The local land use carbon budget (LUCB) balance is an important factor in achieving regional carbon neutrality. As the basic unit of China’s economic development and social governance, the county level is an important part of the realization of the “double carbon” goal. This paper focuses on 1069 county units within the Yangtze River Economic Belt (YREB). It utilizes data on land use, nighttime light, energy consumption, and social and economic factors to construct carbon emission models. The spatiotemporal characteristics of LUCB in these county units are analyzed using standard deviational ellipse (SDE) and spatial autocorrelation methods. Additionally, a zoning study is conducted by examining the economic contribution coefficient (ECC) of carbon emissions, the ecological support coefficient (ESC), and their coupling relationship. The results show that (1) the total land use carbon emissions (LUCE) increased significantly during the research period, and the total carbon sink was relatively stable. (2) The LUCB is spatially high in the east and low in the west, with the center of gravity moving to the southwest as a whole. (3) The LUCB shows positive spatial autocorrelation and has significant spatial agglomeration characteristics, which are mainly high–high and low–low regional agglomeration types. (4) The ECC is high in the east and low in the west, the ESC is high in the west and low in the east, and the coordination and coupling degrees of the two are low. (5) According to the ECC and ESC, the county unit is divided into a low-carbon conservation area, an economic development area, a carbon sink development area, and a comprehensive optimization area. This study is helpful in promoting the sustainable development of carbon neutrality and low carbon in the YREB.

With rapid industrialization and urbanization, the contradiction between the human exploitation of land production and living functions and natural ecosystem service functions has intensified. The issues of how to coordinate the exploitation and conservation functions of land and guide the rational distribution of human activities have become important for global sustainable development, especially considering the realization that multifunctional land use is an effective way to relieve land pressure and improve land use efficiency, that land multifunction has significant spatio-temporal heterogeneity, and that there is a mutual promotion and stress relationship between multifunctional land use. However, few existing studies have discussed the decoupling relationship among land use functions. In this study, a system of 10 sub-functions and 25 indicators was established based on the production function (PDF), living function (LVF), and ecological function (ELF) for 59 cities in the Yellow River Basin (YRB). There are both subjective and objective procedures employed to determine the weights, while an exploratory spatial data analysis is used to analyze the time-based and territorial changes in various functions of land use in the study area from 2000 to 2020. The decoupling relationship between the three functions is detected utilizing the theoretical foundation of the decoupling analysis. The results show that land use is multifunctional, LUFs develop unevenly, and their spatial distribution varies substantially. The results of the decoupling analysis demonstrate that the predominant types of correlations among the land use ELF and PDF and LVF over the research period are strong decoupling and strong negative decoupling correlations, with the former being a dilemma and the latter being a sustainable type of development.