The vertical temperature profile in the lowest 1000 m of the atmosphere determines a number of important physical processes and meteorological phenomena such as high concentrations of anthropogenic air pollutants in urban areas. Long-term monitoring of temperature profiles at high vertical and temporal resolution has only become feasible only recently with the introduction of affordable angular scanning microwave temperature profile radiometers. In this study, we analyzed 2 years of continuous temperature profile measurements with the MTP-5HE instrument in the urbanized coastal Bergen valley, Norway. The data have a 10 min temporal and 50 m vertical spatial resolution, thus, constituting a unique data set for a microclimatic characterization of the atmosphere in this high-latitude valley. We studied a 2 year record of ground-based (G-) and elevated (E-) inversions, their dynamics and connection to large-scale circulations, and the links between the urban air quality and the temperature inversions. G-inversions are commonly observed during wintertime nocturnal hours. The local topographic features allow for the frequent occurrence of G-inversions, even during strong winds of up to 16 m/s. E-inversions exist mostly during spring and summer and only during unusual synoptic circulation with large-scale warm air advection directly above the valley. Events with high air pollution, identified based on measurements of NO2 and particulate matter concentrations, are highly dependent on the existence of G-inversions. Meteorological models poorly capture both G-inversions and E-inversions reducing their utility for the assessment of urban air quality and local weather forecasts.
20 January 2020 in Atmospheric Chemistry and Physics
Urban air quality is one of the most prominent environmental concerns for modern city residents and authorities. Accurate monitoring of air quality is difficult due to intrinsic urban landscape heterogeneity and superposition of multiple polluting sources. Existing approaches often do not provide the necessary spatial details and peak concentrations of pollutants, especially at larger distances from monitoring stations. A more advanced integrated approach is needed. This study presents a very high-resolution air quality assessment with the Parallelized Large-Eddy Simulation Model (PALM), capitalising on local measurements. This fully three-dimensional primitive-equation hydrodynamical model resolves both structural details of the complex urban surface and turbulent eddies larger than 10 m in size. We ran a set of 27 meteorological weather scenarios in order to assess the dispersion of pollutants in Bergen, a middle-sized Norwegian city embedded in a coastal valley. This set of scenarios represents typically observed weather conditions with high air pollution from nitrogen dioxide (NO2) and particulate matter (PM2.5). The modelling methodology helped to identify pathways and patterns of air pollution caused by the three main local air pollution sources in the city. These are road vehicle traffic, domestic house heating with wood-burning fireplaces and ships docked in the harbour area next to the city centre. The study produced vulnerability maps, highlighting the most impacted districts for each weather and emission scenario. Overall, the largest contribution to air pollution over inhabited areas in Bergen was caused by road traffic emissions for NO2 and wood-burning fireplaces for PM2.5 pollution. The effect of emission from ships in the port was mostly restricted to the areas close to the harbour and moderate in comparison. However, the results have contributed to implementation of measures to reduce emissions from ships in Bergen harbour, including provision of shore power.
Street-level urban air pollution is a challenging concern for modern urban societies. Pollution dispersion models assume that the concentrations decrease monotonically with raising wind speed. This convenient assumption breaks down when applied to flows with local recirculations such as those found in topographically complex coastal areas. This study looks at a practically important and sufficiently common case of air pollution in a coastal valley city. Here, the observed concentrations are determined by the interaction between large-scale topographically forced and local-scale breeze-like recirculations. Analysis of a long observational dataset in Bergen, Norway, revealed that the most extreme cases of recurring wintertime air pollution episodes were accompanied by increased large-scale wind speeds above the valley. Contrary to the theoretical assumption and intuitive expectations, the maximum NO2 concentrations were not found for the lowest 10 m ERA-Interim wind speeds but in situations with wind speeds of 3 m s−1. To explain this phenomenon, we investigated empirical relationships between the large-scale forcing and the local wind and air quality parameters. We conducted 16 large-eddy simulation (LES) experiments with the Parallelised Large-Eddy Simulation Model (PALM) for atmospheric and oceanic flows. The LES accounted for the realistic relief and coastal configuration as well as for the large-scale forcing and local surface condition heterogeneity in Bergen. They revealed that emerging local breeze-like circulations strongly enhance the urban ventilation and dispersion of the air pollutants in situations with weak large-scale winds. Slightly stronger large-scale winds, however, can counteract these local recirculations, leading to enhanced surface air stagnation. Furthermore, this study looks at the concrete impact of the relative configuration of warmer water bodies in the city and the major transport corridor. We found that a relatively small local water body acted as a barrier for the horizontal transport of air pollutants from the largest street in the valley and along the valley bottom, transporting them vertically instead and hence diluting them. We found that the stable stratification accumulates the street-level pollution from the transport corridor in shallow air pockets near the surface. The polluted air pockets are transported by the local recirculations to other less polluted areas with only slow dilution. This combination of relatively long distance and complex transport paths together with weak dispersion is not sufficiently resolved in classical air pollution models. The findings have important implications for the air quality predictions over urban areas. Any prediction not resolving these, or similar local dynamic features, might not be able to correctly simulate the dispersion of pollutants in cities.
The Pan-Eurasian Experiment (PEEX) Science Plan, released in 2015, addressed a need for a holistic system understanding and outlined the most urgent research needs for the rapidly changing Arctic-boreal region. Air quality in China, together with the long-range transport of atmospheric pollutants, was also indicated as one of the most crucial topics of the research agenda. These two geographical regions, the northern Eurasian Arctic-boreal region and China, especially the megacities in China, were identified as a “PEEX region”. It is also important to recognize that the PEEX geographical region is an area where science-based policy actions would have significant impacts on the global climate. This paper summarizes results obtained during the last 5 years in the northern Eurasian region, together with recent observations of the air quality in the urban environments in China, in the context of the PEEX programme. The main regions of interest are the Russian Arctic, northern Eurasian boreal forests (Siberia) and peatlands, and the megacities in China. We frame our analysis against research themes introduced in the PEEX Science Plan in 2015. We summarize recent progress towards an enhanced holistic understanding of the land–atmosphere–ocean systems feedbacks. We conclude that although the scientific knowledge in these regions has increased, the new results are in many cases insufficient, and there are still gaps in our understanding of large-scale climate–Earth surface interactions and feedbacks. This arises from limitations in research infrastructures, especially the lack of coordinated, continuous and comprehensive in situ observations of the study region as well as integrative data analyses, hindering a comprehensive system analysis. The fast-changing environment and ecosystem changes driven by climate change, socio-economic activities like the China Silk Road Initiative, and the global trends like urbanization further complicate such analyses. We recognize new topics with an increasing importance in the near future, especially “the enhancing biological sequestration capacity of greenhouse gases into forests and soils to mitigate climate change” and the “socio-economic development to tackle air quality issues”.
19 August 2021 in Atmospheric Chemistry and Physics
Many cities in the world experience significant air pollution from residential wood combustion. Such an advection–diffusion problem as applied to geographically distributed small-scale pollution sources presently does not have a satisfactory theoretical or modeling solution. For example, statistical models do not allow for pollution accumulation in local stagnation zones – a type of phenomena that is commonly observed over complex terrain. This study applies a Parallelized Atmospheric Large-eddy simulation Model (PALM) to investigate dynamical phenomena that control variability and pathways of the atmospheric pollution emitted by wood-burning household stoves. The model PALM runs at spatial resolution of 10 m in an urban-sized modeling domain of 29 km by 35 km with a real spatial distribution of the pollution source and with realistic surface boundary conditions that characterize a medium-sized urban area fragmented by water bodies and hills. Such complex geography is expected to favor local air quality hazards, which makes this study of general interest. The case study here is based on winter conditions in Bergen, Norway. We investigate the turbulent diffusion of a passive scalar associated with small-sized particles (PM2.5) emitted by household stoves. The study considers air pollution effects that could be observed under different policy scenarios of stove replacement; modern woodstoves emit significantly less PM2.5 than the older ones, but replacement of stoves is a costly and challenging process. We found significant accumulation of near-surface pollution in the local stagnation zones. The simulated concentrations were larger than the concentrations obtained only due to the local PM2.5 emission, thus indicating dominant transboundary contribution of pollutants for other districts. We demonstrate how the source of critical pollution can be attributed through model disaggregation of emission from specific districts. The study reveals a decisive role of local air circulations over complex terrain that makes high-resolution modeling indispensable for adequate management of the urban air quality. This modeling study has important policy-related implications. Uneven spatial distribution of the pollutants suggests prioritizing certain limited urban districts in policy scenarios. We show that focused efforts towards stove replacement in specific areas may have a dominant positive effect on the air quality in the whole municipality. The case study identifies urban districts where limited incentives would result in the strongest reduction of the population's exposure to PM2.5.