Relaxor-lead titanate (PbTiO₃) crystals, which exhibit extremely high piezoelectricity, are believed to possess high electro-optic (EO) coefficients. However, the optical transparency of relaxor-PbTiO₃crystals is severely reduced as a result of light scattering and reflection by domain walls, limiting electro-optic applications. Through synergistic design of a ferroelectric phase, crystal orientation, and poling technique, we successfully removed all light-scattering domain walls and achieved an extremely high transmittance of 99.6% in antireflection film–coated crystals, with an ultrahigh EO coefficientr₃₃of 900 picometers per volt (pm V⁻¹), >30 times as high as that of conventionally used EO crystals. Using these crystals, we fabricated ultracompact EO Q-switches that require very low driving voltages, with superior performance to that of commercial Q-switches. Development of these materials is important for the portability and low driving voltage of EO devices.

We report a compact triple-band tunable perfect terahertz metamaterial absorber (TMA) at the subwavelength scale of thickness, which is composed of a planar metallic disk resonator array above a conductive ground plane separated with liquid crystal (LC) mixture. The calculations of terahertz absorption spectra demonstrate triple near-unity absorption bands in the gap plasmonic resonance coupling regime. Three resonance frequencies of the absorber exhibit continuous linear-tunability as changing the refractive index of LC. Remarkably, each peak absorbance of the triple bands maintains at a level of beyond 99% in the whole tuning operation, and the absorbance can remain more than 90% over a wide range of incident angles. Our work suggests that the LC tunable absorber scheme has the potential to overcome the basic difficulty to perform simultaneously multiband spectral tuning and near-unity absorbance with wide angle of incidence and weak polarization dependence. The proposed LC-tunable multiband perfect TMA is promising in the application of biomolecular spectra-selective terahertz imaging and sensing.

An ultrahigh electric field–induced strain of 0.9% (under 1 kV mm ⁻¹ ) is achieved in lead-free ferroelectric crystals.

We investigate narrowband transmission filters based on subwavelength-grating reflectors at normal incidence. Computational results show that the filtering is realized through symmetry-protected mode coupling. The guided mode resonances introduced by the slab layer allow flexible control of the filter frequencies. The quality factor of the filters could exceed 10⁶. Dielectric gratings can be used over the entire range of electromagnetic waves, owing to their scale-invariant operations. Owing to the high refraction index and low index dispersion of semiconductors in the infrared range, these filters can be applied over a broad range from near infrared to terahertz frequencies.