Strong interaction between emitters and plasmonic nanocavity has various applications in quantum fields at room temperature. As Rabi oscillation gives the direct proof to the energy exchange in strong coupling, it is more intuitive and necessary to analyze the interaction in time domain. In this paper, we give the Rabi oscillation in a high-dissipation plasmonic nanocavity by using full-quantum method and draw a new strong coupling criterion about mode volume which provides a significant guidance in plasmonic nanocavitys nanofabrication. Moreover, we reveal the relation between Rabi oscillation and Rabi splitting, which is beneficial for exploring emitter–plasmon hybrid systems time-domain property through frequency-domain response. An emitter–hexagon hybrid system with ultrasmall mode volume is designed to verify our theory. The numerical simulation shows good agreements with our theoretical results. Our work has applications in quantum information and quantum computing in the future.
3 August 2021 in The Journal of Physical Chemistry C
High directional emission and high radiative quantum efficiency are strongly needed when moving a single optical nano-emitter (such as a quantum dot) into the practical realm. However, a typical optical nano-emitter struggles to meet the requirements above, which limits its practical applications in next-generation nano-photonic devices such as single-photon sources. Here, to achieve these features simultaneously, we propose and theoretically investigate a composite plasmonic antenna consisting of a hemispherical solid immersion lens (SIL) and a bowtie plasmonic nano-antenna, wherein a high directional emission of 10° and 2.5 × 103 of Purcell factor have both been enabled. Moreover, we find that directionality and the Purcell factor can be manipulated independently in our antenna, which provides a novel platform for the optimization of single-photon sources.