsible for governing the scale of the quasifission. The role of these factors has been examined explicitly by the experimental ER cross-sections. Thorough comparisons lead us to infer that the entrance channel criteria contribute to a much lower extent than the deformation parameters do. The effect of deformation can be categorized into four rules as validated by all the reactions used except one Uue. The null result from this reaction is explained by the improper choice of the projectile energy, as shown theoretically by means of a statistical model approach, which is valid for a system having a large nucleon number so as to intrinsically have a high density of excited states. The optimal selection of the beam energy sets another rule. Therefore, these five rules can be treated as the rules of thumb for synthesizing the superheavy elements. Application of the first four rules can enable us primarily to spot a suitable reaction, and finally, exploitation of the fifth rule chooses the most appropriate reaction at a preferable excited energy to achieve the highest ER cross-section for a superheavy element.
The x-ray spectra of different targets (Cu, Zn, and Ge) induced by 3–5 MeV/u Si projectile ions have been measured to determine the -shell ionization cross section. A significant difference is observed between the measurements and theoretical estimates, with the latter being about 50% below the experimental results. This underestimation is attributed to the charge exchange from the target shell to projectile and shells. Such an observation can only be possible if the projectile ions attain up to H- and He-like charge states. Corresponding projectile charge state fractions have been evaluated from the Lorentzian charge state distribution, where the mean charge state is taken from the Fermi gas model [W. Brandt et al., Phys. Rev. Lett. 30, 358 (1973)] and the width from the Novikov and Teplova approach [ Phys. Lett. A 378, 1286 (2014)]. The sum of the direct ionization cross section and capture cross sections gives a good agreement with the measured cross sections. Furthermore, we have validated this methodology with available data for a Si ion on Ti target. Such results may be useful in many solid target-based applications.