With the advancement of urbanization in China, effective control of pollutant emissions and air quality have become important goals in current environmental management. Nitrogen dioxide (NO₂), as a precursor of tropospheric ozone and fine particulate matter, plays a significant role in atmospheric chemistry research and air pollution control. However, the uneven ground monitoring stations and low temporal resolution of polar-orbiting satellites set challenges for accurately assessing near-surface NO₂ concentrations. To address this issue, a spatiotemporal refined NO₂ retrieval model was established for China using the geostationary satellite Himawari-8. The spatiotemporal characteristics of NO₂ were analyzed and its contribution factors were explored. Firstly, seven Himawari-8 channels sensitive to NO₂ were selected by using the forward feature selection based on information entropy. Subsequently, a 2DCNN-LSTM network model was constructed, incorporating the selected channels and meteorological variables as retrieval factors to estimate hourly NO₂ in China from March 2018 to February 2020 (with a resolution of 0.05°, per hour). The performance evaluation demonstrates that the full-channel 2DCNN-LSTM model has good fitting capability and robustness (R² = 0.74, RMSE = 10.93), and further improvements were achieved after channel selection (R² = 0.87, RMSE = 6.84). The 10-fold cross-validation results indicate that the R² between retrieval and measured values was above 0.85, the MAE was within 5.60, and the RMSE iwas within 7.90. R² varied between 0.85 and 0.90, showing better validation at mid-day (R² = 0.89) and in spring and fall transition seasons (R² = 0.88 and R² = 0.90). To investigate the cooperative effect of meteorological factors and other air pollutants on NO₂, statistical methods (beta coefficients) were used to test the factor interpretability. Meteorological factors as well as other pollutants were analyzed. From a statistical perspective, PM_2.5, boundary layer height, and O₃ were found to have the largest impacts on near-surface NO₂ concentrations, with each standard deviation change in these factors leading to 0.28, 0.24, and 0.23 in standard deviations of near-surface NO₂, respectively. The findings of this study contribute to a comprehensive understanding of the spatiotemporal distribution of NO₂ and provide a scientific basis for formulating targeted air pollution policies.

Precise cloud and aerosol identification hold paramount importance for a thorough comprehension of atmospheric processes, enhancement of meteorological forecasts, and mitigation of climate change. This study devised an automatic denoising cloud–aerosol classification deep learning algorithm, successfully achieving cloud–aerosol identification in atmospheric vertical profiles utilizing CALIPSO L1 data. The algorithm primarily consists of two components: denoising and classification. The denoising task integrates an automatic denoising module that comprehensively assesses various methods, such as Gaussian filtering and bilateral filtering, automatically selecting the optimal denoising approach. The results indicated that bilateral filtering is more suitable for CALIPSO L1 data, yielding SNR, RMSE, and SSIM values of 4.229, 0.031, and 0.995, respectively. The classification task involves constructing the U-Net model, incorporating self-attention mechanisms, residual connections, and pyramid-pooling modules to enhance the model’s expressiveness and applicability. In comparison with various machine learning models, the U-Net model exhibited the best performance, with an accuracy of 0.95. Moreover, it demonstrated outstanding generalization capabilities, evaluated using the harmonic mean F1 value, which accounts for both precision and recall. It achieved F1 values of 0.90 and 0.97 for cloud and aerosol samples from the lidar profiles during the spring of 2019. The study endeavored to predict low-quality data in CALIPSO VFM using the U-Net model, revealing significant differences with a consistency of 0.23 for clouds and 0.28 for aerosols. Utilizing U-Net confidence and a 532 nm attenuated backscatter coefficient to validate medium- and low-quality predictions in two cases from 8 February 2019, the U-Net model was found to align more closely with the CALIPSO observational data and exhibited high confidence. Statistical comparisons of the predicted geographical distribution revealed specific patterns and regional characteristics in the distribution of clouds and aerosols, showcasing the U-Net model’s proficiency in identifying aerosols within cloud layers.

With the advancement of urbanization in China, effective control of pollutant emissions and air quality have become important goals in current environmental management. Nitrogen dioxide (NO2), as a precursor of tropospheric ozone and fine particulate matter, plays a significant role in atmospheric chemistry research and air pollution control. However, the uneven ground monitoring stations and low temporal resolution of polar-orbiting satellites set challenges for accurately assessing near-surface NO2. To address this issue, a spatiotemporal refined NO2 retrieval model was established for China using the geostationary satellite Himawari-8. The spatiotemporal characteristics of NO2 were analyzed and its contribution factors were explored. Firstly, seven Himawari-8 channels sensitive to NO2 were selected by using the forward feature selection based on information entropy. Subsequently, a 2DCNN-LSTM network model was constructed, incorporating the selected channels and meteorological variables as retrieval factors to estimate hourly NO2 in China from March 2018 to February 2020 (with a resolution of 0.05°, per hour). The performance evaluation demonstrated that the full-channel 2DCNN-LSTM model had good fitting capability and robustness (R2=0.74, RMSE=10.93), and further improvements were achieved after channel selection (R2=0.87, RMSE=6.84). The 10-fold cross-validation results indicated that the R2 between retrieval and measured values was above 0.85, the MAE was within 5.60, and the RMSE was within 7.90. R2 varied between 0.85 and 0.90, showing better validation at mid-day (R2=0.89) and in spring and fall transition seasons (R2 =0.88 and R2 =0.90). To investigate the cooperative effect of meteorological factors and other air pollutants on NO2, statistical methods (Beta coefficients) were used to test the factor interpretability. Meteorological factors as well as other pollutants were analyzed. From a statistical perspective, PM2.5, Boundary Layer Height, and O3 were found to have the largest impacts on near-surface NO2, with each standard deviation change in these factors leading to 0.28, 0.24, and 0.23 in standard deviations of near-surface NO2, respectively. Findings of the study contribute to a comprehensive understanding of the spatiotemporal distribution of NO2 and provide a scientific basis for formulating targeted air pollution policies.