Biomass burning (BB) emits a large volume of trace gases and aerosols into the atmosphere, which can significantly affect the earth’s radiative balance and climate and has negative impacts on air quality and even human health. In late June 2017, an intense BB case, dominated by forest and savanna fires, occurred in Siberia, and it affected the air quality of Northeast China through long-range transport. Here, multisatellite remote-sensing products and ground-based PM_2.5 measurements are used to evaluate the influence of the Siberian smoky plume on Northeast China. The results show that the BB was intense at the early stage when the daily fire count and average fire radiative power exceeded 300 and 200 MW, respectively. The maximum daily fire count reached 1350 in Siberia, and the peak value of instantaneous fire radiative power was as high as 3091.5 MW. High concentrations of CO and aerosols were emitted into the atmosphere by the BB in Siberia. The maximum daily mean values of the CO column concentration and aerosol optical depth (AOD) increased by 3 × 10¹⁷ molec·cm² and 0.5 compared with that during the initial BB stage. In addition, the BB released a large number of absorptive aerosols into the atmosphere, and the UV aerosol index (UVAI) increased by five times at the peak of the event in Siberia. Under the appropriate synoptic conditions and, combined with pyroconvection, the smoky plume was lifted into the upper air and transported to Northeast China, affecting the air quality of Northeast China. The daily mean values of CO concentration, AOD, and UVAI in Northeast China increased by 6 × 10¹⁷ molec·cm², 0.5, and 1.4, respectively, after being affected. Moreover, the concentration of the surface PM_2.5 in Northeast China approximately doubled after being affected by the plume. The results of this study indicate that the air quality of Northeast China can be significantly affected by Siberian BBs under favorable conditions.

Biomass burning (BB) is a driving force for heavy haze in northeastern China (NEC) and shows distinct seasonal features. However, little is known about its climatological aspects, which are important for regional BB management and understanding BB effects on climate and environment. Here, the climatological characteristics of active fires and their dependence on land cover in NEC were studied using Moderate Resolution Imaging Spectroradiometer (MODIS) products. Moreover, the influence of meteorological factors on fire activities was explored. The number of fires was found to have increased significantly from 2003 to 2018; and the annual total FRP (FRP_tot) showed a generally consistent variation with fire counts. However, the mean fire radiative power for each spot (FRP_mean) decreased. Fire activity showed distinctive seasonal variations. Most fires and intense burning events occurred in spring and autumn. Spatially, fires were mainly concentrated in cropland areas in plains, where the frequency of fires increased significantly, especially in spring and autumn. The annual percentage of agricultural fires increased from 34% in 2003 to over 60% after 2008 and the FRP_tot of croplands increased from 12% to over 55%. Fires in forests, savannas, and grasslands tended to be associated with higher FRP_mean than those in croplands. Analysis indicated that the increasing fire count in NEC is mainly caused by agricultural fires. Although the decreasing FRP_mean represents an effective management of BB in recent years, high fire counts and FRP_tot in croplands indicate that the crop residue burning cannot be simply banned and a need instead for effective applications. More efforts should be made on clean utilization of straw. The accumulation of dry biomass, high temperature, and low humidity, and weak precipitation are conducive to the fire activities. This study provides a comprehensive analysis of BB in NEC and provides a reference for regional BB management and control.

The characteristics of turbulence in the planetary boundary layer (PBL) and the aerosol optical and radiative properties during haze and haze–fog mixed episodes on 22–27 January 2021, in Shenyang, a provincial city in Northeast China, were analyzed using meteorological and aerosol observations. During the haze episode, the hourly mean PM_2.5 concentration reached a maximum of 337 µg m⁻³ and visibility decreased to 1.6 km. The PM_2.5 concentration decreased gradually during the haze–fog mixed episode as a result of the scavenging effects of fog, but visibility mostly remained below 1 km owing to high ambient relative humidity (>90%). During the haze–fog mixed episode, an increasing proportion of PM_2.5 led to a higher ratio of the backward to the total scattering coefficient. As fog occurred, downward shortwave radiation arriving at the surface was significantly reduced, and upward longwave radiation increased and almost equaled the downward longwave radiation, which can be used as a good indicator for distinguishing haze and fog. Mechanical turbulence was weak during both episodes, and latent heat flux varied within a wider range during the haze–fog mixed episode. The PBL dynamic structure affected the vertical distribution of aerosols/fog droplets. Aerosol-rich layers appeared at altitudes below 0.5 km and above 0.6 km during the haze episode. The elevated aerosol layer was related to the aerosol transport from upstream polluted areas caused by strong upper-level turbulence, and it began to mix vertically after sunrise because of convective turbulence. Aerosols and fog droplets were mostly trapped in a shallower PBL with a height of 0.2–0.4 km during the haze–fog mixed episode because of weaker turbulence.

The influence of urbanization on the frequent winter aerosol pollution events in Northeast China is not fully understood. The Weather Research and Forecasting Model with Chemistry (WRF–Chem) coupled with urban canopy (UC) models was used to simulate the impact of urbanization on an aerosol pollution process in the Central Liaoning city cluster (CLCC), China. To investigate the main mechanisms of urban expansion and UC on the winter atmospheric environment and the atmospheric diffusion capacity (ADC) in the CLCC, three simulation cases were designed using land-use datasets from different periods and different UC schemes. A comparative analysis of the simulation results showed that the land-use change (LU) and both LU and UC (LUUC) effects lead to higher surface temperature and lower relative humidity and wind speed in the CLCC by decreasing surface albedo, increasing sensible heat flux, and increasing surface roughness, with a spatial distribution similar to the distribution of LU. The thermal effect leads to an increase in atmospheric instability, an increase in boundary layer height and diffusion coefficient, and an increase in the ADC. The LU and LUUC effects lead to a significant decrease in near-surface PM_2.5 concentrations in the CLCC due to changes in meteorological conditions and ADC within the boundary layer. The reduction in surface PM_2.5 concentrations due to the LU effect is stronger at night than during daytime, while the LUUC effect leads to a greater reduction in surface PM_2.5 concentrations during the day, mainly due to stronger diffusion and dilution caused by the effect of urban turbulence within different levels caused by the more complex UC scheme. In this study, the LU and LUUC effects result in greater thermal than dynamic effects, and both have a negative impact on surface PM_2.5 concentrations, but redistribute pollutants from the lower urban troposphere to higher altitudes.

Dust storms have large impacts on air quality and meteorological elements; however, their relationships with atmospheric greenhouse gases (e.g., CO₂) and radiation components remain uncertain. In this study, the co-variation of dust and CO₂ concentrations and its possible influencing mechanism are examined using observations at the Shangdianzi (SDZ) regional Global Atmosphere Watch (GAW) station along with simulations of the Vegetation Photosynthesis and Respiration Model coupled with the Weather Research and Forecasting model (WRF-VPRM), during two dust storm events on 15 and 28 March 2021. During these events, hourly CO₂ concentrations decreased by 40–50 ppm at SDZ while dust concentrations increased to 1240.6 and 712.4 µg m⁻³. The elevated dust increased diffusive shortwave irradiance by 50–60% and decreased direct shortwave irradiance by ~60% along with clouds. The dust events were attributed to the passages of two cold front systems over northern China. At SDZ, during the frontal passages, wind speed increased by 3–6 m s⁻¹, and relative humidity decreased by 50–60%. The CO₂ variations associated with the frontal systems were captured by the WRF-VPRM despite the overestimated surface CO₂ level at SDZ. Biogenic CO₂ flux plays an indistinctive role in the large CO₂ variation at SDZ, as it is weak during the non-growing season. The cold fronts pushed polluted air southeastward over the North China Plain and replaced it with low-CO₂ air from Northwest China, leading to the decline in CO₂. These findings demonstrate that mesoscale synoptic conditions significantly affect the regional transport and dispersion of CO₂, which can influence the prediction of terrestrial carbon balance on a regional scale.