As a new laser-driven ion acceleration technique, we proposed a way to produce impurity-free, highly reproducible, and robust proton beams exceeding 100 MeV using a Coulomb explosion of micron-size hydrogen clusters. In this study, micron-size hydrogen clusters were generated by expanding the cooled high-pressure hydrogen gas into a vacuum via a conical nozzle connected to a solenoid valve cooled by a mechanical cryostat. The size distributions of the hydrogen clusters were evaluated by measuring the angular distribution of laser light scattered from the clusters. The data were analyzed mathematically based on the Mie scattering theory combined with the Tikhonov regularization method. The maximum size of the hydrogen cluster at 25 K and 6 MPa in the stagnation state was recognized to be 2.15 ± 0.10 μ m. The mean cluster size decreased with increasing temperature, and was found to be much larger than that given by Hagena’s formula. This discrepancy suggests that the micron-size hydrogen clusters were formed by the atomization (spallation) of the liquid or supercritical fluid phase of hydrogen. In addition, the density profiles of the gas phase were evaluated for 25 to 80 K at 6 MPa using a Nomarski interferometer. Based on the measurement results and the equation of state for hydrogen, the cluster mass fraction was obtained. 3D particles-in-cell (PIC) simulations concerning the interaction processes of micron-size hydrogen clusters with high power laser pulses predicted the generation of protons exceeding 100 MeV and accelerating in a laser propagation direction via an anisotropic Coulomb explosion mechanism, thus demonstrating a future candidate in laser-driven proton sources for upcoming multi-petawatt lasers.

The size of CO₂ clusters, produced in a supersonic expansion of a mixed-gas of CO₂/He or CO₂/H₂ through a three-staged conical nozzle designed based on the Boldarev's model, has been evaluated by measuring the angular distribution of light scattered from the clusters. The data are analyzed utilizing the Mie scattering theory, and the sizes of CO₂ clusters are estimated as 0.22 μm and 0.25 μm for the cases of CO₂/He and CO₂/H₂ gas mixtures, respectively. The results confirm that the Boldarev's model is reliable enough for the production of micron-sized clusters.

A detailed mathematical model is presented for a submicron-sized cluster formation in a binary gas mixture flowing through a three-staged conical nozzle. By measuring the angular distribution of light scattered from the clusters, the size of CO₂ clusters, produced in a supersonic expansion of the mixture gas of CO₂(30%)/H₂(70%) or CO₂(10%)/He(90%), has been evaluated using the Mie scattering method. The mean sizes of CO₂ clusters are estimated to be 0.28 ± 0.03 μm for CO₂/H₂ and 0.26 ± 0.04 μm for CO₂/He, respectively. In addition, total gas density profiles in radial direction of the gas jet, measuring the phase shift of the light passing through the target by utilizing an interferometer, are found to be agreed with the numerical modeling within a factor of two. The dryness (= monomer/(monomer + cluster) ratio) in the targets is found to support the numerical modeling. The apparatus developed to evaluate the cluster-gas targets proved that our mathematical model of cluster formation is reliable enough for the binary gas mixture.

The generation of highly charged ions in laser plasmas is usually associated with collisional ionization processes that occur in electron–ion collisions. An alternative ionization channel caused by tunnel ionization in an optical field is also capable of effectively producing highly charged ions with ionization potentials of several kiloelectronvolts when the laser intensity q > 10²⁰ W/cm². It is challenging to clearly distinguish the impacts of the optical field and collisional ionizations on the evolution of the charge state of a nonequilibrium plasma produced by the interaction of high-intensity, ultrashort PW-class laser pulses with dense matter. In the present work, it is shown that the answer to this question can be obtained in some cases by observing the X-ray spectral lines caused by the transition of an electron into the K-shell of highly charged ions. The time-dependent calculations of plasma kinetics show that this is possible, for example, if sufficiently small clusters targets with low-density background gas are irradiated. In the case of Ar plasma, the limit of the cluster radius was estimated to be R₀ = 0.1 μm. The calculation results for argon ions were compared with the results of the experiment at the J-KAREN-P laser facility at QST-KPSI.

We have investigated the formation, evolution, and late-time propagation of a laser-generated cylindrical blast wave (BW). The whole blast wave evolution over timescales of several nanoseconds was reconstructed experimentally (via temporally resolved interferometric measurements) and via hydrodynamic simulations that included modeling of nonlocal electron transport and radiation diffusion. Comparison between the experimental results and the simulations indicates that the early expansion phase is characterised by nonlocal electron heat transport causing energy spread on times shorter than the typical timescales for hydrodynamic expansion. Nonlocal electron transport ionizes the gas ahead of the plasma front and gives rise to a smooth radial density gradient. At later times, once the shock is launched and the BW is formed, radiation results in reduced shock velocity compared to the adiabatic case. These investigations provide a suitable and effective platform to benchmark the inclusion of kinetic and radiative effects in fluid modeling of the plasma dynamics over timescales that may be inaccessible to fully kinetic simulations.