In this research, a facile and effective approach was developed for the preparation of well-designed AuPd alloyed catalysts supported on magnetic halloysite nanotubes (HNTs@Fe₃O₄@AuPd). The microstructure and the magnetic properties of HNTs@Fe₃O₄@AuPd were confirmed by transmission electron microscopy (TEM), high resolution TEM (HRTEM), energy-dispersive X-ray spectroscopy (EDS), and vibrating sample magnetometry (VSM) analyses. The catalysts, fabricated by a cheap, environmentally friendly, and simple surfactant-free formation process, exhibited high activities during the reduction of 4-nitrophenol and various other nitroaromatic compounds. Moreover, the catalytic activities of the HNTs@Fe₃O₄@AuPd nanocatalysts were tunable via adjusting the atomic ratio of AuPd during the synthesis. As compared with the monometallic nanocatalysts (HNTs@Fe₃O₄@Au and HNTs@Fe₃O₄@Pd), the bimetallic alloyed HNTs@Fe₃O₄@AuPd nanocatalysts exhibited excellent catalytic activities toward the reduction of 4-nitrophenol (4-NP) to 4-aminophenol. Furthermore, the as-obtained HNTs@Fe₃O₄@AuPd can be recycled several times, while retaining its functionality due to the stability and magnetic separation property.