We investigate tunneling ionization of a model helium atom in a strong circularly polarized short laser pulse using the classical backpropagation method and compare ten different tunneling criteria on the same footing, aiming for a consistent classical picture of the tunneling dynamics. These tunneling criteria are categorized into velocity-based, position-based, and energy-based criteria according to different notions of a tunnel exit. We find that velocity-based criteria give consistent tunneling exit characteristics with nonadiabatic effects fully included. Other criteria are either inconsistent or only able to include nonadiabatic effects partially. Furthermore, we construct a simple tunneling rate formula, identify a term in the rate responsible for the nonadiabatic effects, and demonstrate the importance of this term.
Use of time delays in high-order-harmonic generation (HHG) driven by intense two-color, few-cycle pulses is investigated in order to determine means of optimizing HHG intensities and plateau cutoff energies. Based upon numerical solutions of the time-dependent Schrödinger equation for the H atom as well as analytical analyses, we show that introducing a time delay between the two-color, few-cycle pulses can result in an enhancement of the intensity of the HHG spectrum by an order of magnitude (or more) at the cost of a reduction in the HHG plateau cutoff energy. Results for both positive and negative time delays as well as various pulse carrier-envelope phases are investigated and discussed.
We present a theoretical analysis showing how chirp can be used to sculpt two-color driving laser field waveforms in order to enhance high-order harmonic generation (HHG) and/or extend HHG cutoff energies. Specifically, we consider driving laser field waveforms composed of two ultrashort pulses having different carrier frequencies in each of which a linear chirp is introduced. Two pairs of carrier frequencies of the component pulses are considered: () and (). Our results show how changing the signs of the chirps in each of the two component pulses leads to drastic changes in the HHG spectra. Our theoretical analysis is based on numerical solutions of the time-dependent Schrödinger equation and on a semiclassical analytical approach that affords a clear physical interpretation of how our optimized waveforms lead to enhanced HHG spectra.
An analytic description for the yield, , of high-energy electrons ionized from an atom by a short (few-cycle) laser pulse is obtained quantum mechanically. Factorization of in terms of an electron wave packet and the cross section for elastic electron scattering (EES) is shown to occur only for an ultrashort pulse, while in general involves interference of EES amplitudes with laser-field-dependent momenta. The analytic predictions agree well with accurate numerical results.
Ultrafast processes are now accessible on the attosecond time scale due to the availability of ultrashort XUV laser pulses. Noble-gas and halogen atoms remain important targets due to their giant dipole resonance and Cooper minimum. Here, we calculate photoionization cross section, asymmetry parameter and Wigner time delay using the time-dependent local-density approximation (TDLDA), which includes the electron correlation effects. Our results are consistent with experimental data and other theoretical calculations. The asymmetry parameter provides an extra layer of access to the phase information of the photoionization processes. We find that halogen atoms bear a strong resemblance on cross section, asymmetry parameter and time delay to their noble-gas neighbors. Our predicted time delay should provide a guidance for future experiments on those atoms and related molecules.