To further improve the performance of dielectric elastomer actuaotrs (DEAs), the development of novel elastomers with enhanced electro-mechanical properties is focal for the advancement of the technology. Hence, reliable techniques to assess their electro-mechanical performance are necessary. Characterization of the actuator materials is often achieved by fabricating circular DEAs with the pre-stretch of the membrane fixed by a stiff frame. Because of this set-up, the electrode size relative to the carrier frame’s dimension has an impact on actuator strain and displacement. To allow for comparable results across different studies, the influence of this effect needs to be quantified and taken into account. This paper presents an in-depth study of the active-to-passive ratio by proposing two simplified analytical models for circular DEA and comparing them. The first model is taking the hyperelastic material properties of the dielectric film into account while the second model is a linear elastic lumped parameter model based on the electro-mechanical analogy. Both models lie in good agreement and show a significant linear impact of the radial active-to-passive ratio on the electro-active strain and a resulting maximum of displacement around 50% radial coverage ratio. These findings are validated by experiments with actuators fabricated using silicone membranes. It is shown that the electrode size is not only an important parameter in the experimental design, but in some cases of higher significance for the accuracy of analytical models than the hyperelastic properties of the material. Furthermore, it could be shown that a radial coverage ratio of around 50% is desirable when measuring displacement as it maximizes the displacement and lowers the impact of deviations in electrode sizes due to fabrication errors.

There is increasing interest in the use of novel elastomers with inherent or modified advanced dielectric and mechanical properties, as components of dielectric elastomer actuators (DEA). This requires corresponding techniques to assess their electro-mechanical performance. A common way to test dielectric materials is the fabrication of actuators with pre-stretch fixed by a stiff frame. This results in the problem that the electrode size has an influence on the achievable actuator displacement and strain, which is detrimental to the comparability of experiments. This paper presents an in-depth study of the active-to-passive ratio with the aim of investigating the influence of the coverage ratio on uniaxial actuator displacement and strain. To model the effect, a simple lumped-parameter model is proposed. The model shows that the coverage ratio for maximal displacement is 50%. To validate the model results, experiments are carried out. For this, a rectangular, fiber-reinforced DEA is used to assess the relation of the coverage ratio and deformation. Due to the stiffness of the fibers, highly anisotropic mechanical properties are achieved, leading to the uniaxial strain behavior of the actuator, which allows the validation of the one-dimensional model. To consider the influence of the simplifications in the lumped-parameter model, the results are compared to a hyperelastic model. In summary, it is shown that the ratio of the active-to-passive area has a significant influence on the actuator deformation. Both the model and experiments confirm that an active-to-passive ratio of 50% is particularly advantageous in most cases.

In this study, we investigated the influence of an epoxy end-capped polypropylene oxide crosslinker (epoxy-PPO) on the formation of the crosslinked network structure, the stress–strain response, and the electro-mechanical actuation performance of a maleic anhydride functionalized liquid isoprene rubber (LIR). The crosslinker amount varied from 10 (C-LIR-10) to 50 (C-LIR-50) weight parts per hundred parts (phr) of LIR. The swelling test of the cured rubbers revealed that C-LIR-20 formed the densest crosslinked network with the lowest chloroform uptake value within this series. The crosslinked rubber became stiffer in tensile response upon increasing the epoxy-PPO amount from C-LIR-10 to C-LIR-20 and then softened at higher amounts. The SEM measurements were used to relate this composition-induced softening of the rubbers to the phase morphology evolution from nanoscale homogeneity in C-LIR-10 to microscale segregations of excess crosslinkers in C-LIR-50. The use of epoxy-PPO improved the dielectric constant value of LIR; however, the leakage current through the films also increased from 25 µA DC to 320 µA DC for LIR-30 and LIR-50, respectively, during DEA operation. The electro-mechanical actuation tests with circular actuators showed that the C-LIR-10 elastomer film demonstrated a radial strain of 1.7% on activation at an electric field strength of 17.5 V/µm. At higher crosslinker amounts, the close proximity of excess epoxy-PPO molecules caused leakage current across elastomer films thus diminishing the actuation strain of otherwise relatively softer elastomers with higher dielectric constant values.

Dielectric elastomer actuators (DEAs) are promising candidates for artificial muscle systems due to their lightweight structure, large deformation capabilities, and rapid response to electrical stimulation. This work investigates the electro-mechanical performance of cross-linked synthetic polychloroprene (CR), polyurethane (PUR), and hydrogenated acrylonitrile-butadiene rubbers (HNBR) as alternative dielectric elastomers (DEs) for DEAs. These elastomers demonstrated enhanced dielectric constants of ε r = 8.5 (CR), ε r = 6.4 (PUR), and ε r = 10 (HNBR) compared to ε r values of conventional DEs ε r = 2.3 (Elastosil 2030) and ε r = 4.7 (VHB 4910). Circular DEAs were manufactured to investigate the time-dependent actuation strain at a low excitation field strength of 16 V μm ⁻¹ . CR showed a response time of 1.2 s, indicating potential for fast-response applications. In contrast, the response time of PUR and HNBR is significantly higher (ca. 5 s) caused by a viscoelastic creep deformation. At a field strength of 16 V μm ⁻¹ the electro-active strain of all alternative DEs exceeds that of commercially Elastosil 2030. Among the alternative materials, HNBR exhibits the highest electro-active radial strain (2.2%) at the highest tested field strength of 26 V μm ⁻¹ . A linear-elastic model and a viscoelastic model were implemented in LTspice using electro-mechanical analogies to simulate the actuator behavior. While the linear model effectively estimated the strain magnitude, the viscoelastic model allowed a more accurate representation of the time-dependent actuation dynamics. The results highlight the potential of CR, PUR, and HNBR as viable alternatives for tailored DEA applications across varying actuation speed and strain requirements.